Themed collection Journal of Materials Chemistry A Recent Review Articles
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Sustainable management of lead in perovskite solar cells
A closed-loop management of lead in perovskite solar cells (PSCs) during the device service life and at the end of life is highly essential that determines whether and how this technology can be commercialized.
J. Mater. Chem. A, 2022,10, 15861-15864
https://doi.org/10.1039/D2TA03081K
En route to artificial photosynthesis: the role of polyoxometalate based photocatalysts
The role of polyoxometalate (POM) based photocatalysts in the journey to couple CO2 reduction with water oxidation in a single integrated system provides a substantial contribution in achieving the goal of making artificial photosynthesis a reality.
J. Mater. Chem. A, 2022,10, 13152-13169
https://doi.org/10.1039/D2TA02243E
Towards predictive design of electrolyte solutions by accelerating ab initio simulation with neural networks
Ab initio molecular dynamics can be massively accelerated using equivariant neural networks applicable to predict the properties of electrolyte solutions for predictive design in materials applications.
J. Mater. Chem. A, 2022,10, 19560-19571
https://doi.org/10.1039/D2TA02610D
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Introducing porosity into metal–organic framework glasses
Here we document the reduction in porosity observed in MOFs upon their glass formation, propose routes to improve this porosity, and speculate on prospective future adsorptive applications.
J. Mater. Chem. A, 2022,10, 19552-19559
https://doi.org/10.1039/D2TA02560D
Atomistic insights into the morphology of deposited Li
In this perspective, we attempt to understand the morphology of deposited Li at the atomic level and establish the relationship between the morphology of the deposited Li and reversibility of Li plating/stripping.
J. Mater. Chem. A, 2022,10, 18577-18591
https://doi.org/10.1039/D2TA04974K
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On the challenges of materials and electrochemical characterization of concentrated electrolytes for redox flow batteries
We highlight the status of, and propose future approaches for, rheological, electrochemical, and spectroscopic characterization of concentrated redoxmer electrolytes for energy storage, with an emphasis on nonaqueous redox flow batteries.
J. Mater. Chem. A, 2022,10, 17988-17999
https://doi.org/10.1039/D2TA00690A
Transport tuning strategies in MOF film synthesis – a perspective
Metal–organic frameworks (MOFs), sometimes also known as coordination polymers, are a very versatile group of materials consisting of metal nodes and organic linkers forming a tunable porous structure that can exist in different structural phases.
J. Mater. Chem. A, 2022,10, 14641-14654
https://doi.org/10.1039/D2TA03216C
Can perovskites be efficient photocatalysts in organic transformations?
Designing and developing efficient, robust, and cost-effective photocatalysts that can support a broad scope of chemical bond formations (C–C, C–N, C–O, and C–P) is need of the hour for the emergence of next generation viable technologies.
J. Mater. Chem. A, 2022,10, 12317-12333
https://doi.org/10.1039/D1TA09383E
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iR drop correction in electrocatalysis: everything one needs to know!
This perspective details every single aspects of iRu drop correction in controlled-potential electrocatalysis from fundamentals to the best practices.
J. Mater. Chem. A, 2022,10, 9348-9354
https://doi.org/10.1039/D2TA01393B
Recent advances in oriented metal–organic frameworks for supercapacitive energy storage
The recent advances in oriented MOFs as electrode materials and solution to poor conductivity as well as random orientations have been discussed.
J. Mater. Chem. A, 2022,10, 4475-4488
https://doi.org/10.1039/D1TA10213C
Strategies for designing more efficient electrocatalysts towards the urea oxidation reaction
In this perspective, five typical strategies are summarized for designing highly active electrocatalysts towards the urea oxidation reaction (UOR).
J. Mater. Chem. A, 2022,10, 3296-3313
https://doi.org/10.1039/D1TA09989B
Rational catalyst design for spatial separation of charge carriers in a multi-component photocatalyst for effective hydrogen evolution
This manuscript comprehensively reviews the effect of spatial separation of charge carriers and novel strategies to achieve spatially separated active sites for enhancing photocatalytic hydrogen evolution over different photocatalyst systems.
