Themed collection Celebrating Excellence in Research: 100 Women of Chemistry
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A new family of sesterterpenoids isolated around the Pacific Rim
This review compiles details of the isolation, proposed biogenesis and biological testing of a new family of marine sesterterpenoids isolated around the Pacific Rim between 2009–2017.
Nat. Prod. Rep., 2018,35, 210-219
https://doi.org/10.1039/C7NP00049A
Perspectives on metal–organic frameworks with intrinsic electrocatalytic activity
This highlight article focuses on the rapidly emerging area of electrocatalytic metal–organic frameworks (MOFs) with a particular emphasis on those systems displaying intrinsic activity.
CrystEngComm, 2017,19, 4049-4065
https://doi.org/10.1039/C7CE00215G
An introduction to ratchets in chemistry and biology
This article describes the functions and mechanisms of particle and electron ratchets, and the interplay between theory and experiment in this field of non-equilibrium transport.
Mater. Horiz., 2017,4, 310-318
https://doi.org/10.1039/C7MH00062F
Spatiotemporal hydrogel biomaterials for regenerative medicine
This review highlights recent efforts in using photochemistry to exert dynamic control over the properties of hydrogel biomaterials.
Chem. Soc. Rev., 2017,46, 6532-6552
https://doi.org/10.1039/C7CS00445A
Visible-light-absorbing semiconductor/molecular catalyst hybrid photoelectrodes for H2 or O2 evolution: recent advances and challenges
Herein, we review the recent advances and challenges in the field of visible-light-absorbing semiconductor/molecular catalyst photoelectrodes for H2 and O2 evolution.
Sustainable Energy Fuels, 2017,1, 1641-1663
https://doi.org/10.1039/C7SE00222J
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Multicellular tumor spheroids: a relevant 3D model for the in vitro preclinical investigation of polymer nanomedicines
Application of 3D multicellular tumor spheroids to the investigation of polymer nanomedicines.
Polym. Chem., 2017,8, 4947-4969
https://doi.org/10.1039/C7PY00559H
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Conformational control of the bacterial Clp protease by natural product antibiotics
Natural products targeting the bacterial Clp protease unravel key interfaces for protein–protein–interaction and long-distance conformational control.
Nat. Prod. Rep., 2017,34, 815-831
https://doi.org/10.1039/C6NP00125D
Perovskite oxides – a review on a versatile material class for solar-to-fuel conversion processes
The thermodynamic and defect chemical opportunities and challenges of perovskite oxides used for thermochemical water and carbon dioxide splitting are reviewed.
J. Mater. Chem. A, 2017,5, 11983-12000
https://doi.org/10.1039/C7TA00987A
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Concentration gradient generation methods based on microfluidic systems
Various concentration gradient generation methods based on microfluidic systems are summarized in this paper.
RSC Adv., 2017,7, 29966-29984
https://doi.org/10.1039/C7RA04494A
1,3-N,O-Complexes of late transition metals. Ligands with flexible bonding modes and reaction profiles
1,3-N,O-Chelating ligands are ubiquitous in nature owing to their occurrence as α-chiral amino acids in metalloproteins.
Chem. Soc. Rev., 2017,46, 2913-2940
https://doi.org/10.1039/C6CS00715E
Recent applications of the combination of mesoporous silica nanoparticles with nucleic acids: development of bioresponsive devices, carriers and sensors
The control of many biological roles exerted by nucleic acids turned them into a powerful tool for the development of advanced biotechnological materials when in combination with mesoporous silica nanoparticles.
Biomater. Sci., 2017,5, 353-377
https://doi.org/10.1039/C6BM00872K
Insulin hexamer dissociation dynamics revealed by photoinduced T-jumps and time-resolved X-ray solution scattering
The structural dynamics of insulin hexamer dissociation were studied by the photoinduced temperature jump technique and monitored by time-resolved X-ray scattering.
