Themed collection 2023 Materials Chemistry Frontiers HOT articles
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Surface engineering in CsPbX3 quantum dots: from materials to solar cells
Summarized CsPbX3 QD surface engineering strategies to achieve high-efficiency and high-stability PQD solar cells.
Mater. Chem. Front., 2024,8, 2029-2055
https://doi.org/10.1039/D3QM00911D
Research progress of robust binders with superior mechanical properties for high-performance silicon-based lithium-ion batteries
The mechanical properties of binders are emphasized: the intrinsic mechanical properties of binders and the adhesive strength of the binders with current collectors and active materials. The electronic and ionic conductivities of binders are introduced.
Mater. Chem. Front., 2024,8, 1480-1512
https://doi.org/10.1039/D3QM00839H
Perovskite and layered perovskite oxynitrides for efficient sunlight-driven artificial synthesis
Perovskite and layered perovskite oxynitrides are regarded as promising visible-light-responsive semiconductors for efficient artificial photosynthesis to produce renewable value-added energy resources, including H2, formic acid, and ammonia.
Mater. Chem. Front., 2024,8, 1451-1479
https://doi.org/10.1039/D3QM01019H
Functionalization of pillar[n]arenes towards optically responsive systems via host–guest interactions
In this review, we discuss progress in the field of pillar[n]arene-based optical response systems, focusing on color, fluorescence, circular dichroism, and circularly polarized luminescence signal changes via host–guest interactions.
Mater. Chem. Front., 2024,8, 1212-1229
https://doi.org/10.1039/D3QM01176C
Recent advances on three-dimensional ordered macroporous metal oxide-based photoelectrodes for photoelectrochemical water splitting
Recent advances in 3DOM metal oxide-based photoelectrodes for PEC water splitting are summarized. The advantages of an ordered structure from the perspective of photo-electrocatalysis mechanism and morphological design are also introduced.
Mater. Chem. Front., 2024,8, 1230-1249
https://doi.org/10.1039/D3QM00990D
Recent advances in metal–organic frameworks for water absorption and their applications
Metal–organic frameworks (MOFs) are promising water adsorbents with a controllable absorption humidity range, superior water capacity, and tailorable regeneration conditions.
Mater. Chem. Front., 2024,8, 1171-1194
https://doi.org/10.1039/D3QM00484H
Research advances and applications of ZIF-90 metal–organic framework nanoparticles in the biomedical field
A schematic illustration of ZIF-90 nanocomposites applied to anticancer therapy, biomedical imaging and other fields for the treatment of different diseases.
Mater. Chem. Front., 2024,8, 1195-1211
https://doi.org/10.1039/D3QM01020A
Recent advances in red-emissive carbon dots and their biomedical applications
This review mainly summarizes the research advances in synthetic strategies, optical properties, and biomedical applications of red-emissive carbon dots in recent years.
Mater. Chem. Front., 2024,8, 930-955
https://doi.org/10.1039/D3QM00968H
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Recent advances in metal-based electrocatalysts: from fundamentals and structural regulations to applications in anion-exchange membrane fuel cells
We present a comprehensive understanding of the alkaline hydrogen oxidation reaction (HOR), ammonium oxidation reaction (AOR), and oxygen reduction reaction (ORR) based on metal catalysts for H2 or NH3-fueled alkaline exchange membrane fuel cells.
Mater. Chem. Front., 2024,8, 903-929
https://doi.org/10.1039/D3QM00947E
Reinforcing built-in electric field to enable efficient carrier extraction for high-performance perovskite solar cells
This review presents an overview of the carrier separation and extraction mechanism influenced by the built-in electric field (BEF) in PSCs and various strategies used to enhance the BEF.
Mater. Chem. Front., 2024,8, 956-985
https://doi.org/10.1039/D3QM00956D
Two dimensional oxides for oxygen evolution reactions and related device applications
The oxygen evolution reaction (OER) is a key anode reaction for many renewable energy devices, such as electrocatalytic water splitting devices, Zn–air batteries and CO2 electrolyzers.
