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Abstract | Cited by

Iridium-catalyzed acceptorless dehydrogenative coupling of tertiary amines and arylamines has been developed. A number of benzimidazoles were prepared in good yields. An iridium-mediated C–H activation mechanism is suggested. This finding represents a novel strategy for the synthesis of benzimidazoles.

Graphical abstract: Synthesis of benzimidazoles via iridium-catalyzed acceptorless dehydrogenative coupling

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