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Direct conversion of syngas into aromatics over bifunctional catalyst without net releasing CO2

Abstract

Tandem catalysis via methanol intermediate is a promising route for the direct conversion of syngas into aromatics. However, the simultaneous formation of CO2 is a serious problem. Here, we demonstrate that CO2 is formed by the water-gas shift (WGS) reaction (CO + H2O → CO2 + H2) over a ZnO−ZrO2/H-ZSM-5 catalyst, and the net CO2 formation could be inhibited without affecting the formation of aromatics by co-feeding CO2.

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Supplementary files

Article information


Submitted
22 Jan 2020
Accepted
25 Mar 2020
First published
25 Mar 2020

Chem. Commun., 2020, Accepted Manuscript
Article type
Communication

Direct conversion of syngas into aromatics over bifunctional catalyst without net releasing CO2

W. Zhou, C. Zhou, H. Yin, J. Shi, G. Zhang, X. Zheng, X. Min, Z. Zhang, K. Cheng, J. Kang, Q. Zhang and Y. Wang, Chem. Commun., 2020, Accepted Manuscript , DOI: 10.1039/D0CC00608D

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