Issue 47, 2022

Coincidence study of core-ionized adamantane: site-sensitivity within a carbon cage?

Abstract

We investigate the fragmentation dynamics of adamantane dications produced after core-ionization at the carbon edge followed by Auger decay. The combination of high-resolution electron spectroscopy, energy-resolved electron-ion multi-coincidence spectroscopy and different theoretical models allows us to give a complete characterization of the processes involved after ionization. We show that energy- and site-sensitivity is observed even for a highly-symmetric molecule that lacks any unique atomic site.

Graphical abstract: Coincidence study of core-ionized adamantane: site-sensitivity within a carbon cage?

Article information

Article type
Paper
Submitted
22 Sept. 2022
Accepted
15 Nov. 2022
First published
17 Nov. 2022
This article is Open Access
Creative Commons BY-NC license

Phys. Chem. Chem. Phys., 2022,24, 28994-29003

Coincidence study of core-ionized adamantane: site-sensitivity within a carbon cage?

S. Ganguly, M. Gisselbrecht, P. Eng-Johnsson, R. Feifel, P. Hervieux, Z. Alfaytarouni, R. F. Fink, S. Díaz-Tendero, A. R. Milosavljević, P. Rousseau and S. Maclot, Phys. Chem. Chem. Phys., 2022, 24, 28994 DOI: 10.1039/D2CP04426A

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