Themed collection Journal of Materials Chemistry A Emerging Investigators 2024
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Smart three-phase interface heterojunctions for effective photo(electro)catalytic N2 reduction to ammonia
Light-driven three-phase interface catalysts for the production of green ammonia as one of the key future energy carriers for the net-zero carbon landscape.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02540G
Synthesis and electrocatalytic applications of hybrid nanomaterials containing low-dimensional metals
In this review, recent progress in the synthesis and electrocatalytic applications of hybrid nanomaterials containing low-dimensional metals was outlined and some promising future directions were proposed.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02281E
Polythiophene and its derivatives for all-polymer solar cells
We review polythiophene and its derivative (PT)-based polymer donors for all-PSCs, focusing on material design, morphology optimization strategies, and the selection and design of polymer acceptors that complement their properties.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02245A
The revival of 4H-cyclopenta[2,1-b:3,4-b']dithiophene (CPDT) driven by low-cost and high-performance nonfused-ring electron acceptors
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02180K
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Thermoelectrics for Nuclear Fusion Reactors: Opportunities and Challenges
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02197E
Immobilization of metal active centers in reticular framework materials for photocatalytic energy conversion
To enhance the economy and society's sustainability, prioritizing innovative, green energy conversion methods is essential.
J. Mater. Chem. A, 2024,12, 12907-12925
https://doi.org/10.1039/D4TA01683A
Advanced polyanionic cathode materials for aqueous zinc-ion batteries: from crystal structures, reaction mechanisms, design strategies to future perspectives
This review summarizes the latest research progress in polyanionic cathodes for aqueous Zn-ion batteries from the perspectives of crystal structure, reaction mechanism, and design strategy, finally highlights potential challenges and future outlook.
J. Mater. Chem. A, 2024,12, 12926-12944
https://doi.org/10.1039/D4TA01290A
Designing low-strain cathode materials for long-life all-solid-state batteries
This review provides valuable insights and suggestions for future research on designing low-strain cathode materials for long-life and high-energy-density all-solid-state batteries under low external pressure conditions.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02290D
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Particulate gel liquid marble
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02203C
Realizing a single-phase reaction and K+/vacancy disordering in P2-K0.56Na0.11Li0.12Ni0.22Mn0.66O2 by lithium substitution for potassium-ion batteries
Through the electrochemical ion-exchange method, P2-K0.56Na0.11Li0.12Ni0.22Mn0.66O2 was successfully synthesized as a high-performance cathode with a single-phase reaction and K+/vacancy disordering for potassium-ion batteries.
J. Mater. Chem. A, 2024,12, 14360-14366
https://doi.org/10.1039/D4TA02122C
Bio-inspired sustained entrainment in immiscible liquid–liquid systems for collecting floating oil
Entrainment, where a solid object in a liquid bath moves towards the air phase, is common in industry and daily-life.
J. Mater. Chem. A, 2024,12, 11821-11830
https://doi.org/10.1039/D4TA00025K
Recognizing chiral amino acids with a dual-optical-response system
Histidine/tryptophan and their enantiomers were stepwise recognized by a dual-optical-response system, responding to fluorescence intensity variation and chiroptical activity regulation.
