Issue 7, 2024

High precision and fast classification of different dimensions of Baijiu using an OptGSCV quadratic optimization network combined with AS-LIBS

Abstract

Aiming to tackle the problems of low classification accuracy, difficult data processing, long analysis time, and the influence of subjective consciousness of traditional Baijiu (Chinese liquor), this paper reports a method based on the combination of laser-induced breakdown spectroscopy with high-frequency ultrasonic atomization system (AS-LIBS) and optimized grid search cross validation (Opt-GSCV) for high-precision and rapid classification of Baijiu of different dimensions. Multi-dimensional high-precision classification of 23 Baijiu samples with different series, degrees, and production dates from Shanxi Xinghuacun Fen Wine Factory Co., Ltd was performed. By studying the growth and evolution mechanism of plasma generated by laser excitation, a new method of Baijiu spectral signal acquisition was realized by combining LIBS with Baijiu detection. Aiming at addressing the shortcomings of high breakdown thresholds and poor signal stability due to the direct breakdown of Baijiu with high ethanol content, a high-frequency atomization system based on ultrasonic technology is proposed to realize the efficient extraction of Baijiu plasma spectral signals. With regard to the selection of the number of nodes, weights and thresholds of the implicit layer of the back-propagation (BP) network, an optimization model based on the combination of the particle swarm optimization (PSO) algorithm combined with the genetic algorithm (GA) is proposed to realize the construction of the BP optimal network architecture. By constructing a secondary optimization seeking network model based on OptGSCV, the technical problem of mismatch between optimal parameter selection and optimal network construction is solved, and a new network integrating an intelligent qualitative analysis algorithm and a traditional classification algorithm is realized. The experimental results show that the proposed OptGSCV quadratic optimization network combined with the AS-LIBS multidimensional Baijiu high-precision classification model not only introduces an innovative and high-efficiency detection method for the Baijiu industry, but also provides important technical support and new ideas for the key areas of food safety production and Baijiu quality control.

Graphical abstract: High precision and fast classification of different dimensions of Baijiu using an OptGSCV quadratic optimization network combined with AS-LIBS

Article information

Article type
Paper
Submitted
20 ก.พ. 2567
Accepted
25 เม.ย. 2567
First published
20 พ.ค. 2567

J. Anal. At. Spectrom., 2024,39, 1789-1802

High precision and fast classification of different dimensions of Baijiu using an OptGSCV quadratic optimization network combined with AS-LIBS

H. Jin, X. Hao, N. Li, Y. Han, B. Mo and S. Zhang, J. Anal. At. Spectrom., 2024, 39, 1789 DOI: 10.1039/D4JA00062E

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