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The reversible lithium-ion storage property of viologen has been explored for the first time. The viologen exhibits a reversible capacity of 175 mA h g−1 against lithium at 50 mA g−1 discharge rate, long term cycling performance and good rate capability. The reversible lithiation–delithiation property of the viologen has been confirmed by ex situ NMR studies.

Graphical abstract: Facile synthesis of viologen and its reversible lithium storage property in organic lithium-ion batteries

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