J. Mater. Chem. A, 2024,12, 9421-9426
https://doi.org/10.1039/D3TA07645H
Aluminium Doping to Single-Crystal Nickel-Rich Cathodes: Insights into Electrochemical Degradation and Enhancement
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02355B
Electrochemical reduction of nitrate to ammonia on ultra-stable amorphous Co–P electrocatalyst
Electrocatalytic reduction of nitrate (NO3−) to ammonia (NH3) is garnering increasing interest due to its potential to reduce CO2 emissions as a substitute for the Haber-Bosch process, while also mitigating NO3− pollution.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02299H
Tungstic acid integrated metal–organic frameworks for efficient oxygen evolution reaction
Mimicking the isolated and encapsulated active manganese sites within proteins in nature through the integration of NiFe sites and tungstic acid nanoparticles in an ordered open framework in an isolated manner.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02924K
Regulating catalytic kinetics in nanoclimbing-wall-like NiO/NiCoP hybrids for enhanced overall water splitting
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02232G
In situ growth of active catalytic layer on the commercial stainless steel via a hydrothermal-assisted corrosion process for efficient oxygen evolution reaction
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02234C
Chiromagnetic Co(OH)2 nanoparticles with high asymmetry for electrochemical recognition and detection of ascorbic acid enantiomers
Chiromagnetic Co(OH)2 nanoparticles with tunable asymmetry g-factors achieve AA chiral recognition and nM-level concentration detection.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02192D
Preparation of meso-porous aromatic frameworks for rapid ion extraction from high salt and corrosion environments
Silica nanoparticles were adopted as a template to synthesize mesoporous aromatic frameworks (meso-PAFs). They provide large channels for the transportation of uranyl ions, which give an adsorption capacity of 12.4 mg g−1 in 20 days from seawater.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02244K
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Beyond molecular structure: critically assessing machine learning for designing organic photovoltaic materials and devices
We assess state of machine learning for organic photovoltaic devices and data availability within the field, discuss best practices in representations and model selection, and release a comprehensive dataset of devices and fabrication conditions.
J. Mater. Chem. A, 2024,12, 14540-14558
https://doi.org/10.1039/D4TA01942C
Hydrogen-mediated acid-base transformation of Ni supported Mo5N6 for hydrogenative rearrangement of furfural derivatives
The hydrogenative rearrangement of bioderived furfural derivatives to various cyclopentanone derivatives is vital for synthesizing fine chemicals but challenging owing to the complex cascade reaction network.
J. Mater. Chem. A, 2024,12, 14531-14539
https://doi.org/10.1039/D4TA02076F
Synergistically coupling CoS/FeS2 heterojunction nanosheets on a MXene via a dual molten salt etching strategy for efficient oxygen evolution reaction
CoS/FeS2 heterojunction nanosheets on a MXene with excellent electrocatalytic OER performance are realized by a dual molten salt etching strategy.
J. Mater. Chem. A, 2024,12, 14517-14530
https://doi.org/10.1039/D4TA01999G
Constructing a robust artificial solid electrolyte interphase with a metal–organic framework for a stable Li metal anode
The metal–organic frameworks (MOFs) coating layer can promote homogeneous Li deposition.
J. Mater. Chem. A, 2024,12, 14408-14418
https://doi.org/10.1039/D4TA02158D
Semiconductor-cluster-loaded ionic covalent organic nanosheets with enhanced photocatalytic reduction reactivity of nitroarenes
A composite catalyst, developed by electrostatic self-assembly of anionic semiconductor clusters onto 2D cationic CONs, boosts photocatalytic selective nitroarene reduction through a strong internal electric field and the II-scheme mechanism.
J. Mater. Chem. A, 2024,12, 14398-14407
https://doi.org/10.1039/D4TA02087A
Boosting oxygen activation by CoP/carbon nitride photocatalyst in low-concentration H2S oxidation
The introduction of CoP could efficiently facilitate the electron transfer from CN towards O2 and enrich the production of ·O2−, which was indispensable in photocatalytic H2S oxidation.
