Issue 48, 2021
From the journal:

Physical Chemistry Chemical Physics

The electron that breaks the catalyst's back – excited state dynamics in intermediates of molecular photocatalysts†

Carolin Müller, ORCID logo ab   Ilse Friedländer,b   Benedikt Bagemihl, ORCID logo c   Sven Rau ORCID logo c  and  Benjamin Dietzek-Ivanšić ORCID logo *abd  

* Corresponding authors

a Friedrich Schiller University Jena, Institute of Physical Chemistry, Helmholtzweg 4, Jena, Germany
E-mail: benjamin.dietzek@uni-jena.de
Fax: +49-3641-948302
Tel: +49-3641-948360

b Leibniz Institute of Photonic Technology, Research Department Functional Interfaces, Albert-Einstein-Str. 9, Jena, Germany

c Institute of Inorganic Chemistry I, Ulm University, Albert-Einstein-Allee 11, Ulm, Germany

d Friedrich Schiller University Jena, Center for Energy and Environmental Chemistry Jena (CEEC Jena), Lessingstraße 8, 07743 Jena, Germany

Abstract

In situ spectroelectrochemical studies focussing on the Franck–Condon region and sub-ns electron transfer processes in Ru(II)-tpphz-Pt(II) based photocatalysts reveal that single-electron reduction effectively hinders intramolecular electron transfer between the photoexcited Ru chromophore and the Pt center.

Graphical abstract: The electron that breaks the catalyst's back – excited state dynamics in intermediates of molecular photocatalysts

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Article information

DOI
https://doi.org/10.1039/D1CP04498B
Article type
Paper
Submitted
01 Oct 2021
Accepted
25 Nov 2021
First published
25 Nov 2021

Phys. Chem. Chem. Phys., 2021,23, 27397-27403

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The electron that breaks the catalyst's back – excited state dynamics in intermediates of molecular photocatalysts

C. Müller, I. Friedländer, B. Bagemihl, S. Rau and B. Dietzek-Ivanšić, Phys. Chem. Chem. Phys., 2021, 23, 27397 DOI: 10.1039/D1CP04498B

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