Photochem. Photobiol. Sci., 2018,17, 874-882
https://doi.org/10.1039/C8PP00034D
Transfer hydrogenation of carbon dioxide and bicarbonate from glycerol under aqueous conditions
Catalytic transfer hydrogenation of CO2 from glycerol to afford formic and lactic acid is an attractive path to valorizing two waste streams. The process is significantly more thermodynamically favorable than direct CO2 hydrogenation.
Chem. Commun., 2018,54, 6184-6187
https://doi.org/10.1039/C8CC03157F
A thumb-size electrochemical system for portable sensors
A thumb-size and precise electrochemical system is designed for sensors in size and cost sensitive applications.
Analyst, 2018,143, 2760-2764
https://doi.org/10.1039/C8AN00645H
One-of-a-kind: a microporous metal–organic framework capable of adsorptive separation of linear, mono- and di-branched alkane isomers via temperature- and adsorbate-dependent molecular sieving
Clean separation of linear, monobranched, and dibranched alkanes is achieved using a flexible, microporous metal–organic framework (MOF).
Energy Environ. Sci., 2018,11, 1226-1231
https://doi.org/10.1039/C8EE00459E
The alkyne-tag Raman imaging of coronatine, a plant pathogen virulence factor, in Commelina communis and its possible mode of action
Coronatine, a virulence factor of plant bacteria, facilitates bacterial infection through an ER (endoplasmic reticulum)-mediated mechanism and works by affecting the ethylene signaling pathway.
Org. Biomol. Chem., 2018,16, 3348-3352
https://doi.org/10.1039/C8OB00097B
A new organic compound of 2-(2,2-diphenylethenyl)anthracene (DPEA) showing simultaneous electrical charge transport property and AIE optical characteristics
DPEA shows good charge carrier mobility and AIE efficient luminescence.
J. Mater. Chem. C, 2018,6, 3856-3860
https://doi.org/10.1039/C8TC00763B
Mesoporous manganese phthalocyanine-based materials for electrochemical water oxidation via tailored templating
Electrochemical water splitting using non-noble metals as catalysts is of increasing importance for the future energy sector.
Catal. Sci. Technol., 2018,8, 1517-1521
https://doi.org/10.1039/C7CY02484C
Spatially resolved coding of λ-orthogonal hydrogels by laser lithography
A λ-orthogonal reaction system is introduced, where visible light induced radical thiol–ene and UV light induced NITEC (Nitrile-Imine mediated Tetrazole–Ene Conjugation) ligations are consecutively employed to fabricate and functionalize PEG-based hydrogels.
Chem. Commun., 2018,54, 2436-2439
https://doi.org/10.1039/C7CC09619D
Size dependent surface reconstruction in detonation nanodiamonds
Sub 3 nm diamond particles show size- and shape-dependent surface reconstructions, which have significant impact to their functionality and performance.
Nanoscale Horiz., 2018,3, 213-217
https://doi.org/10.1039/C7NH00125H
Controlling the lectin recognition of glycopolymers via distance arrangement of sugar blocks
Control of molecular recognition via living radical polymerization.
Chem. Commun., 2018,54, 82-85
https://doi.org/10.1039/C7CC07107H
Photo-induced ring-closure via a looped flow reactor
Looped flow processes are an efficient and versatile tool to synthesize cyclic macromolecular materials.
React. Chem. Eng., 2017,2, 826-829
https://doi.org/10.1039/C7RE00124J
Degradable gold core–mesoporous organosilica shell nanoparticles for two-photon imaging and gemcitabine monophosphate delivery
The synthesis of degradable gold core–mesoporous organosilica shell nanoparticles is described.
Mol. Syst. Des. Eng., 2017,2, 380-383
https://doi.org/10.1039/C7ME00058H
Is more better? A comparison of tri- and tetrapeptidic catalysts
From an enzymatic perspective, there is a general notion that the bigger and more complex a catalytically active peptide is the more enzyme-like and the better it should become. But is this really true?
Org. Biomol. Chem., 2017,15, 5877-5881
https://doi.org/10.1039/C7OB01039G
Coaxial Ag–base metal nanowire networks with high electrochemical stability for transparent and stretchable asymmetric supercapacitors
Based on electrochemically stable Ag–Ni and Ag–Fe core–shell nanowire networks, a transparent and stretchable asymmetric supercapacitor was demonstrated.
