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Issue 44, 2018
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Synthetic studies on daphniglaucins

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Abstract

The synthetic approach to the core framework of daphniglaucin-type Daphniphyllum alkaloids is described herein. The B–C ring was constructed via a Rh-catalyzed [3+2] cycloaddition. Continuous quaternary centers were installed through [3+2] cycloaddition and alkylation. The attempt to build the A–D ring motif using dipolar cycloaddition of azomethine ylides was extensively investigated.

Graphical abstract: Synthetic studies on daphniglaucins

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Publication details

The article was received on 17 Apr 2018, accepted on 03 May 2018 and first published on 03 May 2018


Article type: Communication
DOI: 10.1039/C8CC03063D
Chem. Commun., 2018,54, 5554-5557

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    Synthetic studies on daphniglaucins

    Y. Qiu, J. Zhong, S. Du and S. Gao, Chem. Commun., 2018, 54, 5554
    DOI: 10.1039/C8CC03063D

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