J. Mater. Chem. A, 2022,10, 25380-25405
https://doi.org/10.1039/D2TA06609B
Metal-related electrocatalysts for Li–CO2 batteries: an overview of the fundamentals to explore future-oriented strategies
This work comprehensively introduces recent innovative work on metal-related electrocatalysts for Li–CO2 batteries.
J. Mater. Chem. A, 2022,10, 25406-25430
https://doi.org/10.1039/D2TA05756E
Mechanistic insights into metal, nitrogen doped carbon catalysts for oxygen reduction: progress in computational modeling
Computational modeling has been used to acquire knowledge of the active site structure, reaction kinetics, and stability of metal, nitrogen co-doped carbon electrocatalysts, which exhibit encouraging activity for oxygen reduction reaction.
J. Mater. Chem. A, 2022,10, 23959-23972
https://doi.org/10.1039/D2TA05991F
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Spatioselective surface chemistry for the production of functional and chemically anisotropic nanocellulose colloids
In this review, we explain the influence and role of the multiscale hierarchy of cellulose fibers in their chemical modifications as exemplified through recent advances in the spatioselective surface chemistry of nanocelluloses.
J. Mater. Chem. A, 2022,10, 23413-23432
https://doi.org/10.1039/D2TA05277F
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Insights into sustainable aerogels from lignocellulosic materials
Aerogels have been considered to be revolutionary solid-state materials due to their highly porous structure, low density, large surface area, and low thermal conductivity, which can be applied in the many modern fields of industry.
J. Mater. Chem. A, 2022,10, 23467-23482
https://doi.org/10.1039/D2TA04994E
Advanced preparation and application of transition metal selenides in lithium–sulfur batteries: a review
In this review, we systematically summarize the working mechanism in the cycle process of the batteries, the preparation ways, the research progress and future developments of transition metal selenides in Li–S cells.
J. Mater. Chem. A, 2022,10, 23433-23466
https://doi.org/10.1039/D2TA05576G
Underlying physics and chemistry of ferroic-photocatalysis: a critical review
The significance of ferroelectric and ferroelastic materials physico-chemistry is summarized and detailed for various photocatalytic reactions, followed by an outlook on future advancements.
J. Mater. Chem. A, 2022,10, 22977-22991
https://doi.org/10.1039/D2TA05294F
Advanced electrolyte systems with additives for high-cell-voltage and high-energy-density lithium batteries
Given that battery-powered electric vehicles and other power equipment put forward higher requirements for long recharge mileage, the development of high-performance lithium batteries (LBs) has become necessary.
J. Mater. Chem. A, 2022,10, 22929-22954
https://doi.org/10.1039/D2TA07696A
NaK alloy: underrated liquid metal
Liquid metals are poised to become vital for numerous challenges in materials science. However, the sodium–potassium liquid alloy (NaK) is severely underutilized. Meanwhile, it has exceptional physical and chemical properties and deserves more attention.
J. Mater. Chem. A, 2022,10, 22955-22976
https://doi.org/10.1039/D2TA06882F
Molecular structure-controlled synthesis of sulfur-containing polymers for rechargeable Li–S batteries
Strategies for the molecular structure-controlled synthesis of sulfur polymers used in Li–S batteries are summarized, thus presenting the opportunities and challenges for the development of sulfur polymers in the future.
J. Mater. Chem. A, 2022,10, 22896-22914
https://doi.org/10.1039/D2TA06500B
Metal-doping of halide perovskite nanocrystals for energy and environmental photocatalysis: challenges and prospects
This review summarized the characteristics of halide perovskite nanocrystals in photocatalytic applications. Critical insights are also provided into the existing challenges and prospects for these photocatalysts in photocatalytic applications.
J. Mater. Chem. A, 2022,10, 22915-22928
https://doi.org/10.1039/D2TA06851F
Shaping techniques of adsorbents and their applications in gas separation: a review
This paper reviews recent advances in the shaping adsorbents: alternative geometric forms, key metrics for evaluation, typical steps of main shaping techniques, etc., are discussed, which can serve as a reference for structured adsorbent design.
