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Sequential Deposition Route to Efficient Sb2S3 Solar Cells

Abstract

We report a facile two-step sequential deposition method to prepare Sb2S3 thin films, where antimony acetate and thiourea are utilized as antimony and sulfur sources, respectively. The sequential deposition of two precursor materials followed by a swift annealing at mild temperature leads to a high-quality Sb2S3 films. The detailed reaction mechanism is revealed on the bases of structural and compositional analyses. By optimizing the concentration of thiourea and annealing temperature, uniform and flat Sb2S3 thin films are obtained with either sulfur-deficient or sulfur-rich. Finally, planar heterojunction solar cell based on the as-prepared Sb2S3 film delivers a high power conversion efficiency of 5.69%, which is a top value in planar heterojunction Sb2S3 solar cells fabricated by solution approach. This research provides a convenient and low-cost approach for the deposition of Sb2S3 films for efficient solar cell applications.

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Publication details

The article was received on 27 Aug 2018, accepted on 08 Oct 2018 and first published on 10 Oct 2018


Article type: Paper
DOI: 10.1039/C8TA08296K
Citation: J. Mater. Chem. A, 2018, Accepted Manuscript
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    Sequential Deposition Route to Efficient Sb2S3 Solar Cells

    L. Zhang, C. Wu, W. liu, S. Yang, M. Wang, T. Chen and C. Zhu, J. Mater. Chem. A, 2018, Accepted Manuscript , DOI: 10.1039/C8TA08296K

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