Issue 50, 2021

Solvation vs. surface charge transfer: an interfacial chemistry game drives cation motion

Abstract

Electrolyte structure and ion solvation dynamics determine ionic conductivities, and ion (de)solvation processes dominate interfacial chemistry and electrodeposition barriers. We elucidate electrolyte effects facilitating or impeding Li+ diffusion and deposition, and evaluate structural and energetic changes during the solvation complex pathway from the bulk to the anode surface.

Graphical abstract: Solvation vs. surface charge transfer: an interfacial chemistry game drives cation motion

Supplementary files

Article information

Article type
Communication
Submitted
16 Mar 2021
Accepted
24 May 2021
First published
25 May 2021

Chem. Commun., 2021,57, 6189-6192

Solvation vs. surface charge transfer: an interfacial chemistry game drives cation motion

S. Angarita-Gomez and P. B. Balbuena, Chem. Commun., 2021, 57, 6189 DOI: 10.1039/D1CC01408K

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