Ultrathin g-C3N4 nanosheets with an extended visible-light-responsive range for significant enhancement of photocatalysis

Yanfang Yang; Jingjing Chen; Zhiyong Mao; Na An; Dajian Wang; Bradley D. Fahlman

doi:10.1039/C6RA26172H

Ultrathin g-C₃N₄ nanosheets with an extended visible-light-responsive range for significant enhancement of photocatalysis

Yanfang Yang,†^a Jingjing Chen,†^b Zhiyong Mao,*^a Na An,^b Dajian Wang*^b and Bradley D. Fahlman^c

* Corresponding authors

^a School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, P. R. China
E-mail: mzhy984@163.com

^b Tianjin Key Laboratory for Photoelectric Materials and Devices, Tianjin University of Technology, Tianjin 300384, P. R. China
E-mail: djwang@tjut.edu.cn

^c Department of Chemistry & Biochemistry and Science of Advanced Materials Program, Central Michigan University, Mount Pleasant, MI, USA 48859

Abstract

Ultrathin graphitic carbon nitride (g-C₃N₄) nanosheets were synthesized via thermal exfoliation of bulk urea-derived g-C₃N₄ under an argon atmosphere. As a visible-light responsive photocatalyst, this material exhibits a much superior photocatalytic activity in pollution degradation and H₂ evolution than bulk g-C₃N₄, as a result of the extended region of visible light response and the enhanced surface area of ultrathin g-C₃N₄ nanosheets. These findings may provide a promising and facile approach to the design of high-performance photocatalysts.

This article is part of the themed collection: Photocatalysis

Article information

https://doi.org/10.1039/C6RA26172H

Article type

Paper

Submitted

02 ⵏⵓⵡ 2016

Accepted

10 ⴷⵓⵊ 2016

First published

12 ⵉⵏⵏ 2017

This article is Open Access

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RSC Adv., 2017,7, 2333-2341

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Ultrathin g-C₃N₄ nanosheets with an extended visible-light-responsive range for significant enhancement of photocatalysis

Y. Yang, J. Chen, Z. Mao, N. An, D. Wang and B. D. Fahlman, RSC Adv., 2017, 7, 2333 DOI: 10.1039/C6RA26172H

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Ultrathin g-C₃N₄ nanosheets with an extended visible-light-responsive range for significant enhancement of photocatalysis

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Ultrathin g-C₃N₄ nanosheets with an extended visible-light-responsive range for significant enhancement of photocatalysis

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