Nanoscale Horiz., 2017,2, 199-204
https://doi.org/10.1039/C7NH00024C
Solution-processed 2-dimensional hole-doped ionic graphene compounds
Solution-based direct assembly of centimeter-square sizes of graphene–fluorofullerene multilayers with a tunable work function, up to 5.7 eV, and a remarkable chemical stability is demonstrated.
Mater. Horiz., 2017,4, 456-463
https://doi.org/10.1039/C7MH00068E
Solid-state-processing of δ-PVDF
Solid-state pressing is used to produce, in one single-step and without the need to mechanically stretch thin foils, ferroelectric structures from the commodity polymer poly(vinylidene fluoride) (PVDF) with comparable piezoelectric properties to biaxially stretched β-PVDF.
Mater. Horiz., 2017,4, 408-414
https://doi.org/10.1039/C7MH00007C
Effective separation of aromatic and aliphatic amino acid mixtures using ionic-liquid-based aqueous biphasic systems
Ionic-liquid-based aqueous biphasic systems allow an efficient and selective separation of aliphatic and aromatic amino acid mixtures usually present in protein hydrolysates or fermentation broths.
Green Chem., 2017,19, 1850-1854
https://doi.org/10.1039/C6GC03060B
A cobalt(II) complex with unique paraSHIFT responses to anions
A cobalt(II) complex can distinguish between anions by observing the paramagnetic 1H NMR shift.
Chem. Commun., 2017,53, 3571-3574
https://doi.org/10.1039/C7CC00619E
Chiral expression of adsorbed (MP) 5-amino[6]helicenes: from random structures to dense racemic crystals by surface alloying
The chiral expression of a molecule on a surface is driven from a random solid solution on Cu(100) to a racemic crystal on a Sn/Cu(100) alloy.
Chem. Commun., 2017,53, 130-133
https://doi.org/10.1039/C6CC06785A
Porous silicon–graphene oxide core–shell nanoparticles for targeted delivery of siRNA to the injured brain
A chemically targeted luminescent porous silicon–graphene oxide core–shell nanoparticle delivers siRNA for more effective gene silencing.
Nanoscale Horiz., 2016,1, 407-414
https://doi.org/10.1039/C6NH00082G
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A two-qubit molecular architecture for electron-mediated nuclear quantum simulation
A molecular architecture where two vanadyl-based qubits are linked together is herein described and investigated as a platform for quantum simulation.
Chem. Sci., 2018,9, 6183-6192
https://doi.org/10.1039/C8SC01695J
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Pyrene hydrogel for promoting direct bioelectrochemistry: ATP-independent electroenzymatic reduction of N2
We demonstrate a novel hydrogel material to facilitate direct bioelectrochemistry of a wide range of redox proteins and enable ATP-independent electroenzymatic reduction of N2 by nitrogenase.
Chem. Sci., 2018,9, 5172-5177
https://doi.org/10.1039/C8SC01638K
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Taming a monomeric [Cu(η6-C6H6)]+ complex with silylene
Realization of a hitherto elusive unsupported η6 binding mode of benzene to a copper(I) cation employing silylene as a ligand. The back-donation from Cu to Si(II) diminishes the repulsion between d-electrons and the benzene ring and enforces the η6 binding mode.
Chem. Sci., 2018,9, 4333-4337
https://doi.org/10.1039/C8SC00459E
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A benzylic linker promotes methyltransferase catalyzed norbornene transfer for rapid bioorthogonal tetrazine ligation
Benzylic AdoMet analogs enable highly efficient enzymatic transfer of norbornenes to nucleic acids and subsequent tetrazine ligation.
Chem. Sci., 2017,8, 7947-7953
https://doi.org/10.1039/C7SC03631K
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Generalized-active-space pair-density functional theory: an efficient method to study large, strongly correlated, conjugated systems
Predicting ground- and excited-state properties of open-shell organic molecules by electronic structure theory can be challenging because an accurate treatment has to correctly describe both static and dynamic electron correlation.
