Issue 32, 2024

A lignocellulosic biomass-derived polyurethane elastomer with high toughness and excellent crack tolerance

Abstract

Polyurethane (PU) elastomers play an indispensable role in our society due to their unique properties. The synthesis of high-performance PU elastomers from biomass is important to meet the needs of sustainable development. In the current study, liquified waste banana pseudo-stems are utilized as chain extenders for the synthesis of PU elastomers, and the obtained materials exhibit desirable tensile strength (up to ∼30 MPa), excellent toughness (∼389.7 MJ m−3) and exceptionally high fracture energy (∼666.9 kJ m−2). The extraordinary mechanical properties primarily stem from the strong energy dissipation of hydrogen bonds, microphase separation, and strain-induced crystallization. We believe that the current work can offer a new protocol for the preparation of sustainable polymers and the efficient utilization of waste natural resources.

Graphical abstract: A lignocellulosic biomass-derived polyurethane elastomer with high toughness and excellent crack tolerance

Supplementary files

Article information

Article type
Paper
Submitted
27 mar 2024
Accepted
26 jun 2024
First published
03 jul 2024

J. Mater. Chem. A, 2024,12, 20967-20974

A lignocellulosic biomass-derived polyurethane elastomer with high toughness and excellent crack tolerance

X. Guo, K. Zhang, Y. Dong, J. Qin, Y. Xiang and H. Zhu, J. Mater. Chem. A, 2024, 12, 20967 DOI: 10.1039/D4TA02029D

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