Mater. Chem. Front., 2024,8, 880-902
https://doi.org/10.1039/D3QM00848G
Applications of multifunctional metal–organic frameworks in perovskite photovoltaics: roles, advantages and prospects
Recent progress of applications of multifunctional MOFs in achieving efficient, durable and eco-friendly perovskite photovoltaics is systematically reviewed, and the profound prospects of MOFs inadvancing development of optoelectronics are outlined.
Mater. Chem. Front., 2024,8, 869-879
https://doi.org/10.1039/D3QM01001E
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Self-assembled molecules as selective contacts for efficient and stable perovskite solar cells
In this review, we summarize the recent advances about self-assembled molecules (SAMs) applied as selective hole or electron contacts for perovskite solar cells.
Mater. Chem. Front., 2024,8, 681-699
https://doi.org/10.1039/D3QM01017A
Panchromatic porphyrin-based dye-sensitized solar cells: from cosensitization to concerted companion dye approaches
In this review, cosensitization, concerted companion and other strategies, enabling porphyrin sensitizers to achieve panchromatic absorption and the resulting high photovoltaic performance, are briefly summarized and discussed.
Mater. Chem. Front., 2024,8, 652-680
https://doi.org/10.1039/D3QM00770G
Recent progress in bimetallic carbide-based electrocatalysts for water splitting
This review provides recent progresses in bimetallic carbides (Bi-TMCs) catalysts for the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) in water splitting.
Mater. Chem. Front., 2024,8, 627-651
https://doi.org/10.1039/D3QM00819C
Advances in the mechanism investigation for the oxygen evolution reaction: fundamental theory and monitoring techniques
Fundamental theory and monitoring techniques of the OER mechanism: a review.
Mater. Chem. Front., 2024,8, 603-626
https://doi.org/10.1039/D3QM00935A
Towards separator safety of lithium-ion batteries: a review
The recent advance of high-safety separators with high mechanical strength, high thermal stability and good lithium dendritic resistance is the main focus in this review. The future challenges and perspectives of separators are provided for building high safety rechargeable lithium batteries.
Mater. Chem. Front., 2024,8, 309-340
https://doi.org/10.1039/D3QM00951C
Recent progress on 2D material-based nanoarchitectures for small molecule electro-oxidation
In this review, we comprehensively summarize the recent advancements in the controlled fabrication as well as relationship between 2D nanoarchitectures and electrochemical performances in the electro-oxidation of small molecules used in DLFC.
Mater. Chem. Front., 2024,8, 404-433
https://doi.org/10.1039/D3QM00905J
Anti-freezing multifunctional conductive hydrogels: from structure design to flexible electronic devices
In this review, we systematically provide an overview of anti-freezing multifunctional conductive hydrogel-based flexible electronics and summarize the design strategies, properties, applications and perspectives.
Mater. Chem. Front., 2024,8, 381-403
https://doi.org/10.1039/D3QM00902E
Functional dielectric materials for high-performance solid-state batteries
Functional dielectric materials can regulate the migration, diffusion and deposition of cations in solid-state batteries, leading to high performance.
Mater. Chem. Front., 2024,8, 354-380
https://doi.org/10.1039/D3QM00964E
Polypyrrole micro/nanostructures and their soft materials in versatile forms: construction and applications
Key issues regarding the syntheses of polypyrrole nanomaterials and their recent application were discussed. Polypyrrole derived dispersions, hydrogels, membranes and composites were outlined by considering improved conductivity and processability.
Mater. Chem. Front., 2024,8, 434-454
https://doi.org/10.1039/D3QM00826F
Coupling electrochemical CO2 reduction with value-added anodic oxidation reactions: progress and challenges
This review presents recent advances and future challenges of emerging and potential alternative anodic reactions with high energy-efficiency and value-added products in overall CO2 electrolysis.
Mater. Chem. Front., 2024,8, 341-353
https://doi.org/10.1039/D3QM00625E
Colorful variation of tetraphenylethene derivatives in the solid state
This review provides a clear overview of the multi-stimuli responsive properties of tetraphenylethene derivatives in the solid state.
Mater. Chem. Front., 2024,8, 104-132
https://doi.org/10.1039/D3QM00621B
Critical challenges and opportunities for the commercialization of alkaline electrolysis: high current density, stability, and safety
Alkaline electrolysis technology, which enables the production of “green hydrogen,” holds significant importance in the global pursuit of carbon neutrality.
