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4,21-Dehydrogeissoschizine (5) was proven to be a metabolic intermediate in the enzymatic synthesis of cathenamine (6) and its transformation products ajmalicine (7), 19-epiajmalicine (8), and tetrahydroalstonine (9); the enzyme catalysing the synthesis of (6) from (5) was identified and named cathenamine synthase.
M. Rueffer, C. Kan-Fan, H. Husson, J. Stöckigt and M. H. Zenk, J. Chem. Soc., Chem. Commun., 1979, 1016 DOI: 10.1039/C39790001016
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