Chem. Sci., 2017,8, 2741-2750
https://doi.org/10.1039/C6SC05036K
Hydrogen consumption and methanogenic community evolution in anodophilic biofilms in single chamber microbial electrolysis cells under different startup modes
GeoChips based on mcrA and cytochrome genes to evaluate community structure variety of methanogens and electron transfer process.
Environ. Sci.: Water Res. Technol., 2018,4, 1839-1850
https://doi.org/10.1039/C8EW00357B
Impact of excess PbI2 on the structure and the temperature dependent optical properties of methylammonium lead iodide perovskites
Excess PbI2 in MAPbI3 thin films has no direct impact on the electronic structure but changes the temperature dependence of the exciton binding energy and the phase transition behaviour.
J. Mater. Chem. C, 2018,6, 7512-7519
https://doi.org/10.1039/C8TC02237B
A versatile method for the selective core-crosslinking of hyaluronic acid nanogels via ketone-hydrazide chemistry: from chemical characterization to in vivo biodistribution
Nanogels show long in vivo blood circulation time and high tumor accumulation.
Biomater. Sci., 2018,6, 1754-1763
https://doi.org/10.1039/C8BM00396C
Electron scattering in large water clusters from photoelectron imaging with high harmonic radiation
The scattering of low kinetic energy electrons in large water clusters can be treated as an intermediate case between gas and condensed phase scattering.
Phys. Chem. Chem. Phys., 2018,20, 16364-16371
https://doi.org/10.1039/C8CP02148A
A sequential enzyme-activated and light-triggered pro-prodrug nanosystem for cancer detection and therapy
A sequential enzyme-activated and light-triggered pro-prodrug has been developed for cancer biomarker detection and on-demand therapy.
J. Mater. Chem. B, 2018,6, 2547-2556
https://doi.org/10.1039/C7TB01989K
Fully automated, on-site isolation of cfDNA from whole blood for cancer therapy monitoring
Fully integrated lab-on-a-disc for cfDNA isolation allows real-time monitoring of tumor mutation status during targeted therapy.
Lab Chip, 2018,18, 1320-1329
https://doi.org/10.1039/C8LC00165K
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Tuning mobility and stability of lithium ion conductors based on lattice dynamics
Ionic conductivity and stability of Li-ion conductors are rationalized on the same footing using lattice-dynamics descriptors.
Energy Environ. Sci., 2018,11, 850-859
https://doi.org/10.1039/C7EE03364H
Aqueous vs. nonaqueous Zn-ion batteries: consequences of the desolvation penalty at the interface
Comparison of intercalation of Zn2+ in layered V3O7·H2O in non-aqueous and aqueous electrolytes reveals a much higher desolvation penalty at the non-aqueous interface, a major factor in dictating the kinetics.
Energy Environ. Sci., 2018,11, 881-892
https://doi.org/10.1039/C8EE00378E
Local chemistry of the surfactant's head groups determines protein stability in reverse micelles
Protein stability in reverse micelles is determined by local chemical interactions between the surfactant molecules and the protein groups.
Phys. Chem. Chem. Phys., 2018,20, 8515-8522
https://doi.org/10.1039/C8CP00407B
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Polymorphism of chlorpropamide on liquid-assisted mechanical treatment: choice of liquid and type of mechanical treatment matter
Different types of mechanical treatment (tableting, grinding, milling, etc.) are important technological operations in the pharmaceutical industry.
CrystEngComm, 2018,20, 1797-1803
https://doi.org/10.1039/C7CE02221B
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Temporal trends of halogenated flame retardants in the atmosphere of the Canadian Great Lakes Basin (2005–2014)
Temporal and spatial trends of total air concentrations (gas + particle) of halogenated flame retardants at the Canadian Great Lakes Basin were assessed (2005–2014).
Environ. Sci.: Processes Impacts, 2018,20, 469-479
https://doi.org/10.1039/C7EM00549K
Physicochemical properties of air discharge-generated manganese oxide nanoparticles: comparison to welding fumes
Physicochemical properties of manganese nanoparticles are key to adverse health effects.