J. Mater. Chem. A, 2022,10, 22853-22895
https://doi.org/10.1039/D2TA04352A
Atomically dispersed metal catalysts for the electrochemical nitrogen reduction reaction
The current breakthroughs in designing atomically dispersed metal catalysts for the electrochemical N2 reduction reaction are summarized from both experimental and theoretical points of view. The outstanding performances of these catalysts are emphasized.
J. Mater. Chem. A, 2022,10, 22331-22353
https://doi.org/10.1039/D2TA06187B
Doping engineering: modulating the intrinsic activity of bifunctional carbon-based oxygen electrocatalysts for high-performance zinc–air batteries
Bifunctional carbon-based oxygen electrocatalysts in Zinc–air batteries. .
J. Mater. Chem. A, 2022,10, 21797-21815
https://doi.org/10.1039/D2TA05914B
Rational design, application and dynamic evolution of Cu–N–C single-atom catalysts
This review summarizes the recent research progress on the preparation strategy, regulation mechanism of the coordination environment, catalytic performance and dynamic evolution process of Cu–N–C single-atom catalysts.
J. Mater. Chem. A, 2022,10, 21769-21796
https://doi.org/10.1039/D2TA06050G
Vanadium-free NASICON-type electrode materials for sodium-ion batteries
Sodium-ion batteries (SIBs) have been rapidly developed as an effective replacement or supplement for lithium-ion batteries (LIBs) due to the high natural abundance and low cost of sodium resources.
J. Mater. Chem. A, 2022,10, 21816-21837
https://doi.org/10.1039/D2TA05653D
Emerging two-dimensional nanostructured manganese-based materials for electrochemical energy storage: recent advances, mechanisms, challenges, and prospects
The review summarizes the progress of emerging 2D manganese-based materials as advanced electrode materials for EES.
J. Mater. Chem. A, 2022,10, 21197-21250
https://doi.org/10.1039/D2TA05309H
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Covalent organic framework supported palladium catalysts
Covalent organic frameworks (COFs), as highly porous crystalline structures, are newly emerging materials designed with tuneable features.
J. Mater. Chem. A, 2022,10, 20707-20729
https://doi.org/10.1039/D2TA05234B
Redox-induced thermocells for low-grade heat harvesting: mechanism, progress, and their applications
In this paper, we provide a comprehensive description of redox-induced thermocells, including the mechanism, progress, and applications.
J. Mater. Chem. A, 2022,10, 20730-20755
https://doi.org/10.1039/D2TA05742E
Recent advancement in heterogeneous CO2 reduction processes in aqueous electrolyte
This review provides an in-depth general overview on various types of heterogeneous CO2 reduction in aqueous phase with a detailed discussion on EC, PEC and PV-EC/PEC processes including a thorough coverage on the futuristic MEA system.
J. Mater. Chem. A, 2022,10, 20667-20706
https://doi.org/10.1039/D2TA03441G
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Electronic structure engineering for electrochemical water oxidation
Strategies for regulating the electronic structure of transition-metal-based electrocatalysts through doping, heterostructure, oxygen vacancies, alloy, and strain engineering are investigated.
J. Mater. Chem. A, 2022,10, 20218-20241
https://doi.org/10.1039/D2TA04833G
Current research situation and future prospect of superwetting smart oil/water separation materials
Smart materials with convertible wettability interfaces enable to sustainably treat oil spills and purify oily wastewater.
J. Mater. Chem. A, 2022,10, 20190-20217
https://doi.org/10.1039/D2TA04469B
2D non-carbide MXenes: an emerging material class for energy storage and conversion
This review provides a comprehensive overview of the synthesis, properties, applications, current challenges, and the prospects of non-carbide MXenes, viz., carbonitride and nitride MXenes.
J. Mater. Chem. A, 2022,10, 20174-20189
https://doi.org/10.1039/D2TA05392F
Recent advancements in poly-Si/SiOx passivating contacts for high-efficiency silicon solar cells: technology review and perspectives
The paper provides an outline of the present status in lab and industry of TOPCon structure. Additionally, this review discusses the remaining hurdles and the promise with the aim of providing guidance for the development of TOPCon solar cells.
J. Mater. Chem. A, 2022,10, 20147-20173
https://doi.org/10.1039/D2TA04730F
Two-dimensional carbide/nitride (MXene) materials in thermal catalysis
In this article, we systematically summarize MXenes as both catalysts and supports in thermal catalysis, emphasizing the termination groups, active sites, and the metal–MXene interactions.
