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Catalytic enhancement on Ti–Zr complex oxide particles for electrochemical hydrogenation of oxalic acid to produce an alcoholic compound by controlling electronic states and oxide structures

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Abstract

Ti1−xZrxO2 complex oxide particles with 0.02 ≤ x ≤ 0.1 show superior catalytic performances for the direct power storage into glycolic acid via electroreduction of oxalic acid. The atomic pair distribution function analysis of X-ray total scatterings suggested that structural periodicity is the key factor for the catalytic enhancement.

Graphical abstract: Catalytic enhancement on Ti–Zr complex oxide particles for electrochemical hydrogenation of oxalic acid to produce an alcoholic compound by controlling electronic states and oxide structures

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Publication details

The article was received on 01 Aug 2019, accepted on 12 Oct 2019 and first published on 14 Oct 2019


Article type: Communication
DOI: 10.1039/C9CY01541H
Catal. Sci. Technol., 2019, Advance Article

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    Catalytic enhancement on Ti–Zr complex oxide particles for electrochemical hydrogenation of oxalic acid to produce an alcoholic compound by controlling electronic states and oxide structures

    M. Yamauchi, S. Hata, H. Eguchi, S. Kitano, T. Fukushima, M. Higashi, M. Sadakiyo and K. Kato, Catal. Sci. Technol., 2019, Advance Article , DOI: 10.1039/C9CY01541H

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