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The themed collection includes contributions from molecular inorganic chemists, biological chemists, electrochemists, and theoreticians who are working toward understanding and developing productive transformations of small molecules: dinitrogen, carbon dioxide, carbon monoxide, dihydrogen and dioxygen. Contributions will describe the activation of these molecules and, in particular, metal-mediated transformations of these small molecules such as reduction, oxidation, and bond forming and breaking events. This issue is Guest Edited by Louise A. Berben and Jason Love. New articles will be added to this collection as they are published.