Themed collection Journal of Materials Chemistry A HOT Papers
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Emerging electrochemical humidity sensors for zero power consumption and self-powered humidity detection: a perspective
This perspective summarizes recent advances in electrochemical humidity sensors and mainly focuses on three aspects: working principles; humidity sensing and power generation performances; self-powered humidity detection system.
J. Mater. Chem. A, 2024,12, 14975-14985
https://doi.org/10.1039/D3TA06283J
Hydrogen generation from atmospheric water
Green hydrogen, produced by water splitting with renewables, faces water scarcity issues. Atmospheric moisture, a stable source, offers an alternative. This article reviews technologies and challenges of using atmospheric water for H2 production.
J. Mater. Chem. A, 2024,12, 12381-12396
https://doi.org/10.1039/D4TA00848K
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Latest advances on in situ and operando X-ray-based techniques in photoelectrocatalytic systems
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03068K
Recent advances and perspectives of 1D/2D carbon materials for high-performance flexible zinc ion batteries
This review provides a summary of recent advancements in 1D/2D carbon materials (carbon nanotubes, graphene, MXenes, and carbon fibers) for FZIBs. It mainly introduces the functions of 1D/2D carbon materials in enhancing the performance of FZIBs.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03650F
Electrochemical CO2 reduction on Pd-based electrodes: from mechanism understanding to rational catalyst design
This review summarizes the progressive understanding of the mechanism of the Pd-catalyzed CO2 reduction reaction, together with recent advances in the rational design of Pd-based electrocatalysts.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02379J
Hybrid passive cooling: towards the next breakthrough of radiative sky cooling technology
A critical review of the regulatory mechanisms, structural design, cooling performance, and applications of hybrid cooling to advance its commercial use in passive cooling.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03122A
Regulation of intermediate microenvironment for efficient C–C coupling in electrochemical CO2 reduction
This review summarizes the recent progress in the regulation of local reaction intermediates and protons near active sites and discusses how their microenvironment affects the C–C coupling efficiency in the electrocatalytic CO2RR.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02224F
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Review of carbon-support-free platinum and non-platinum catalysts for polymer electrolyte fuel cells: will they feature in future vehicles?
Carbon-support-free platinum and non-platinum catalysts are reviewed to clarify the source of recent controversial results and to propose experimental conditions for their use in future fuel cell vehicles.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02664K
CO2-tolerant perovskite cathodes for enhanced solid oxide fuel cells: advancements, challenges, and strategic perspectives
This review analyzes advancements in CO2-resistant perovskite cathodes for solid oxide fuel cells, detailing CO2-poisoning mechanisms, evaluation methods, enhancement strategies, and characterization techniques for future cathode development.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02455A
Functional high-entropy alloys: promising catalysts for high-performance water splitting
State-of-the-art HEAs with outstanding water splitting performance is rationally designed, which provides a blueprint for the design of a next-generation platform for hydrogen regeneration.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02271H
Recent advances in scanning electrochemical microscopy for probing the sites in electrocatalysts
In this review, we summarized the application methods of SECM in electrochemical reactions and also discussed the challenges and prospects of SECM in characterizing the activity of electrocatalysts.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA01292E
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Prospects of polymer coatings for all solid-state and emerging Li-ion batteries
We summarize the influence of polymer coatings on cathode particles for electrochemical energy storage applications. We report on the effect of different polymer types, their properties, and their influence on thermo-electro-chemical behavior.
J. Mater. Chem. A, 2024,12, 14186-14205
https://doi.org/10.1039/D4TA01061B
Carbon-based double-metal-site catalysts: advances in synthesis and energy applications
Dual-metal site catalysts embedded in a carbon matrix (referred to as DMSCs) are gaining significant interest in sustainable energy research.
J. Mater. Chem. A, 2024,12, 11749-11770
https://doi.org/10.1039/D4TA00727A
Structure–property–performance relationship of vanadium- and manganese-based metal–organic frameworks and their derivatives for energy storage and conversion applications
The current review discusses on vanadium- and manganese-based metal–organic frameworks and their derivatives for energy storage and conversion applications along with the potential future advancements in these fields.
