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Collaborative enhancement from Pb2+ and F in Pb2(NO3)2(H2O)F2 generates the largest second harmonic generation effect among nitrates

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Abstract

The first metal nitrate fluoride nonlinear optical material, Pb2(NO3)2(H2O)F2, was synthesized with the largest second harmonic generation (SHG) effect (12 × KH2PO4) among nitrates. Theoretical calculations revealed the synergistic effect of [NO3], lone pair electrons in Pb2+, and F for the SHG effect. The F also promoted the blue-shift of the ultraviolet cut-off edge.

Graphical abstract: Collaborative enhancement from Pb2+ and F− in Pb2(NO3)2(H2O)F2 generates the largest second harmonic generation effect among nitrates

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Publication details

The article was received on 05 Jun 2017, accepted on 09 Jul 2017 and first published on 10 Jul 2017


Article type: Communication
DOI: 10.1039/C7CC04340F
Citation: Chem. Commun., 2017, Advance Article
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    Collaborative enhancement from Pb2+ and F in Pb2(NO3)2(H2O)F2 generates the largest second harmonic generation effect among nitrates

    G. Peng, Y. Yang, Y. Tang, M. Luo, T. Yan, Y. Zhou, C. Lin, Z. Lin and N. Ye, Chem. Commun., 2017, Advance Article , DOI: 10.1039/C7CC04340F

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