Environ. Sci.: Nano, 2018,5, 696-707
https://doi.org/10.1039/C7EN01046J
Determining the uncertainty in microstructural parameters extracted from tomographic data
The procedure for binarization of X-ray tomographic data affects the quantitative analysis of microstructural parameters in lithium ion battery electrodes.
Sustainable Energy Fuels, 2018,2, 598-605
https://doi.org/10.1039/C7SE00498B
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A solution-processable dissymmetric porous organic cage
A dissymmetric, soluble, porous organic cage from a low-cost racemic precursor.
Mol. Syst. Des. Eng., 2018,3, 223-227
https://doi.org/10.1039/C7ME00090A
Calibration and evaluation of PUF-PAS sampling rates across the Global Atmospheric Passive Sampling (GAPS) network
Here we present and evaluate a method to determine PUF-PAS sampling rates (RS), and the effective sampling volume (Veff), for gas-phase chemical compounds deployed anywhere in the world.
Environ. Sci.: Processes Impacts, 2018,20, 210-219
https://doi.org/10.1039/C7EM00360A
Aluminum nanostructures with strong visible-range SERS activity for versatile micropatterning of molecular security labels
A ciphertext-embedded machine-readable micro-QR code is constructed using structurally uniform visible-range SERS-active Al nanostructures with an average SERS enhancement factor of >104.
Nanoscale, 2018,10, 575-581
https://doi.org/10.1039/C7NR07793A
Magnetic bead-based peptide extraction methodology for tissue imaging
MALDI-TOF imaging mass spectrometry (IMS) is a common technique used for analyzing tissue samples, as it allows the user to detect multiple different analytes simultaneously.
Analyst, 2018,143, 133-140
https://doi.org/10.1039/C7AN00757D
A dendritic catiomer with an MOF motif for the construction of safe and efficient gene delivery systems
The dendritic catiomer using biocompatible Zr-MOFs as the core exhibited a markedly higher transfection efficiency and lower cytotoxicity than the commercial gold standard branched PEI25k in A549 cells.
J. Mater. Chem. B, 2017,5, 8322-8329
https://doi.org/10.1039/C7TB01966A
Heterogeneous endotoxin detection bioassay using drug–nanoparticle bioconjugates: an optimization study
Design and development of a simple and ultrasensitive dot blot bioassay for endotoxin detection in serum.
Mol. Syst. Des. Eng., 2017,2, 470-477
https://doi.org/10.1039/C7ME00037E
Singlet oxygen-mediated one-pot chemoselective peptide–peptide ligation
We here describe a furan oxidation based site-specific chemical ligation approach using unprotected peptide segments.
Org. Biomol. Chem., 2017,15, 8140-8144
https://doi.org/10.1039/C7OB02245J
Effective potentials induced by self-assembly of patchy particles
Effective colloid–colloid interactions can be tailored through the addition of a complex cosolute.
Soft Matter, 2017,13, 6051-6058
https://doi.org/10.1039/C7SM01293D
Biodegradation of graphene oxide-polymer nanocomposite films in wastewater
The polymer present in the nanocomposite is degraded by microorganisms present in the wastewater.
Environ. Sci.: Nano, 2017,4, 1808-1816
https://doi.org/10.1039/C7EN00396J
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Detection of sulfenic acid in intact proteins by mass spectrometric techniques: application to serum samples
A new developed strategy for the specific detection and quantification of cysteine sulfenic acid (SA) using molecular and elemental mass spectrometric (MS) techniques.
RSC Adv., 2017,7, 44162-44168
https://doi.org/10.1039/C7RA06241A
Polymerization of silyl ketenes using alkoxide initiators: a combined computational and experimental study
The atomic composition and chemical structure of polymers is fundamental to dictating properties and applications.
