Frontier orbital assignment in iminophosphanes in carried out by utilizing a linear relationship between differences in optical transitions and ionisation potentials confirming the ambident reaction behaviour of these compounds.
E. Niecke, D. Gudat, W. W. Schoeller and P. Rademacher, J. Chem. Soc., Chem. Commun., 1985, 1050 DOI: 10.1039/C39850001050
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