Issue 20, 2024

Constructing poly(ethylene oxide)-based composite solid electrolytes: starting from the internal mechanism in batteries

Abstract

Solid polymer electrolytes (SPEs) represented by poly(ethylene oxide) (PEO) stand out in the realms of environmental sustainability and processability. Their high flexibility, a characteristic of polymer materials, renders them irreplaceable in applications such as wearable devices and flexible electronic components, positioning them as promising candidates for large-scale commercialization in the future. Nonetheless, PEO-based SPEs exhibit limitations in their ionic conductivity, electrochemical stability windows, and mechanical properties. This article delves into the intrinsic mechanisms of PEO-based SPEs, analyzes the genesis of their current limitations, and summarizes the progress in research strategies that modify PEO-based SPEs through the fabrication of composite solid electrolytes.

Graphical abstract: Constructing poly(ethylene oxide)-based composite solid electrolytes: starting from the internal mechanism in batteries

Article information

Article type
Review Article
Submitted
23 maj 2024
Accepted
21 avg 2024
First published
23 avg 2024

Mater. Chem. Front., 2024,8, 3446-3463

Constructing poly(ethylene oxide)-based composite solid electrolytes: starting from the internal mechanism in batteries

J. Wang, X. Liu, N. Zhang, P. Wang, Y. Zhu, J. Shu, C. Li and T. Yi, Mater. Chem. Front., 2024, 8, 3446 DOI: 10.1039/D4QM00428K

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