Themed collection Organic Electronics – Ecofriendly and/or sustainable materials, processes, devices, and applications

18 items
Editorial

Introduction to Organic Electronics – Ecofriendly and/or sustainable materials, processes, devices, and applications

Professor Gregory C. Welch introduces the Journal of Materials Chemistry C and Materials Advances joint themed collection on Organic Electronics – Ecofriendly and/or sustainable materials, processes, devices, and applications.

Graphical abstract: Introduction to Organic Electronics – Ecofriendly and/or sustainable materials, processes, devices, and applications
Review Article

Ubiquitous clean and sustainable energy-driven self-rechargeable batteries realized by and used in organic electronics

This article provides a review of various types of self-rechargeable batteries powered by ubiquitous clean and sustainable energy sources.

Graphical abstract: Ubiquitous clean and sustainable energy-driven self-rechargeable batteries realized by and used in organic electronics
Open Access Review Article

Advances in applying C–H functionalization and naturally sourced building blocks in organic semiconductor synthesis

This review presents the recent advances in the synthesis of organic semiconductors using C–H functionalization and naturally sourced building blocks to facilitate the large-scale production and commercialization of organic semiconductors.

Graphical abstract: Advances in applying C–H functionalization and naturally sourced building blocks in organic semiconductor synthesis
Review Article

Low-cost materials for organic solar cells

This review summarizes the recent advances in low-cost materials for OSCs from the aspects of the synthetic method, active materials, interfacial materials and processing solution.

Graphical abstract: Low-cost materials for organic solar cells
Review Article

Peptide-based novel small molecules and polymers: unexplored optoelectronic materials

Optoelectronic devices such as photovoltaics (solar cells), organic light-emitting diodes (OLEDs), thin-film transistors, and electrochromism based on peptide molecular/materials and their strategic design.

Graphical abstract: Peptide-based novel small molecules and polymers: unexplored optoelectronic materials
Communication

An air-stable n-type bay-and-headland substituted bis-cyano N–H functionalized perylene diimide for printed electronics

Design, synthesis, and characterization of an electron deficient N-H functionalized perylene diimide, with halogen-free solvent solubility, for air-stable transistor operation.

Graphical abstract: An air-stable n-type bay-and-headland substituted bis-cyano N–H functionalized perylene diimide for printed electronics
Open Access Paper

Phosphorus-modified Pt@Cu surfaces for efficient electrocatalysis of hydrogen evolution

Phosphorus-modified Pt@Cu (Pt/P@Cu) was fabricated through a one-step method as a self-standing electrocatalyst, leading to increased surface activity sites, reduced charge transfer resistance and enhanced HER performance in neutral medium.

Graphical abstract: Phosphorus-modified Pt@Cu surfaces for efficient electrocatalysis of hydrogen evolution
Paper

A phenothiazine-fused electroactive bilayer helicene: design, synthesis, ACQ-to-AIE transformation and photophysical properties

Study of the photophysical, electrochemical and photoconductive properties of SPS-PY-PT and a comparative analysis with PY-PT-Un. In addition, the ACQ and AIE phenomena and time-resolved microwave conductivity (TRMC) are analysed.

Graphical abstract: A phenothiazine-fused electroactive bilayer helicene: design, synthesis, ACQ-to-AIE transformation and photophysical properties
Open Access Paper

Self-assembly of PBTTT–C14 thin films in supercritical fluids

In order to develop more atom-economical deposition methods for polymer semiconductors, we investigated physical supercritical fluid deposition (p-SFD) to form thin films of a popular bithiophene semiconducting polymer (PBTTT).

Graphical abstract: Self-assembly of PBTTT–C14 thin films in supercritical fluids
Open Access Paper

Influence of pH-neutral lithium polystyrenesulfonate polyelectrolyte on the energy band structure and performance of organic solar cells

We investigate the effect of the polyelectrolyte lithium poly(styrene sulfonate) (Li:PSS) on the electronic band structure of organic solar cells and find that it functions as a hole transport layer, allowing improved efficiency and device stability.

