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Construction of the highly oxidized bicyclo[3.2.1]octane CD ring system of aconitine via a late stage enyne cycloisomerization

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Abstract

A strategy for synthesizing the highly oxidized bicyclo[3.2.1]octane CD rings of aconitine is reported. The key features of the synthesis include a ring-closing metathesis to form the C-ring as well as the application of a ruthenium-catalysed enyne cycloisomerization to assemble the bridged CD ring system of aconitine.

Graphical abstract: Construction of the highly oxidized bicyclo[3.2.1]octane CD ring system of aconitine via a late stage enyne cycloisomerization

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Publication details

The article was received on 22 Aug 2018, accepted on 05 Oct 2018 and first published on 06 Oct 2018


Article type: Communication
DOI: 10.1039/C8CC06819D
Citation: Chem. Commun., 2018, Advance Article
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    Construction of the highly oxidized bicyclo[3.2.1]octane CD ring system of aconitine via a late stage enyne cycloisomerization

    X. Zhou, Y. Liu, R. Zhou, H. Song, X. Liu and Y. Qin, Chem. Commun., 2018, Advance Article , DOI: 10.1039/C8CC06819D

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