Polym. Chem., 2017,8, 5381-5387
https://doi.org/10.1039/C7PY00858A
Extending charge separation lifetime and distance in patterned dye-sensitized SnO2–TiO2 μm-thin films
Charge separation in dye sensitized SnO2–TiO2 μm-thin films was substantially extended by an innovative patterning design strategy.
Phys. Chem. Chem. Phys., 2017,19, 22684-22690
https://doi.org/10.1039/C7CP04486K
Sample preparation of lipstick for further Cd and Pb determination by ICP-MS: is the use of complexing acids really necessary?
In this work, the use of complexing acids (HF and HCl) combined with HNO3 was evaluated for lipstick digestion and further Cd and Pb determination by ICP-MS.
J. Anal. At. Spectrom., 2017,32, 1780-1788
https://doi.org/10.1039/C7JA00139H
Effect of trehalose polymer regioisomers on protein stabilization
Polymers with different trehalose side chain regioisomers were synthesized and compared for insulin stabilization.
Polym. Chem., 2017,8, 4781-4788
https://doi.org/10.1039/C7PY00700K
β-Pyridylenolate zinc catalysts for the ring-opening homo- and copolymerization of ε-caprolactone and lactides
Eleven zinc β-quinolylenolates with varying substituents have been synthesized, and some of these complexes are excellent catalysts for the ring-opening homo- and copolymerization of ε-CL and LAs.
Dalton Trans., 2017,46, 9846-9858
https://doi.org/10.1039/C7DT01877K
A robust analytical method for the determination of pesticide residues in wastewater
The aim of this research was to develop an analytical method for the detection and confirmation of 13 pesticide residues in wastewater.
Anal. Methods, 2017,9, 4167-4174
https://doi.org/10.1039/C7AY00704C
A field analysis of lampricide photodegradation in Great Lakes tributaries
Field measurements, laboratory experiments, and kinetic modeling demonstrate that photodegradation of lampricides is limited in Great Lake tributaries.
Environ. Sci.: Processes Impacts, 2017,19, 891-900
https://doi.org/10.1039/C7EM00173H
Multi-functional polyimides containing tetraphenyl fluorene moieties: fluorescence and resistive switching behaviors
A tetraphenyl fluorene (TPF) moiety in the polyimide main chain or in the side chain has a remarkable impact on the resistive switching behaviors and fluorescence properties of the polymers.
J. Mater. Chem. C, 2017,5, 6457-6466
https://doi.org/10.1039/C7TC01807J
A species-specific double isotope dilution strategy for the accurate quantification of platinum–GG adducts in lung cells exposed to carboplatin
Measurement uncertainty of Pt–GG quantification in human lung cells by species-specific double IDMS.
J. Anal. At. Spectrom., 2017,32, 1320-1330
https://doi.org/10.1039/C7JA00078B
Highly efficient and stable low-temperature processed ZnO solar cells with triple cation perovskite absorber
Although ZnO is a compatible electron transport layer (ETL) for perovskite solar cells (PSCs), the fact that MAPbI3 easily undergoes thermal decomposition on a low-temperature processed ZnO surface limits the use of one-step deposition of perovskite and hence the resulting photovoltaic performance. The triple cation perovskite prepared with a one-step deposition method is demonstrated to be a stable light absorber in highly efficient PSCs with low-temperature processed ZnO as the ETL.
J. Mater. Chem. A, 2017,5, 13439-13447
https://doi.org/10.1039/C7TA03331A
Dehydrogenation of cyclic amines by a coordinatively unsaturated Cp*Ir(III) phosphoramidate complex
The reaction of a Cp*Ir(III) phosphoramidate complex with secondary amines gives amine, imine-bound Cp*Ir(III) hydride complexes resulting from amine dehydrogenation.
Dalton Trans., 2017,46, 8621-8625
https://doi.org/10.1039/C7DT01499F
About this collection
Celebrating Excellence in Research: 100 Women of Chemistry is a collection of high quality papers from across the RSC Publishing portfolio. As the name of the collection suggests, the excellence comes first - all papers included have previously been judged to be of outstanding quality by the reviewers, editors, or readers.
You can read an Introduction to this collection on the RSC Publishing Blog.