Graphical abstract: Influence of pH-neutral lithium polystyrenesulfonate polyelectrolyte on the energy band structure and performance of organic solar cells
Open Access Paper

Chalcogen-substituted PCBM derivatives as ternary components in PM6:Y6 solar cells

Chalcogen-substituted PCBM derivatives are a promising approach to enhance power efficiency in ternary organic solar cells (TOSCs).

Graphical abstract: Chalcogen-substituted PCBM derivatives as ternary components in PM6:Y6 solar cells
Paper

Highly efficient hybrid light-emitting transistors incorporating MoOx/Ag/MoOx semi-transparent electrodes

Light-emitting transistors (LETs) couple the switching function of a transistor with the light-emitting function of LEDs. We demonstrate improved light out-coupling efficiency in LETs using oxide – metal – oxide type semitransparent electrodes.

Graphical abstract: Highly efficient hybrid light-emitting transistors incorporating MoOx/Ag/MoOx semi-transparent electrodes
Open Access Paper

2,9-Dibenzo[b,def]chrysene as a building block for organic electronics

A new series of three donor–acceptor conjugated polymers based on a low-cost, easily accessible vat dye called Vat orange 1 have been prepared. The polymers have bandgap values ranging from 1.61 to 1.86 eV.

Graphical abstract: 2,9-Dibenzo[b,def]chrysene as a building block for organic electronics
Open Access Paper

Temperature-dependent morphology-electron mobility correlations of naphthalene diimide-indacenodithiophene copolymers prepared via direct arylation polymerization

A series of defect-free n-type copolymers poly(naphthalene diimide-alt-indacenodithiophene) P(NDI-IDT) comprising alternating naphthalene diimide (NDI) and indacenodithiophene (IDT) units is prepared using atom-economic direct arylation polycondensation (DAP).

Graphical abstract: Temperature-dependent morphology-electron mobility correlations of naphthalene diimide-indacenodithiophene copolymers prepared via direct arylation polymerization
Paper

Improving the charge transport performance of solution-processed organic field-effect transistors using green solvent additives

Green solvent additives were employed as non-solvents in binary solvent systems to enable the pre-aggregation of organic semiconductors and enhance the electrical performance of organic field-effect transistors and complementary-like inverters.

Graphical abstract: Improving the charge transport performance of solution-processed organic field-effect transistors using green solvent additives
Open Access Paper

Synthesis of push–pull triarylamine dyes containing 5,6-difluoro-2,1,3-benzothiadiazole units by direct arylation and their evaluation as active material for organic photovoltaics

Direct (hetero)-arylation was used to prepare two push–pull molecules. Optimization of the experimental coupling conditions and their preliminary evaluation as active materials in simple air-processed organic solar cells are reported herein.

Graphical abstract: Synthesis of push–pull triarylamine dyes containing 5,6-difluoro-2,1,3-benzothiadiazole units by direct arylation and their evaluation as active material for organic photovoltaics
Open Access Paper

Fabrication of an autonomously self-healing flexible thin-film capacitor by slot-die coating

Flexible self-healing pressure sensors were prepared by slot-die onto a flexible substrate, and were characterized using multiple tools to investigate their response to mechanical deformation and their properties before and after self-healing.

Graphical abstract: Fabrication of an autonomously self-healing flexible thin-film capacitor by slot-die coating
Open Access Paper

Impact of subtle change in branched amino acid on the assembly and properties of perylene bisimides hydrogels

We investigate how apparent slight changes to the chemical structure of amino acid-functionalised perylene bisimides (PBIs) affect the self-assembled aggregates formed and their resulting physical and optical properties.

Graphical abstract: Impact of subtle change in branched amino acid on the assembly and properties of perylene bisimides hydrogels
18 items

About this collection

Guest Edited by Prof. Gregory C. Welch, University of Calgary.

Organic electronics is a fascinating field of study where conjugated materials can be tuned at the molecular scale to tailor properties for use in a myriad of advanced applications. Organic photovoltaics, transistors, light emitting didoes, photo detectors, batteries, supercapacitors, thermo electrics, and electrochromics are but a few technologies actively investigated.

This themed collection features articles from across this topic, including sustainable designs, atom-economical synthesis, green-solvent processing, low-power device operation, device bio-degradability/recyclability, up-scaling and next-generation applications for organic electronics in a sustainable world.

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