Mater. Chem. Front., 2024,8, 41-81
https://doi.org/10.1039/D3QM00730H
The role of organic spacers in 2D/3D hybrid perovskite solar cells
This review highlights the crucial role of organic spacers in the fabrication process and formation mechanism of different types of 2D/3D perovskites for PSCs including the bulk incorporation model, surface treatment model, and the coexisting model.
Mater. Chem. Front., 2024,8, 82-103
https://doi.org/10.1039/D3QM00726J
Materials design and applications of n-type and ambipolar organic electrochemical transistors
With the rapid development of n-type and ambipolar OECT materials, OECTs have been widely used in constructing logic circuits, electrophysiological recording, biosensing, and neuromorphic computing.
Mater. Chem. Front., 2024,8, 133-158
https://doi.org/10.1039/D3QM00828B
A critical review on amorphous–crystalline heterostructured electrocatalysts for efficient water splitting
This review presents comprehensive details on recent developments in the fabrication of different amorphous–crystalline heterostructures, their compositions, and the resulting physicochemical properties for OER, HER, and overall water splitting.
Mater. Chem. Front., 2023,7, 6254-6280
https://doi.org/10.1039/D3QM00940H
Effects of metal size on supported catalysts for CO2 hydrogenation
Tuning the metal size in loaded catalysts to increase the activity and selectivity of desirable products in CO2 hydrogenation is widely investigated in heterogeneous catalysis.
Mater. Chem. Front., 2023,7, 6411-6426
https://doi.org/10.1039/D3QM00384A
Recent advances in mechanistic understanding and catalyst design for alkaline hydrogen evolution reactions
This review presents recent progress in alkaline HERs, covering mechanistic insights, catalyst development, and device performance. It also addresses challenges and future directions for high-performance alkaline HER catalysts.
Mater. Chem. Front., 2023,7, 6366-6388
https://doi.org/10.1039/D3QM00600J
Paradigm in single-atom electrocatalysts for dinitrogen reduction to ammonia
Single-atom catalysts (SACs) are a new class of electrocatalysts for the electrochemical nitrogen reduction reaction.
Mater. Chem. Front., 2023,7, 6427-6445
https://doi.org/10.1039/D3QM00269A
Progress in optical properties of chiral metal clusters: circular dichroism and circularly polarized luminescence
This review aims to elucidate how the regulation of chiral metal cluster structures affects their circular dichroism or circularly polarized luminescence (CPL) signals, with the ultimate objective of providing a reference for the rational design of CPL materials in the future.
Mater. Chem. Front., 2023,7, 6389-6410
https://doi.org/10.1039/D3QM00747B
DNA as highly biocompatible carriers for drug delivery
This review aims to provide an overview of existing research on the use of various nucleic acid-based nanocarriers for drug delivery and summarize recent advances, including targeting strategies of DNA-based carriers, and the types of drugs that can be incorporated into the carriers.
Mater. Chem. Front., 2023,7, 6345-6365
https://doi.org/10.1039/D3QM00395G
Polymer-based electrolytes for solid-state lithium batteries with a wide operating temperature range
Polymer-based electrolytes with regulated molecular structures demonstrate excellent temperature tolerance and are ideal for solid-state lithium batteries.
Mater. Chem. Front., 2023,7, 6305-6317
https://doi.org/10.1039/D3QM00759F
Acid-scavenging separators promise long-term cycling stability of lithium-ion batteries
Acid-scavenging separators are an efficient way to inhibit the acidification of traditional LiPF6-containing electrolytes. This paper reviews the development and achievements of acid-scavenging separators to enhance their practical application capabilities and future developments.
Mater. Chem. Front., 2023,7, 6318-6344
https://doi.org/10.1039/D3QM00709J
Advances in organic field-effect transistors based on metal–organic coordination materials and applications
The recent developments in organic field-effect transistors based on metal–organic coordination materials and related applications are reviewed.
Mater. Chem. Front., 2023,7, 6281-6304
https://doi.org/10.1039/D3QM00720K
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3D shape morphing of stimuli-responsive composite hydrogels
Programmable 3D shape morphing of stimuli-responsive hydrogels is of great interest for the fabrication of soft actuators and robots. The corporation of hydrogel matrices and functional additives is discussed in this review.