J. Mater. Chem. A, 2022,10, 19444-19465
https://doi.org/10.1039/D2TA03481F
Approaching a stable oxygen redox reaction in lithium-rich cathode materials: structural perspectives from mechanism to optimization
We review the oxygen redox reaction in lithium-rich cathodes from structural perspectives. The structure–OR coupling, structural evolution, and efficient structural control strategies are introduced, followed by an outlook on future rational design.
J. Mater. Chem. A, 2022,10, 19387-19411
https://doi.org/10.1039/D2TA02228A
Advances in understanding and regulation of sulfur conversion processes in metal–sulfur batteries
The fundamental understanding and rational regulation of effective metal–sulfur conversion reactions in metal–sulfur batteries.
J. Mater. Chem. A, 2022,10, 19412-19443
https://doi.org/10.1039/D2TA02217F
Spin-polarized excitons and charge carriers in chiral metal halide semiconductors
Introducing chirality into metal halide semiconductors brings spin-polarized charges and excitons, exotic chiroptical and spintronic properties, as well as application potential in optoelectronics and spintronics devices.
J. Mater. Chem. A, 2022,10, 19367-19386
https://doi.org/10.1039/D2TA02207A
Current state-of-the-art characterization methods for probing defect passivation towards efficient perovskite solar cells
Several advanced characterization methods used for defect passivation were reviewed, including capacitance measurements, spectrometry and microscopy characterizations, as well as some newly applied in situ techniques.
J. Mater. Chem. A, 2022,10, 19278-19303
https://doi.org/10.1039/D2TA02263J
Development of catalysts and electrolyzers toward industrial-scale CO2 electroreduction
Here we summarize the recent developments of catalysts and electrolyzers for the CO2 reduction reaction, which have improved product selectivity and enabled the delivery of industrial-scale current densities.
J. Mater. Chem. A, 2022,10, 19254-19277
https://doi.org/10.1039/D2TA02086F
Recent strategies for activating the basal planes of transition metal dichalcogenides towards hydrogen production
The currently strategies for activating the TMDC basal planes toward hydrogen evolution reaction were summarized, which are divided into internal and external regulation, depending on whether the pristine structure is altered or not.
J. Mater. Chem. A, 2022,10, 19067-19089
https://doi.org/10.1039/D2TA02458F
Manganese-based layered oxides for electrochemical energy storage: a review of degradation mechanisms and engineering strategies at the atomic level
In this review, particular attention is focused on the atomic degradation mechanisms of Mn-based layered oxide materials induced by the Jahn–Teller effect and the manipulative strategies for structural stability are highlighted.
J. Mater. Chem. A, 2022,10, 19231-19253
https://doi.org/10.1039/D2TA02242G
Reactive oxygen species on transition metal-based catalysts for sustainable environmental applications
We highlight the defect engineering of transition metal catalysts to tailor reactive oxygen species in advanced oxidation processes in a controlled manner for sustainable environmental applications.
J. Mater. Chem. A, 2022,10, 19184-19210
https://doi.org/10.1039/D2TA02188A
Carbon nanomaterials–polymer composites for perovskite solar cells: preparation, properties and applications
An overview of carbon–polymer nanocomposites for perovskite solar cells.
J. Mater. Chem. A, 2022,10, 19211-19230
https://doi.org/10.1039/D2TA02175G
Understanding (photo)electrocatalysis for the conversion of methane to valuable chemicals through partial oxidation processes
The review overviews the mechanism of C–H activation through electron–hole mediated pathways in photo and electrocatalysis, and introduces various strategies to increase the conversion of CH4 as well as the selectivity to desired products.
J. Mater. Chem. A, 2022,10, 19107-19128
https://doi.org/10.1039/D2TA02257E
Organic electrolyte design for practical potassium-ion batteries
In this review, recent electrolyte design strategies and progress are given, along with the discussion of relative key features and properties, as well as the practical design and considerations.