J. Mater. Chem. A, 2024,12, 11149-11175
https://doi.org/10.1039/D4TA00736K
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Advances in the direct electro-conversion of captured CO2 into valuable products
A comprehensive review of direct captured CO2 electro-conversion technology, a promising Carbon Capture and Utilization (CCU) technology that can achieve both techno-economic and environmental viability.
J. Mater. Chem. A, 2024,12, 10597-10613
https://doi.org/10.1039/D4TA01178C
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A review of noble metal-free high entropy alloys for water splitting applications
Nano-sized high entropy alloy (HEA) catalysts have attracted much attention as extraordinary electrocatalysts in water-splitting applications, i.e., the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER).
J. Mater. Chem. A, 2024,12, 9933-9961
https://doi.org/10.1039/D4TA00690A
Doping engineering of phosphorus-based polyanion-type cathodes for sodium storage: a review
This review addresses four key factors and underlying mechanisms of doping engineering from crystal-field, molecular orbital, and ligand-field theory.
J. Mater. Chem. A, 2024,12, 9268-9295
https://doi.org/10.1039/D4TA00652F
Metal/covalent–organic framework based thin film nanocomposite membranes for advanced separations
Metal/covalent organic frameworks (MOFs/COFs), with orderly aligned pores and adjustable pore characteristics, offer advantages over traditional fillers in constructing thin film nanocomposite (TFN) membranes for task-specific separations.
J. Mater. Chem. A, 2024,12, 7975-8013
https://doi.org/10.1039/D4TA00578C
Exploring the mechanisms of magnetic fields in supercapacitors: material classification, material nanostructures, and electrochemical properties
The review illustrates that the magnetic field effect can promote the generation of different nanostructures in material synthesis, achieve the transition from 1D to 2D and 3D structures in material assembly and improve the energy density of supercapacitor by the direct and indirect roles.
J. Mater. Chem. A, 2024,12, 6165-6189
https://doi.org/10.1039/D3TA07658J
Recent advances on metal–organic frameworks for deep purification of olefins
The efficient removal of trace impurities is significant for the production of high-purity olefins. This review summarizes the latest advancements in the deep purification of ethylene and propylene using MOF materials.
J. Mater. Chem. A, 2024,12, 5563-5580
https://doi.org/10.1039/D4TA00330F
Chemical pre-lithiation of LiMn2O4 balances the low first cycle efficiency of silicon anodes
Prelithiation of LiMn2O4 balances the low first cycle efficiency of silicon anodes for improvements in energy density and prospective cell chemistry enabled by naturally abundant elements.
J. Mater. Chem. A, 2024,12, 14354-14359
https://doi.org/10.1039/D4TA02544J
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Tailoring bismuth defects in Bi2WO6 nanosheets for photocatalytic C–H activation
Tailoring the bismuth defects in ultrathin Bi2WO6 nanosheets can efficiently activate the C–H bond in toluene to produce benzaldehyde under light irradiation.
J. Mater. Chem. A, 2024,12, 11841-11847
https://doi.org/10.1039/D4TA01573H
Novel heat storage ionomer binder for thermal management of Li-ion batteries
A novel heat storage ionomer binder with highly efficient heat-storage ability is proposed to function as an internal temperature conditioner, which allows the battery to function steadily over a wider temperature range.
J. Mater. Chem. A, 2024,12, 7508-7514
https://doi.org/10.1039/D3TA07490K
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Adsorptive molecular sieving of aromatic hydrocarbons over cyclic aliphatic hydrocarbons via an intrinsic/extrinsic approach
An efficient adsorptive molecular sieving strategy to separate aromatic and cyclic aliphatic hydrocarbons via an intrinsic/extrinsic approach.
J. Mater. Chem. A, 2024,12, 6875-6879
https://doi.org/10.1039/D3TA06602A
Three-dimensional porous NiCoP foam enabled high-performance overall seawater splitting at high current density
Three-dimensional porous NiCoP foam supported on Ni foam is a superb bifunctional electrocatalyst for overall seawater splitting, attaining a large current density of 1000 mA cm−2 at a low cell voltage of 1.97 V with robust stability over 300 hours.
