Reconstruction of bimetal CoFe0.13-MOF to enhance the catalytic performance in the oxygen evolution reaction

Kexin Yang; Zeqi Jin; Qicheng Zhang; Qiming Chen; Wenchao Peng; Yang Li; Fengbao Zhang; Qing Xia; Xiaobin Fan

doi:10.1039/D1CC06314F

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Reconstruction of bimetal CoFe_0.13-MOF to enhance the catalytic performance in the oxygen evolution reaction†

Kexin Yang,‡^a Zeqi Jin,‡^a Qicheng Zhang,^a Qiming Chen,^a Wenchao Peng,

^ab Yang Li,

^ab Fengbao Zhang,^ab Qing Xia

*^a and Xiaobin Fan

*^ab

Author affiliations

* Corresponding authors

^a School of Chemical Engineering and Technology, State Key Laboratory of Chemical Engineering, Collaborative Innovation Center of Chemical Science and Engineering, Tianjin University, Tianjin 300072, People's Republic of China

^b Chemistry and Chemical Engineering Guangdong Laboratory, Shantou, China
E-mail: xiaqing@tju.edu.cn, xiaobinfan@tju.edu.cn

Abstract

Oxygen evolution reaction (OER) is a key process in electrochemical energy conversion systems. This paper found that the solvothermal reconstruction could resume the original morphology and generate more oxygen vacancies on the surface of oxyhydroxide. The reconstructed electrocatalyst (re-CoFe_0.13O_xH_y) presents promising long-term stability (>85 h) under 1 M KOH condition without replacing the electrolyte.

This article is part of the themed collection: ChemComm Milestones – First Independent Articles

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Article information

DOI: https://doi.org/10.1039/D1CC06314F
Article type: Communication
Submitted: 09 11月 2021
Accepted: 03 12月 2021
First published: 04 12月 2021

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Chem. Commun., 2022,58, 1115-1118

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Reconstruction of bimetal CoFe_0.13-MOF to enhance the catalytic performance in the oxygen evolution reaction

K. Yang, Z. Jin, Q. Zhang, Q. Chen, W. Peng, Y. Li, F. Zhang, Q. Xia and X. Fan, Chem. Commun., 2022, 58, 1115 DOI: 10.1039/D1CC06314F

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Chemical Communications