Synthesis and application of thiocarbamates via thiol-dioxazolone modified Lossen rearrangement

Yu Jiang; Ming Li; Shuxin Liu; Rui Li; Yubin Zheng; Wangze Song; Nan Zheng

doi:10.1039/D2CC05198B

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Synthesis and application of thiocarbamates via thiol-dioxazolone modified Lossen rearrangement†

Yu Jiang,‡^a Ming Li,‡^a Shuxin Liu,^a Rui Li,^a Yubin Zheng,^a Wangze Song

*^a and Nan Zheng

*^a

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* Corresponding authors

^a Department of Polymer Science & Materials, School of Chemical Engineering, Dalian University of Technology, Dalian, P. R. China
E-mail: nzheng@dlut.edu.cn, wzsong@dlut.edu.cn

Abstract

Thiocarbamates could be synthesized in green solvents via thiol-dioxazolone modified Lossen rearrangement under transition-metal free, additive free, and mild conditions. Polythiocarbamates were further prepared with excellent self-healing and shape-memory properties, showing great potential in the development of functional materials.

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DOI: https://doi.org/10.1039/D2CC05198B
Article type: Communication
Submitted: 21 Sep 2022
Accepted: 05 Oct 2022
First published: 20 Oct 2022

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Chem. Commun., 2022,58, 12353-12356

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Synthesis and application of thiocarbamates via thiol-dioxazolone modified Lossen rearrangement

Y. Jiang, M. Li, S. Liu, R. Li, Y. Zheng, W. Song and N. Zheng, Chem. Commun., 2022, 58, 12353 DOI: 10.1039/D2CC05198B

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Chemical Communications

Synthesis and application of thiocarbamates via thiol-dioxazolone modified Lossen rearrangement†

Abstract

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Synthesis and application of thiocarbamates via thiol-dioxazolone modified Lossen rearrangement

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