J. Mater. Chem. A, 2024,12, 2680-2684
https://doi.org/10.1039/D3TA07898A
Synergistic integration of PdCu alloy on TiO2 for efficient photocatalytic CO2 reduction to CH4 with H2O
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA04354E
Electrolyte Engineering for the Mass Exfoliation of Graphene Oxide Across Wide Oxidation Degrees
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02654C
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Multinuclear solid-state NMR investigation of structurally diverse low-dimensional hybrid metal halide perovskites
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02833C
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Alkali-promoted indium oxide as highly active and selective catalyst for the photo-thermal CO2 hydrogenation
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA04387A
Surface Defects Induced Polarization Manipulation in Cu2SnS3 for Boosting Electrochemical CO2 Reduction
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA04092A
Mitigating Magnetic Frustration to Improve Single-Crystalline Nonstoichiometric Li1.06Ni0.90Mn0.04O2 for Lithium-Ion Batteries
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03933E
Magnetic field-governed kinetics in silicon dioxide-based anode towards high performing lithium-ion magneto-batteries
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03612C
Macroscale and durable near-zero wear performance on steel surfaces achieved by natural ternary deep eutectic solvents
Macroscale and durable near-zero wear performance of ternary deep eutectic solvent-based lubricants was elaborated by systematic experimental analysis and molecular dynamics simulation.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03216K
Band and microstructure engineering toward high thermoelectric performance in SnTe
AgBiS2 alloying combining with Ge doping facilitates the band convergence and suppresses the phonon transport, leading to a competitive zT of 1.6 in SnTe.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03729D
Tailoring of PVDF for retrieval of piezoelectric powders to optimize piezo-catalytic water treatment
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03219E
Device engineering of chalcogenide photodiodes with reduced dark current and enhanced stability for underwater light communication
For photodetectors based on chalcogenide semiconductor materials, a novel device structure has been proposed that utilizes a Se/Sb bilayer to replace conventional organic transport layers and noble metal electrodes.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02832E
High-output tubular triboelectric nanogenerator for wave energy collection and its application in self-powered anti-corrosion applications
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02760D
Cu2+-induced surface structure transformation on Au nanocubes from a concave to a convex configuration: mechanism and catalytic performance
Surface structures of Au nanocubes were tuned from concave to flat to convex using trace amounts of copper ions, and their corresponding catalytic performances were investigated.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03282A
Conjugated microporous polytriphenylamine as a high-performance anion-capture electrode for hybrid capacitive deionization with ultrahigh areal adsorption capacity
We report conjugated microporous polytriphenylamine as a high-performance anion-capture electrode for capacitive deionization (CDI), thus opening a new pathway for the rational design of advanced polymer-based anodes in CDI and beyond.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA04010D
Amphiphilic Interface for Constructing Uniform Composite Solid-State Electrolyte towards Long-Life All-Solid-State Sodium Metal Batteries
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03309D
In-situ Generated α-Co(OH)2/Co3Mo derived from Co-Mo-N for enhanced electrochemical hydrogen evolution reaction
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA04274C
Spatial decoupling strategy boosted alkaline hydrogen evolution for an efficient solar-driven AEM electrolyzer
Substrate modification achieves spatial decoupling of the hydrogen evolution reaction process, thereby greatly improving the efficiency and stability of the catalyst.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03872J
Improved and scalable method for the preparation of Sn-doped hexagonal tungsten bronze-type iron fluoride materials as cathode for sodium-ion batteries
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03267E
Carbon nanosheet-supported CrN nanoparticles as efficient and robust oxygen reduction electrocatalysts in acidic media and seawater Zn-air batteries
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA04066J
Achieving a safe high-voltage Lithium-metal battery by tailoring electrolyte system
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA02958E
Ultra-temperature and high thermal stability thermosensitive high-entropy ceramics up to 1873 K
The problem of stability degradation is solved by adjusting the lattice distortion, resulting in ceramics with the highest ceiling temperature and excellent thermal stability.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03260H
Improving the high-voltage high-rate performance of a P2 layered oxide cathode by a dual-ion doping strategy for sodium-ion batteries
Synergy between Ti4+ and F− dual-doping significantly improves the cycling stability of P2-Na0.67Ni0.33Mn0.67O2 at high voltage and enhances its rate performance by suppressing the P2–O2 transition.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03250K
Selective detection of NO using the perovskite-type oxide LaMO3 (M = Cr, Mn, Fe, Co, and Ni) as the electrode material for yttrium-stabilized zirconia-based electrochemical sensors
An yttrium-stabilized zirconia-based electrochemical sensor with LaCrO3 as the electrode material was used to selectively detect NO.
