Conversion of {Fe(NO)2}10 dinitrosyl iron to nitrato iron(III) species by molecular oxygen

Kelsey M. Skodje; Paul G. Williard; Eunsuk Kim

doi:10.1039/C2DT30443K

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Dalton Transactions

Issue 26, 2012

The international journal for inorganic, organometallic and bioinorganic chemistry

Impact Factor 3.838 48 Issues per Year Indexed in MEDLINE

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Conversion of {Fe(NO)₂}¹⁰ dinitrosyl iron to nitrato iron(III) species by molecular oxygen

Kelsey M. Skodje,^a Paul G. Williard^a and Eunsuk Kim*^a

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Department of Chemistry, Brown University, Providence, USA
E-mail: eunsuk_kim@brown.edu

Dalton Trans., 2012,41, 7849-7851

DOI: 10.1039/C2DT30443K
Received 23 Feb 2012, Accepted 03 Apr 2012
First published online 11 Apr 2012

This article is part of themed collection: New Talent: Americas

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A new {Fe(NO)₂}¹⁰ dinitrosyl iron complex possessing a 2,9-dimethyl-1,10-phenanthroline ligand has been prepared. This complex exhibits dioxygenase activity, converting NO to nitrate (NO₃⁻) anions. During the oxygenation reaction, formation of reactive nitrating species is implicated, as shown in the effective o-nitration with a phenolic substrate.

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Conversion of {Fe(NO)₂}¹⁰ dinitrosyl iron to nitrato iron(III) species by molecular oxygen

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Conversion of {Fe(NO)2}10 dinitrosyl iron to nitrato iron(III) species by molecular oxygen

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Conversion of {Fe(NO)₂}¹⁰ dinitrosyl iron to nitrato iron(III) species by molecular oxygen