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Issue 2, 2016
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Operando XAFS of supported Pd nanoparticles in flowing ethanol/water mixtures: implications for catalysis

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Abstract

Ethanol–water, a prototypical ‘green’ solvent mixture, cannot be considered as inert toward supported Pd nanoparticles. We establish severe size dependencies in Pd redox behavior, persistent gradients in Pd phase in a plug-flow situation, and that Pd nanoparticles are contaminated with hydrogen derived from the solvent.

Graphical abstract: Operando XAFS of supported Pd nanoparticles in flowing ethanol/water mixtures: implications for catalysis

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Supplementary files

Article information


Submitted
14 Jul 2015
Accepted
07 Aug 2015
First published
12 Aug 2015

This article is Open Access

Green Chem., 2016,18, 406-411
Article type
Communication
Author version available

Operando XAFS of supported Pd nanoparticles in flowing ethanol/water mixtures: implications for catalysis

M. A. Newton, J. B. Brazier, E. M. Barreiro, S. Parry, H. Emmerich, L. A. Adrio, C. J. Mulligan, K. Hellgardt and K. K. (. Hii, Green Chem., 2016, 18, 406 DOI: 10.1039/C5GC01600B

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