Issue 19, 2021

Renewable bio-based adhesive fabricated from a novel biopolymer and soy protein

Abstract

In this study, a bio-based soy protein adhesive derived from environmentally friendly and renewable enzymatic hydrolysis lignin (EHL), epoxidized soybean oil (ESO), and soy protein isolate (SPI), was successfully prepared. A novel biopolymer (EHL-ESO), as a multifunctional crosslinker, was firstly synthesized from modified EHL and ESO, and then crosslinked with soy protein isolate to obtain a bio-based soy protein adhesive. The structure, thermal properties, and adhesion performance of the obtained soy protein adhesives were determined by Fourier transform infrared spectroscopy (FTIR), thermogravimetric analysis (TGA), scanning electron microscopy (SEM) and wet shear strength. The maximum degradation temperature of SPI/EHL-ESO adhesives (332–343 °C) was higher than that of the pristine SPI adhesive (302 °C). Moreover, plywood bonded by the modified adhesive reached a maximum wet shear strength value of 1.07 MPa, a significant increase of 101.8% from the plywood bonded by pristine SPI adhesive. The enhancements in the thermal stability and wet shear strength were attributed to the formation of a dense crosslinking network structure. This work not only highlights the potential to replace petroleum-based polymers, but also presents a green approach to fabricate fully bio-based soy protein adhesive for preparing all-biomass wood composite materials.

Graphical abstract: Renewable bio-based adhesive fabricated from a novel biopolymer and soy protein

Article information

Article type
Paper
Submitted
29 jan 2021
Accepted
16 mar 2021
First published
23 mar 2021
This article is Open Access
Creative Commons BY license

RSC Adv., 2021,11, 11724-11731

Renewable bio-based adhesive fabricated from a novel biopolymer and soy protein

S. Chen, Y. Chen, Z. Wang, H. Chen and D. Fan, RSC Adv., 2021, 11, 11724 DOI: 10.1039/D1RA00766A

This article is licensed under a Creative Commons Attribution 3.0 Unported Licence. You can use material from this article in other publications without requesting further permissions from the RSC, provided that the correct acknowledgement is given.

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