J. Mater. Chem. A, 2022,10, 19090-19106
https://doi.org/10.1039/D2TA02223K
Quasi-2D halide perovskite crystals and their optoelectronic applications
The unique semiconductor properties, synthetic strategies, and corresponding optoelectronic applications of quasi-2D halide perovskite crystals are summarized and discussed in this review.
J. Mater. Chem. A, 2022,10, 19169-19183
https://doi.org/10.1039/D2TA02219B
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Controlled local orientation of 2D nanomaterials in 3D devices: methods and prospects for multifunctional designs and enhanced performance
The review provides the recent progress in the processing of functional devices using oriented 2D nanomaterials and highlights the alignment strategies that contributed to the enhancement of device performance.
J. Mater. Chem. A, 2022,10, 19129-19168
https://doi.org/10.1039/D2TA01926D
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Perovskites: weaving a network of knowledge beyond photovoltaics
In this review we highlight the benefits of perovskites beyond photovoltaic technology, focusing on their use as lasers, light-emitting diodes or sensors, including technologies such as gamma-ray detection or aerospace applications.
J. Mater. Chem. A, 2022,10, 19046-19066
https://doi.org/10.1039/D2TA01135B
Recent advances in structural regulation and optimization of high-performance solar-driven interfacial evaporation systems
The latest advances in the synthesis and structural regulation of photothermal nanomaterials, the construction and optimization of interfacial evaporators, and the innovative design of solar-driven interfacial evaporation systems are introduced.
J. Mater. Chem. A, 2022,10, 18509-18541
https://doi.org/10.1039/D2TA05666F
It takes two: advances in employing the interactions between black phosphorous and metals in various applications
The two-dimensional black phosphorus can interact with metal compounds to form BP–M composites, showing tailored properties. This review summarizes BP–Ms in different applications, revealing the challenges and prospects of this composite material.
J. Mater. Chem. A, 2022,10, 18490-18508
https://doi.org/10.1039/D2TA05490F
Recent advances of crosslinkable organic semiconductors in achieving solution-processed and stable optoelectronic devices
Crosslinkable organic semiconductors in optoelectronic devices have attracted extensive attention due to the outstanding advantages of strong solvent resistance and stable film morphology.
J. Mater. Chem. A, 2022,10, 18542-18576
https://doi.org/10.1039/D2TA05358F
Solar-driven interfacial evaporation for water treatment: advanced research progress and challenges
Solar-driven interface evaporation, with photothermal materials as the core component, has an excellent seawater desalination effect and potential application prospect in the field of water treatment.
J. Mater. Chem. A, 2022,10, 18470-18489
https://doi.org/10.1039/D2TA03321F
Graphene oxide as a versatile platform for emerging hydrovoltaic technology
Graphene oxide has been demonstrated as a promising platform for hydrovoltaic technology. A wide variety of GO-based hydrovoltaic materials with distinctly different morphological, mechanical and functional features have been created.
J. Mater. Chem. A, 2022,10, 18451-18469
https://doi.org/10.1039/D2TA04830B
Tailoring the selectivity and activity of oxygen reduction by regulating the coordination environments of carbon-supported atomically dispersed metal sites
This review discloses the controllable ORR selectivity and activity based on the coordination environment regulation of the carbon supported atomically dispersed metal sites (C-ADMSs).
J. Mater. Chem. A, 2022,10, 17948-17967
https://doi.org/10.1039/D2TA05110A
Fused ring A–DA′D–A (Y-series) non-fullerene acceptors: recent developments and design strategies for organic photovoltaics
The fundamental principles of the molecular design of Y-series NFAs (A–DA′D–A) are described, together with their achievements, comprehension, and impact on the photoelectric characteristics, photovoltaic performance, and film morphology.
J. Mater. Chem. A, 2022,10, 17968-17987
https://doi.org/10.1039/D2TA04501J
Recent advances in microporous metal–organic frameworks as promising adsorbents for gas separation
We herein not only provide a comprehensive overview of the most important advances in the development of MOFs as separating materials for gas separation over the last five years, but also provide an update of the current challenges in this active field.
J. Mater. Chem. A, 2022,10, 17878-17916
https://doi.org/10.1039/D2TA04835C
In situ characterization of lithium-metal anodes
In situ characterization, as a real-time monitoring method, is used to address various issues in Li metal anodes.The application of in situ characterization helps to promote the further commercialization of Li-metal batteries.