Mater. Chem. Front., 2023,7, 5989-6034
https://doi.org/10.1039/D3QM00856H
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Cross-linking strategies for hole transport/emissive layers in quantum-dot light-emitting diodes
To avoid the interlayer erosion challenge in the IJP process and direct patterning process of the QD emissive layer (EML), cross-linking strategies have been introduced to construct solvent-resistant films (hole transport layers or QD EMLs) upon exposure to heat or light.
Mater. Chem. Front., 2023,7, 6130-6140
https://doi.org/10.1039/D3QM00831B
Rational design of efficient electrocatalysts for hydrogen production by water electrolysis at high current density
Challenges and design strategies of electrocatalysts for high-current–density water electrolysis.
Mater. Chem. Front., 2023,7, 6035-6060
https://doi.org/10.1039/D3QM00722G
Application of MOF-derived materials as electrocatalysts for CO2 conversion
This review summarizes the four main synthesis strategies of MOF-derived materials, and the feasibility and challenges of MOF-derived materials in ECO2RR are discussed.
Mater. Chem. Front., 2023,7, 6107-6129
https://doi.org/10.1039/D3QM00835E
Variable halide perovskites: diversification of anti-counterfeiting applications
This review emphasizes how the dimensionality, coordination number and bond length of halide perovskites (HPs) regulate their photoluminescence. HPs have good application potential due to their sensitivity to light, solvent, heat etc., facilitating anti-counterfeiting and encryption/decryption.
Mater. Chem. Front., 2023,7, 6085-6106
https://doi.org/10.1039/D3QM00595J
Recent advances in designing solid-state electrolytes to reduce the working temperature of lithium batteries
This review paper summarizes the current methods to reduce the operating temperature of solid-state lithium batteries.
Mater. Chem. Front., 2023,7, 6061-6084
https://doi.org/10.1039/D3QM00662J
Recent advances in regulating the excited states of conjugated thermally activated delayed fluorescence polymers for high-efficiency OLEDs
Several methods are summarized for controlling the excited states of TADF conjugated polymers, covering: (a) maintaining suitable ΔEST; (b) localized triplet excited state assisted reverse intersystem crossing; (c) hyperfine coupling facilitates reverse intersystem crossing.
Mater. Chem. Front., 2023,7, 6141-6153
https://doi.org/10.1039/D3QM00799E
Recent progress in metal–organic frameworks for the separation of gaseous hydrocarbons
This review highlights recent research progress in MOF materials for the important separation of gaseous hydrocarbons, especially for ethylene, propylene, and butadiene. The uniqueness of MOFs to achieve those progress is also outlined.
Mater. Chem. Front., 2023,7, 5693-5730
https://doi.org/10.1039/D3QM00430A
Recent advances in aggregation-induced emission (AIE)-based chemosensors for the detection of organic small molecules
This review provides an overview of the progress in the development of AIE-based organic small molecule probes for detecting biologically important molecules, drug molecules, volatile organic compounds, and explosives over the past five years.
Mater. Chem. Front., 2023,7, 5561-5660
https://doi.org/10.1039/D3QM00679D
Macroscopic alignment of metal–organic framework crystals in specific crystallographic orientations
This review explores synthetic strategies for macroscopic aligned MOFs, enhancing properties without structural designs or post-synthetic reactions.
Mater. Chem. Front., 2023,7, 5545-5560
https://doi.org/10.1039/D3QM00678F
Non-precious metal-based catalysts for water electrolysis to produce H2 under industrial conditions
The design strategies for improving mass transfer, intrinsic activity, and durability of non-precious catalysts, and the scale-up methods for industrial application are summarized to reduce the cost of hydrogen production.
Mater. Chem. Front., 2023,7, 5661-5692
https://doi.org/10.1039/D3QM00557G
MXene-based nanocomposites: emerging candidates for the removal of antibiotics, dyes, and heavy metal ions
Fabrication of MXene-based nanocomposites. Photocatalytic properties of nanocomposites. MXene-based membranes for the separation of toxic pollutants, such as antibiotic drugs, dyes, etc. MXene-based nanocomposites as absorbents for heavy metal removal.
