Issue 4, 2023

Designing strategies and enhancing mechanism for multicomponent high-entropy catalysts

Abstract

High-entropy materials (HEMs) are new-fashioned functional materials in the field of catalysis owing to their large designing space, tunable electronic structure, interesting “cocktail effect”, and entropy stabilization effect. Many effective strategies have been developed to design advanced catalysts for various important reactions. Herein, we firstly review effective strategies developed so far for optimizing HEM-based catalysts and the underlying mechanism revealed by both theoretical simulations and experimental aspects. In light of this overview, we subsequently present some perspectives about the development of HEM-based catalysts and provide some serviceable guidelines and/or inspiration for further studying multicomponent catalysts.

Graphical abstract: Designing strategies and enhancing mechanism for multicomponent high-entropy catalysts

Article information

Article type
Review Article
Submitted
21 nov 2022
Accepted
27 dec 2022
First published
03 jan 2023
This article is Open Access

All publication charges for this article have been paid for by the Royal Society of Chemistry
Creative Commons BY license

Chem. Sci., 2023,14, 771-790

Designing strategies and enhancing mechanism for multicomponent high-entropy catalysts

H. Xu, Z. Jin, Y. Zhang, X. Lin, G. Xie, X. Liu and H. Qiu, Chem. Sci., 2023, 14, 771 DOI: 10.1039/D2SC06403K

This article is licensed under a Creative Commons Attribution 3.0 Unported Licence. You can use material from this article in other publications without requesting further permissions from the RSC, provided that the correct acknowledgement is given.

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