J. Mater. Chem. A, 2022,10, 17917-17947
https://doi.org/10.1039/D2TA04309B
Aerogels in passive solar thermal desalination: a review
Driven by renewable energy, solar-thermal technology holds promising potential for effective freshwater production with a reduced carbon footprint.
J. Mater. Chem. A, 2022,10, 17857-17877
https://doi.org/10.1039/D2TA05216D
Reaction mechanism and selectivity regulation of photocatalytic nitrate reduction for wastewater purification: progress and challenges
The excess emission of nitrate into wastewater is inevitable by the abundant use of fertilizers and other chemicals, which poses a huge threat to the environment and human health.
J. Mater. Chem. A, 2022,10, 17357-17376
https://doi.org/10.1039/D2TA04611C
Structural design and control of photocatalytic nitrogen-fixing catalysts
In this paper, we mainly discuss the structure and design of photocatalytic nitrogen-fixing materials, such as introducing various vacancies on the catalyst surface, conducting element doping and constructing heterojunctions.
J. Mater. Chem. A, 2022,10, 17377-17394
https://doi.org/10.1039/D2TA03977J
Emerging green technologies for recovery and reuse of spent lithium-ion batteries – a review
We introduce recycling mechanisms and emerging green recycling technologies related to spent LIBs. We propose a new system to evaluate the environmental indicators of different recycling methods, the prospects and directions of spent Li recycling.
J. Mater. Chem. A, 2022,10, 17053-17076
https://doi.org/10.1039/D2TA03295C
Marine polysaccharide-based electromagnetic absorbing/shielding materials: design principles, structure, and properties
An investigation of design principles, preparation processes and structural properties is carried out to predict the development tendency of marine polysaccharide-based electromagnetic response materials which cater to the current targeted demands.
J. Mater. Chem. A, 2022,10, 17023-17052
https://doi.org/10.1039/D2TA03529D
Ammonia borane as an efficient direct fuel in alkaline fuel cells: mechanism, catalysts, applications, and challenges
Ammonia borane as an efficient direct fuel in alkaline fuel cells: mechanism, catalysts, applications, and challenges.
J. Mater. Chem. A, 2022,10, 16779-16794
https://doi.org/10.1039/D2TA03062D
Recent advances of non-lithium metal anode materials for solid-state lithium-ion batteries
This review, for the first time, systematically summarizes the application of C, Si, Sn, Bi, metal hydrides and lithium titanate as anode materials in solid-state lithium batteries.
J. Mater. Chem. A, 2022,10, 16761-16778
https://doi.org/10.1039/D2TA03905B
Fibrous triboelectric nanogenerators: fabrication, integration, and application
The recent progress in fibrous triboelectric nanogenerators (F-TENGs) is comprehensively introduced, with a special focus on their different fabrication techniques.
J. Mater. Chem. A, 2022,10, 15881-15905
https://doi.org/10.1039/D2TA03813G
MBenes: progress, challenges and future
The synthesis methods, properties and applications for energy storage and electrocatalysis of MBenes were summarized. Furthermore, discussions and perspectives on the existing problems, major challenges and future development of MBenes were provided.
J. Mater. Chem. A, 2022,10, 15865-15880
https://doi.org/10.1039/D2TA03482D
Multifunctional materials for photo-electrochemical water splitting
The rise in world pollution and energy demand has aggravated the energy crisis and depletion of non-renewable energy resources. Here, we review multifunctional materials that can be used for photoelectrochemical water splitting for clean energy production.
J. Mater. Chem. A, 2022,10, 15906-15931
https://doi.org/10.1039/D2TA01869A
Emerging ruthenium single-atom catalysts for the electrocatalytic hydrogen evolution reaction
Synthesis strategies, characterization methods, and various supports for Ru-based single-atom catalysts and their HER performance are reviewed.
J. Mater. Chem. A, 2022,10, 15370-15389
https://doi.org/10.1039/D2TA03860A
About this collection
This collection contains recent Review-type articles published by Journal of Materials Chemistry A, the home for high impact applications, properties and synthesis of exciting new materials for energy and sustainability. New articles will be added to this collection as soon as possible after publication.