J. Mater. Chem. A, 2024,12, 18234-18247
https://doi.org/10.1039/D4TA02809K
Ultrahigh energy storage capacities in high-entropy relaxor ferroelectrics
This study shows that entropy engineering can enhance the energy-storage performance of lead-free BNT-based dielectrics, achieving a recoverable energy density of 11.24 J cm−3 and 88.3% efficiency, with excellent stability and rapid discharge.
J. Mater. Chem. A, 2024,12, 18224-18233
https://doi.org/10.1039/D4TA03637A
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Ultrathin NiO nanosheets anchored to a nitrogen-doped dodecahedral carbon framework for aqueous potassium-ion hybrid capacitors
The hierarchical and interconnected architecture of NiO/N-HPC promotes efficient electrolyte penetration, shortens ion transport path, and accelerates reaction kinetics, leading to a high-performance aqueous potassium-ion hybrid capacitor.
J. Mater. Chem. A, 2024,12, 18157-18166
https://doi.org/10.1039/D4TA01608D
Analysis of the mechanism for enhanced crystalline quality of wide-bandgap Cu(In,Ga)Se2 films by pre-deposited Ag
Ag doping achieves high-quality wide-bandgap CIGS films by controlling the (In,Ga)2Se3 film growth preference and Ag–Cu ion exchange process.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA02513J
Low-temperature suitability of flexible photo-rechargeable devices integrated with hydrogel-based lithium-ion batteries and perovskite solar cells
The flexible photo-rechargeable device with an OEE of 12.88% displays good low-temperature suitability and safety without overcharge-induced thermal runaway.
J. Mater. Chem. A, 2024,12, 18214-18223
https://doi.org/10.1039/D4TA03076A
In situ switchable nanofiber films based on photoselective asymmetric assembly towards year-round energy saving
An in situ switchable photoselective polymer film, assembled from asymmetric optical nanofibers, achieves high-threshold power regulation through elimination and restoration of scattering interfaces, facilitating a wide range of temperature control.
J. Mater. Chem. A, 2024,12, 18304-18312
https://doi.org/10.1039/D4TA03558E
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Controlling the steepness of gate-opening behavior on elastic layer-structured metal–organic framework-11 via solvent-mediated phase transformation
The phase of the precursor of ELM-11 affects the steepness of its gate-opening behavior, and this phase can be controlled by solvent-mediated phase transformation.
J. Mater. Chem. A, 2024,12, 18193-18203
https://doi.org/10.1039/D4TA02068E
Iron single-atom anchored N-doped carbon: an efficient catalyst for one-pot, scaled-up pentazolate synthesis
An efficient and recyclable iron single-atom catalyst with FeN4 sites has been fabricated, which can facilitate the formation of an Fe(IV)O intermediate and achieve scaled-up pentazolate synthesis via a three-step, one-pot process.
J. Mater. Chem. A, 2024,12, 18096-18103
https://doi.org/10.1039/D4TA03312D
Probing metal/high-entropy perovskite heterointerfaces for efficient and sustainable CO2 electroreduction
A novel high-entropy Sr2Fe0.4V0.4Mo0.4Ni0.4Ti0.6O6−δ (SFVMNT) perovskite, coated with in situ exsolved NiFe alloy nanoparticles, is proposed as a promising cathode material for solid electrolysis cells for CO2 electrolysis.
J. Mater. Chem. A, 2024,12, 18182-18192
https://doi.org/10.1039/D4TA02372B
Achieving long-lived photogenerated holes in ZnIn2S4 loaded with CoOx clusters for enhanced photocatalytic pure water splitting
Ultra-small CoOx clusters efficiently capture holes and prolong the lifetime of trapped holes, as well as boost surface water oxidation, thus remarkably improving the photocatalytic pure water splitting performance of ZnIn2S4.
J. Mater. Chem. A, 2024,12, 18204-18213
https://doi.org/10.1039/D4TA02620A
All-inorganic Sb2S3-based two-terminal tandem solar cells enable over 10.9% efficiency employing a concise interconnection layer
Sb2S3-based two terminal tandem solar cells (2T-TSCs) are reported for the first time with the assistance of lead sulfide quantum dot rear cells. The PCE of the champion TSC reaches 10.92%. Our work opens the door for Sb2S3 based 2T-TSCs.