J. Mater. Chem. A, 2024,12, 14508-14516
https://doi.org/10.1039/D4TA02258K
Thermal Properties and Lattice Anharmonicity of Li-ion Conducting Garnet Solid Electrolyte Li6.5La3Zr1.5Ta0.5O12
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02264E
A recrystallized organic cathode with high electrical conductivity for fast sodium-ion storage
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02302A
A steric hindrance-driven amorphization strategy on MOF/COF for boosting CO2 separation in mixed matrix membranes
The amorphous MOF/COF exposed Lewis basic sites and open metal sites in MMMs, improving the CO2/CH4 separation performance.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA01357C
Ligand-regulated Ni-based coordination compounds to promote self-reconstruction for improved oxygen evolution reaction
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03086A
Diluent-mediated interfacial reactions in localized-high-concentration electrolytes for fast-charging lithium-ion batteries
The “marionette” effect of various diluents in localized-high-concentration electrolytes subtly controls solvent and additive interactions and refines interfacial chemistry for enhancing Li-ion battery performance, particularly in extreme conditions.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02103G
Wrinkled Ir-MnOx nanospheres as pH-universal electrocatalysts for oxygen evolution reaction
Wrinkled Ir-doped manganese oxide (Ir-MnOx) nanospheres have been prepared via a facile metal–organic framework-directed strategy as pH-universal OER electrocatalysts.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02888K
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Harnessing a Ti-based MOF for selective adsorption and visible-light-driven water remediation
This study demonstrates the potential of a novel 2D-SBU COK-47-Ti MOF for visible-light-driven wastewater treatment through selective adsorption and photodegradation and shows its excellent performance superior to that of TiO2 and MIL-125-Ti.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA01967A
Amino acid salt induced PbI2 crystal orientation optimization for high-efficiency perovskite solar cells with long-term stability
By introducing potassium L-glutamate, residual PbI2 at the buried perovskite interface is eliminated, leading to enhanced photoelectric performance in perovskite solar cells.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02248C
Amphiphilic Janus patch-grafted hydrogels for salt-rejecting solar water desalination
The wettability of Janus hydrogel could be precisely regulated via modulating the amphiphilic Janus patch size and surface coverage to develop an excellent evaporator with a superior solar evaporation rate and salt ion rejection ratio.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02327G
Designing atomic Ni/Cu pairs on a reactive BiOCl surface for efficient photo-chemical HCO3−-to-CO conversion
Atomically dispersed Ni/Cu pairs on a BiOCl substrate were fabricated by a solvothermal method. The optimal sample (Ni1/Cu1-BOC) exhibited superior HCO3−R activity and CO selectivity, due to efficient charge transfer and HCO3− protonation.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02199A
Direct visualisation of metal–defect cooperative catalysis in a Ru-doped defective MOF-808
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA01689K
Fluoride Frameworks as Potential Calcium Battery Cathodes
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02426E
Facile synthesis of Fe3C/rGO via an in situ assembly route as an effective cocatalyst of Pt toward methanol electrooxidation
In this paper, the Pt–Fe3C/rGO catalyst is synthesized by an in situ assembly strategy. The strong interaction between Fe3C and Pt is favorable for boosting the methanol electrooxidation activity, CO anti-poisoning ability and remarkable stability.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA01995D
A multi-functional electrolyte additive for fast-charging and flame-retardant lithium-ion batteries
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02153C
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Designing rock salt phase enriched surface in Mn-based partially disordered spinel cathode materials for mitigating degradation in Li-ion batteries
A novel Mn-based Sp-DRX electrode engineered to initiate favorable early phase transitions, effectively delaying detrimental transitions to extend battery life.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02173H
Atomically Ordered Ir3Ti Intermetallics for pH-Universal Overall Water Splitting
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02304H
Wholly Degradable Quasi-Solid-State Thermocells for Low-Grade Heat Harvest and Precise Thermal Sensing
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02254H
Enabling Stable Aqueous Zn Metal Anodes by Scandium Acetate Electrolyte Additives
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02133A
Interfacial tuning of the graphite anode for potassium ion intercalation in a wide temperature range
An electrolyte design strategy is proposed for graphite anode in potassium-ion batteries working in a wide temperature range.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02499K
Substituted quinoxaline based small-molecule donor guests enable 19% efficiency ternary organic solar cells
Two novel guest molecules were designed and incorporated into the PM6:L8-BO system, which could enhance the crystallinity and optimize vertical phase distribution. Ternary OSCs achieved a remarkable PCE of 19.04% with enhanced stability.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02282C
Regulation of a Ni3Sn2 intermetallic catalyst using highly dispersed Pd species to boost propyne semi-hydrogenation
Introduction of highly dispersed Pd into well-regulated structures of a Ni3Sn2 intermetallic catalyst contributes to excellent catalytic performance for propyne semi-hydrogenation.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02342K
Low-coordinated Co–Mn diatomic sites derived from metal–organic framework nanorods promote electrocatalytic CO2 reduction
The diatomic L-Co1Mn1-NC catalyst, featuring low-coordinated Co/Mn centers on nanorod-shaped carbon, boosts CO2-to-CO conversion. Its unique microenvironment enhances d–d interaction and charge delocalization, facilitating CO desorption in the CO2RR.
