The syntheses of the first homoleptic U(III) and U(IV) amidate complexes are described. These can be interconverted by chemical reduction/oxidation, showing an unusual change in coordination number from four in the U(III) complex to eight in the U(IV) complex in the solid state structures.
M. D. Straub, S. Hohloch, S. G. Minasian and J. Arnold, Dalton Trans., 2018, 47, 1772 DOI: 10.1039/C7DT04813K
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