The deprotonated nitrogen atoms in the barbital anions in calcium barbital trihydrate are involved either in co-ordination to the calcium cations or as acceptors in hydrogen bonds, whereas the non-deprotonated ones are involved as donors to form isolated hydrogen-bonded barbital dimers.
B. Berking, J. Chem. Soc. D, 1971, 674 DOI: 10.1039/C29710000674
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