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Abstract | Cited by

Several unimolecular photobase generators capable of catalyzing upconversion nanoparticle-assisted anionic thiol-epoxy click photopolymerization are presented. The fabricated polymers, with a curing depth of 11.8 cm, are dual-wavelength responsive and display shape memory function, showing great potential for the construction of smart medical devices and robots.

Graphical abstract: Photobase-catalysed anionic thiol-epoxy click photopolymerization under NIR irradiation: from deep curing to shape memory

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