The negative excess volumes found by Staveley and co-workers for liquid mixtures of argon and krypton are related to equation-of-state parameters for the pure liquids and the excess free energy according to the theory of solutions developed recently and successfully applied heretofore to mixtures of non-polar polyatomic molecules.
H. Höcker and P. J. Flory, Trans. Faraday Soc., 1968, 64, 1188 DOI: 10.1039/TF9686401188
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