Issue 10, 2023

Improving performances of the electrode/electrolyte interface via the regulation of solvation complexes: a review and prospect

Abstract

The electrode/electrolyte interface (EEI) is a research hotspot in lithium-ion batteries, while the electrolyte solvation complex can be regarded as a factor that cannot be ignored in determining the performance of the EEI. From the perspective of the electrolyte solvation complex, this review summarizes the effects of solvation complexes on the composition of an EEI film and the Li+ desolvation process, and further clarifies the internal mechanism of the electrolyte composition controlling solvation chemistry. Finally, combined with doubtful points that are not comprehensively considered in the regulation of solvated complexes, this review puts forward some cutting-edge views, which are of great significance for future guidance in improving the performance of lithium-ion batteries.

Graphical abstract: Improving performances of the electrode/electrolyte interface via the regulation of solvation complexes: a review and prospect

Article information

Article type
Minireview
Submitted
28 Dec. 2022
Accepted
06 Febr. 2023
First published
07 Febr. 2023

Nanoscale, 2023,15, 4772-4780

Improving performances of the electrode/electrolyte interface via the regulation of solvation complexes: a review and prospect

Y. Quan, S. Wu, K. Yang, L. Hu, X. Zhang, X. Hu, H. Liang and S. Li, Nanoscale, 2023, 15, 4772 DOI: 10.1039/D2NR07273D

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