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Issue 68, 2017
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Collaborative enhancement from Pb2+ and F in Pb2(NO3)2(H2O)F2 generates the largest second harmonic generation effect among nitrates

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Abstract

The first metal nitrate fluoride nonlinear optical material, Pb2(NO3)2(H2O)F2, was synthesized with the largest second harmonic generation (SHG) effect (12 × KH2PO4) among nitrates. Theoretical calculations revealed the synergistic effect of [NO3], lone pair electrons in Pb2+, and F for the SHG effect. The F also promoted the blue-shift of the ultraviolet cut-off edge.

Graphical abstract: Collaborative enhancement from Pb2+ and F− in Pb2(NO3)2(H2O)F2 generates the largest second harmonic generation effect among nitrates

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Article information


Submitted
05 Jun 2017
Accepted
09 Jul 2017
First published
10 Jul 2017

Chem. Commun., 2017,53, 9398-9401
Article type
Communication

Collaborative enhancement from Pb2+ and F in Pb2(NO3)2(H2O)F2 generates the largest second harmonic generation effect among nitrates

G. Peng, Y. Yang, Y. Tang, M. Luo, T. Yan, Y. Zhou, C. Lin, Z. Lin and N. Ye, Chem. Commun., 2017, 53, 9398
DOI: 10.1039/C7CC04340F

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