J. Mater. Chem. A, 2024,12, 13694-13702
https://doi.org/10.1039/D4TA02261K
Intercalation pseudocapacitance of sodium-ion storage in TiO2(B)
Layered TiO2(B) displays intercalation pseudocapacitance for rapid Na+ storage, and the capacities and capacitor-like behaviors are independent of the surface area and morphology.
J. Mater. Chem. A, 2024,12, 13770-13777
https://doi.org/10.1039/D4TA02211D
Metal-free polymeric and molecular disorder/order semiconductor heterojunctions for the visible-light photocatalytic Minisci reaction
The PTCDA/g-C3N4 system, with three interfaces, not only effectively suppresses carrier recombination, facilitating the conversion of ˙O2− to 1O2, but also promotes the formation of products through the absorption of visible light.
J. Mater. Chem. A, 2024,12, 13760-13769
https://doi.org/10.1039/D4TA01440E
Multifunctional PMMA intermediate layer for sequentially deposited organic photovoltaics
Polymethyl methacrylate (PMMA) was optimally distributed vertically in the active layer through sequential deposition. With a maximum efficiency of 18.1%, OPVs based on PM6/PMMA/L8-BO outperformed PMMA-free devices.
J. Mater. Chem. A, 2024,12, 13751-13759
https://doi.org/10.1039/D4TA01335B
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The potential of zero charge and solvation effects on single-atom M–N–C catalysts for oxygen electrocatalysis
Ab initio molecular dynamics and DFT calculations are comprehensively performed to investigate the linear correlation between the point of zero charge, solvation effects, and the binding energy of HO* adsorption on single-atom catalyst surface.
J. Mater. Chem. A, 2024,12, 13742-13750
https://doi.org/10.1039/D4TA02285H
Bending two-dimensional Cu(I)-based coordination networks to inverse electrocatalytic HER/CO2RR selectivity
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA01982B
Plasmonic Cu-Ni bimetal nanoparticles coupled with ultrathin CdS nanosheet for remarkably improved photocatalytic H2 generation under visible-light irradiation
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02353F
Porous Cu/C Nanofibers Promote Electrochemical CO2-to-Ethylene Conversion via High CO2 Availability
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02358G
Germanium doping effect on the photoelectronic performance of alternating cations in the interlayer space GA(MA)3(Pb1−xGex)3I10
The pivotal role of Ge doping is found in finely adjusting the bandgap, enhancing carrier mobility, and improving optical-electronic properties and photovoltaic response.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02141J
Vampire bat's tongue-inspired superhydrophilic flexible origami channel for directional and spontaneous liquid manipulation
An improved bat-tongue-inspired superhydrophilic origami channel with liquid manipulation and collecting ability.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02252A
Self-supported Ni/Ni3N1−x heterostructures with abundant nitrogen vacancies as efficient electrocatalysts for ethylene glycol oxidation
Self-supported Ni/Ni3N1−x heterostructures with abundant nitrogen vacancies as efficient electrocatalysts for ethylene glycol oxidation.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02346C
Engineering modulated microscale assembly of MOF derived iron/nickel selenide for optimizing the oxygen evolution reaction
The macropores within carbon skeleton-supported FeSe2/NiSe2 derived from MOF assemblies are meticulously engineered at the micrometer scale and the OER electrocatalytic performance exhibits a significant dependence on the micrometer-scale dimensions.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02452D
Gate bias modulation towards organic electrochemical transistors with ultra-high cycling stability
The combination of appropriate gate bias and innovative structure design can significantly enhance the cycling stability of organic electrochemical transistors, which is crucial for controllable and extended lifetime of functional bioelectronics.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02276A
Morphology-enhanced piezoelectric performance of SnS nanobelts for acetaminophen degradation
This study reveals the enhanced piezoelectric activity of SnS nanobelts with step edges compared to nanobelts/nanoparticles and nanobelts, demonstrating superior catalytic performance for acetaminophen degradation in water.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02531H
Grafting a Rh–bipyridine complex on carbon nitride through coordination: ligand modification of single-atom Rh for enhanced CO2 reduction and inhibited H+ reduction
When 2,2′-bipyridine coordinates with a single atom Rh to form a single site Rh–bipyridine molecular cocatalyst, the hydrogen production rate is effectively inhibited and the CO generation is significantly increased.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA01974A
Self-assembled two-dimensional metal–organic framework membranes as nanofluidic osmotic power generators
2D ZnTCPP membranes with nanopores of 1.2 nm and interlayer spacing of 0.9 nm exhibit excellent osmotic power generation.