Mater. Chem. Front., 2023,7, 5519-5544
https://doi.org/10.1039/D3QM00667K
Chevrel phases: synthesis, structure, and electrocatalytic applications
This review summarizes the current advancements of Chevrel phases as electrocatalysts, covering the crystalline structures, synthesis methods, and electrocatalysis applications, with a focus on how crystal structure affects the performance.
Mater. Chem. Front., 2023,7, 5500-5518
https://doi.org/10.1039/D3QM00546A
Key modification strategies for the rational design of hematite to promote photoelectrochemical water oxidation: a review of recent advances
In this review article, multiple modification strategies for hematite, including controlling the morphology, heterojunction engineering, doping engineering, modification of co-catalyst and other modifications are proposed.
Mater. Chem. Front., 2023,7, 5333-5354
https://doi.org/10.1039/D3QM00927K
Ionic liquids in the scope of lithium-ion batteries: from current separator membranes to next generation sustainable solid polymer electrolytes
We present a review on the current state-of-the-art of ionic liquids for the development of electrolytes, both conventional and solid-state. This review article provides a thorough summary of the developments achieved in this field.
Mater. Chem. Front., 2023,7, 5046-5062
https://doi.org/10.1039/D3QM00852E
Recent advances in the rational design of alkaline OER catalysts: from electronic structures to industrial applications
Rational design of high-performance OER catalyst based on the fundamental electronic structure to industrial requirements.
Mater. Chem. Front., 2023,7, 5187-5214
https://doi.org/10.1039/D3QM00588G
Recent advances in nanotechnology for combating Alzheimer's disease
This review provides an overview of recent advances in nanotechnology that are achieved to improve the therapeutic efficiency for treating Alzheimer's disease.
Mater. Chem. Front., 2023,7, 5171-5186
https://doi.org/10.1039/D3QM00493G
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Porous organic cages for gas separations
This review aims to provide a comprehensive overview of the recent advancements made in gas separations utilizing porous organic cages (POCs).
Mater. Chem. Front., 2023,7, 5247-5262
https://doi.org/10.1039/D3QM00715D
Fabrication strategies for high quality halide perovskite films in solar cells
Fabrication strategies for high quality halide perovskite films in solar cells are reviewed from the aspects of intermediate engineering, reaction-controlled, additive-controlled, and mass-controlled crystal growth.
Mater. Chem. Front., 2023,7, 5309-5332
https://doi.org/10.1039/D3QM00496A
Synthesis and advantages of spinel-type composites
In this review, basic structural characteristics of spinels are introduced and then the composite effects and methods are highlighted. An overview focusing on different synthesis and modulation methods is given, based on an in-depth understanding of the relationship between structure and activity.
Mater. Chem. Front., 2023,7, 5288-5308
https://doi.org/10.1039/D3QM00416C
Organic–inorganic hybrid perovskite materials and their application in transistors
Hybrid organic–inorganic perovskites (HOIPs) are emerging materials for versatile electronics. This review focuses on the HOIP-based field-effect transistor (FET) and the potential applications of HOIPs in functional FETs.
Mater. Chem. Front., 2023,7, 5215-5246
https://doi.org/10.1039/D3QM00697B
Organic luminescent crystals: role of packing structures and optical properties
This review focuses on understanding the role of molecular packing structures and optical properties in π-conjugated organic luminescent crystals. The various applications and future prospects of this research field are also proposed.
Mater. Chem. Front., 2023,7, 5104-5119
https://doi.org/10.1039/D3QM00494E
Metal–organic frameworks for the photocatalytic oxygen reduction reaction to hydrogen peroxide
We detail the production process of H2O2 involving mechanisms, detection methods, and performance evaluation, and also summarize and predict the modifying ways of MOF catalysts for the photocatalytic ORR to H2O2, incorporating the challenges faced.
Mater. Chem. Front., 2023,7, 5120-5139
https://doi.org/10.1039/D3QM00468F
Carbohydrate–macrocycle conjugates for biomedical applications
We summarized the development of macrocycle-carbohydrate conjugates and their biomedical application in the past decade, and provided our contention regarding the future trend of this topic.
