We describe a Mn(II)-catalyzed, biocompatible, and economical strategy for selective and efficient synthesis of both P(O)–O and P(O)–C compounds via a dehydrogenative phospha-Brook rearrangement, with broad substrate scope and mechanistic validation from control and kinetic studies.
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H. J. Phukan, A. Samanta, K. Mohar, A. Mondal, R. Dihingia and D. Srimani, Chem. Commun., 2026, Advance Article , DOI: 10.1039/D6CC01657J
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