We report a base-catalysed synthesis of substituted pyridines from α,β-unsaturated ketones (or arylmethylketones) and N-(4H-1,2,4-triazol-4-yl)imines, where the latter serve as both an N-source and a building block. This versatile protocol provides access to 2,4,6-triarylpyridines, 2,4-diaryl-5-methylpyridines, 5-methylpyridines, and alicyclic [b]-fused pyridines.
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N. V. Beletskii, O. F. Frolova, B. A. Fedorinov, M. N. Karmatskaya, E. N. Kuznetsova and S. N. Mantrov, Org. Biomol. Chem., 2025, 23, 10901 DOI: 10.1039/D5OB01776A
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