Mater. Chem. Front., 2023,7, 5263-5287
https://doi.org/10.1039/D3QM00540B
MOFs meet membrane: application in water treatment and separation
Metal–organic frameworks (MOFs) are solid crystalline materials formed by the self-assembly of organic ligands and metal ions or clusters. Combining the advantages of membrane separation and MOFs, MOFs-based membranes are used in water treatment.
Mater. Chem. Front., 2023,7, 5140-5170
https://doi.org/10.1039/D3QM00487B
Recent progress in organic–metal complexes for organic photovoltaic applications
Organic–metal complexes (OMCs) are endowed with new functions and properties due to the characteristics of valence changes of metal ions and the diversity of organic molecular structures.
Mater. Chem. Front., 2023,7, 5063-5103
https://doi.org/10.1039/D3QM00603D
Recent advances in the synthesis and catalytic applications of metal–organic framework/covalent organic framework composites
MOF/COF composites constructed by heterojunction, functionalization, or integration show enhanced performance in photo-, thermo-, and electrocatalysis. This review is informative for rational design and mechanism understanding of MOF/COF catalysts.
Mater. Chem. Front., 2023,7, 4782-4809
https://doi.org/10.1039/D3QM00565H
Recent advances in interface engineering of thermoelectric nanomaterials
Thermoelectric (TE) materials are auspicious candidates for direct thermal–electrical energy conversion applications.
Mater. Chem. Front., 2023,7, 4707-4722
https://doi.org/10.1039/D3QM00419H
Polymeric nanomaterials with aggregation-induced emission characteristics
Polymeric nanomaterials with aggregation-induced emission (AIE) characteristics have attracted significant attention from the scientific community because of their extensive biomedical applications.
Mater. Chem. Front., 2023,7, 4768-4781
https://doi.org/10.1039/D3QM00562C
Recent progress in borate-based short-wavelength nonlinear optical crystals with boron–oxygen skeleton modification
Recent progress and prospects of borate-based short-wavelength NLO crystals with modified boron-oxygen skeleton have been surveyed and analyzed focusing on the crystal structure features, cutoff edges, birefringence and SHG responses.
Mater. Chem. Front., 2023,7, 4683-4692
https://doi.org/10.1039/D3QM00451A
Near-infrared organic light-emitting materials, devices and applications
In this article, we overview the latest advancements in organic near-infrared (NIR) materials, light-emitting devices and their applications. Moreover, we discuss the current limitations and future prospects for the NIR technology.
Mater. Chem. Front., 2023,7, 4744-4767
https://doi.org/10.1039/D3QM00585B
Electronic and geometric modulations of catalysts for electrochemical CO2 reduction reaction
Modulations of electronic structures of active sites and geometric structures of catalyst supports play important roles in electrocatalytic activity and selectivity for the carbon dioxide reduction reaction.
Mater. Chem. Front., 2023,7, 4723-4743
https://doi.org/10.1039/D3QM00364G
Eco-friendly and ultrathin solar cells featuring nanocrystals: advances and perspectives
A comprehensive and critical review of the emerging eco-friendly solar cells such as AgBiS2 is presented with the goal of further advancing the photovoltaic performance and stability.
Mater. Chem. Front., 2023,7, 4693-4706
https://doi.org/10.1039/D3QM00334E
Recent advances and perspectives of emerging two-dimensional transition metal carbide/nitride-based materials for organic pollutant photocatalysis
This review outlines the fabrication strategies, morphological structures, electronic properties and applications of MXene based materials for photocatalysis in the treatment of recalcitrant organic pollutants (dyes, phenols, antibiotics and pharmaceuticals).
Mater. Chem. Front., 2023,7, 4658-4682
https://doi.org/10.1039/D3QM00288H
Progress of polyethersulfone composites and their applications in biomedical engineering
This review summarizes recent advances in polyethersulfone composites membranes, microspheres and fibers, and corresponding applications including hemodialysis, blood perfusion, extracorporeal membrane oxygenation etc.
Mater. Chem. Front., 2023,7, 4215-4235
https://doi.org/10.1039/D3QM00357D
About this collection
Read our on-going collection of the hottest research published as advanced article from Materials Chemistry Frontiers in 2023. These articles are recommended by reviewers as being of significant novelty and interest. Congratulations to all the authors whose articles are featured!