The 13C–14N nuclear spin coupling constants for isocyanides have been observed using the proton-decoupled 13C n.m.r. method, and the results compared with the corresponding coupling constant for cyanides together with the theoretical values obtained by molecular orbital calculations.
I. Morishima, A. Mizuno, T. Yonezawa and K. Goto, J. Chem. Soc. D, 1970, 1321 DOI: 10.1039/C29700001321
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