Issue 8, 2023

Parsing the basic principles to build efficient heterostructures toward electrocatalysis

Abstract

Electrocatalysis can facilitate the reaction kinetics in many electrochemical energy conversion devices. Heterostructural catalysts are important candidates due to their sufficient tunability of components and electronic states. So far however, no basic principles have been provided to guide the rational selection of components and catalytic mechanisms of such high-efficiency heterostructures. This article is aimed at parsing the inherent principles of universal component selection strategies from the perspective of compatibility in electron structures or physical properties. The catalytic mechanism of these as-obtained heterostructural catalysts is also systematically analyzed, and the foreseeable research on the structure–activity relationship of heterostructural catalysts is then discussed. This would enable researchers in this field to conduct related works in a guiding way.

Graphical abstract: Parsing the basic principles to build efficient heterostructures toward electrocatalysis

Article information

Article type
Chemistry Frontiers
Submitted
17 jan 2023
Accepted
09 mrt 2023
First published
10 mrt 2023

Inorg. Chem. Front., 2023,10, 2220-2225

Parsing the basic principles to build efficient heterostructures toward electrocatalysis

J. Zhu and S. Mu, Inorg. Chem. Front., 2023, 10, 2220 DOI: 10.1039/D3QI00117B

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