J. Mater. Chem. A, 2024,12, 18148-18156
https://doi.org/10.1039/D4TA01881H
Biotopologically structured composite materials for low temperature energy storage
A biotopologically structured configuration constructed by an energy-saving electrodeposition method for low-temperature supercapacitors.
J. Mater. Chem. A, 2024,12, 18137-18147
https://doi.org/10.1039/D4TA02625J
Balancing the triple conductivity of zinc-doped cathodes for proton-conducting solid oxide fuel cells
The Zn-doped BCF36 cathode boosts proton conductivity, lowers hydration energy and achieves a peak power density of 998.6 mW cm−2 at 600 °C with a polarization resistance of 0.151 Ω cm2 for a single cell with the BCFZ10 cathode.
J. Mater. Chem. A, 2024,12, 18175-18181
https://doi.org/10.1039/D4TA02584A
Atomically ordered Ir3Ti intermetallics for pH-universal overall water splitting
Atomically ordered Ir3Ti intermetallics on carbon nanotubes exhibit remarkable performance for pH-universal overall water splitting.
J. Mater. Chem. A, 2024,12, 18167-18174
https://doi.org/10.1039/D4TA02304H
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Advancing anode-less lithium metal batteries: ZnF2 modification and in situ structural regulation for enhanced performance
A novel LiF@LiZn10/Li composite foil was developed as an effective anode for lithium metal batteries. The uniform lithiophilic substrate and the LiF-rich SEI optimize Li+ deposition.
J. Mater. Chem. A, 2024,12, 18127-18136
https://doi.org/10.1039/D4TA02431A
High-strength thermochromic and mechanochromic liquid-crystal elastomers with responsive shape memory and dynamic adhesion
Versatile CLCEs with a loosely crosslinking density were developed, which exhibit exceptional high mechanical performances and responsive functionalities including thermochromic, mechanochromic, shape memory, and dynamic adhesion behaviors.
J. Mater. Chem. A, 2024,12, 18117-18126
https://doi.org/10.1039/D4TA02010C
N/O coordinated s-block potassium atoms as highly active sites for electroreduction of CO2 to CO
The synthesized K–N, O/C catalyst demonstrates remarkable CO selectivity with over 90% Faraday efficiency (FE) in a wide potential window between −0.5 V and −0.9 V vs. RHE and the FE of CO is nearly unchanged during 24 h stability experiment.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03780D
Structurally oriented black phosphorus/MXene heterostructured fibers for flexible supercapacitors with enhanced ion transport and capacitive charge storage
Structurally oriented BP/Ti3C2Tx heterostructured fibers with high conductivity, excellent mechanical properties and high specific capacitance were fabricated via electrostatic assembly for high-performance flexible fiber supercapacitors.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03914A
Accelerating the generation and discovery of high-performance donor materials for organic solar cells by deep learning
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03944K
Generating zeolite crystals with mesoscopic aperiodic structure to promote catalytic hydroisomerization
Nanocrystalline *MRE zeolite domains registered in quasicrystal-like, decagonal order is generated, which has strong acidity, reduced unidimensional channel length and mesopores, exhibiting enhanced n-dodecane hydroisomerization properties.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA01303D
Design and synthesis of organic radical functionalized vanadium pentoxide towards long-life aqueous zinc ion batteries
A facile “two-in-one” strategy was proposed to achieve a V2O5-TEMPO cathode for large capacity and long-life zinc–organic batteries.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03354J
Reactivity and durability of TiO2 photoanodes with dominant high-energy (211) facets
We report a successful preparation of a TiO2 photoanode with dominant (211) facets on various substrates. This photoanode can be used in rooftop PEC systems due to its low cost, high stability, good durability and acceptable efficiency.
J. Mater. Chem. A, 2024, Advance Article
https://doi.org/10.1039/D4TA03737E
Revealing the critical pore size for hydrogen storage via simultaneous enclathration and physisorption in activated carbon
J. Mater. Chem. A, 2024, Accepted Manuscript
https://doi.org/10.1039/D4TA03607G
About this collection
This on-going web collection features all the articles published in Journal of Materials Chemistry A in 2024 marked as HOT, as recommended by referees. Congratulations to all the authors whose articles are featured!