J. Mater. Chem. A, 2024,12, 13153-13159
https://doi.org/10.1039/D4TA01350F
A general strategy to prepare macro-/mesoporous materials from thermoplastic elastomer blends
This work demonstrates a simple method to prepare hierarchically porous materials. The introduction of macropores in mesoporous matrix enables its improved sorbent performance against pollutants for water remediation.
J. Mater. Chem. A, 2024,12, 13139-13152
https://doi.org/10.1039/D4TA01590H
The construction of a photocatalytic fuel cell based on piezoelectric-enhanced dual heterojunctions of PVDF–HFP supported 2D/3D composites toward photocatalytic degradation of tetracycline
Degradation sketch of a membrane fuel cell system constructed from I- and S-scheme heterojunction electrodes.
J. Mater. Chem. A, 2024,12, 13247-13265
https://doi.org/10.1039/D4TA01361A
Superhydrophilic covalent organic frameworks accelerate photocatalytic production of hydrogen peroxide through proton channels
Superhydrophilic COFs with D–A structure accelerate photocatalytic synthesis of H2O2 using water as a proton supply reservoir.
J. Mater. Chem. A, 2024,12, 13116-13126
https://doi.org/10.1039/D4TA01785D
Co–Co2C catalysts supported on carbon-coated ordered mesoporous silica with promoted CO insertion and C–C coupling for higher alcohol synthesis from syngas
Co–Co2C catalysts supported on carbon-coated ordered mesoporous silica showed superior performance for HAS than catalysts with uncoated and amorphous supports.
J. Mater. Chem. A, 2024,12, 13127-13138
https://doi.org/10.1039/D4TA01179A
Optimizing the active interface structure of MnO2 to achieve sustainable water oxidation in an acidic medium
Developing cost-effective electrocatalysts for the oxygen evolution reaction (OER) in proton exchange membrane (PEM) water electrolysis is crucial to achieving large-scale hydrogen production through water electrolysis.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02256D
A hybrid-aqueous biphasic electrolyte for suppressed shuttle effects and self-discharge of zinc bromide batteries
A strategy of using an ion-conductive biphasic electrolyte was adopted to suppress the shuttle effects of polybromides in Zn–Br2 batteries.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA01798F
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Phase stability and charge compensation in disordered rock salt compounds based on nickel and titanium
The synthesis of Ni/Ti disordered rock salt compounds (DRX) features the fast formation of a layered phase before the DRX structure becomes favored by entropy. Electrochemically the compounds exhibit significant structural and electronic hysteresis.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02265C
Sustainable design of non-fluorinated yet oleophobic fibrous surfaces
Fluorine-free oleophobic fabrics that can repel ethanol are demonstrated, but the fabric construction largely determines the capillary resistance and current wettability theory is only predictive for plain weave fabric structures.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA01659A
About this collection
Journal of Materials Chemistry A is pleased to present this themed collection highlighting the rising stars of materials chemistry research in 2023. This special collection showcases the very best work from materials chemists in the early stages of their independent career.
Each contributor was recommended by experts in their fields as carrying out work with the potential to influence future directions in materials chemistry with applications in energy and sustainability. Congratulations to all the outstanding researchers featured!
See also:
Journal of Materials Chemistry B Emerging Investigators 2024
Journal of Materials Chemistry C Emerging Investigators 2024