Issue 40, 2021

MOF-based electrocatalysts for high-efficiency CO2 conversion: structure, performance, and perspectives

Abstract

Electroreduction of CO2 to produce chemicals and fuels is recognized as a promising technology to reduce greenhouse gas emissions, particularly by using renewable energy. In doing so, it is possible to achieve net-zero or negative emissions. A catalyst, however, is needed to facilitate the electroreduction of CO2 under ambient conditions. Recently, metal–organic frameworks (MOFs) and their derivatives have gained growing attention in materials research due largely to their high surface area, unique local chemical structures, and extraordinary properties. MOF-based electrocatalysts are of particular interest for CO2 conversion with high activity, selectivity, and stability. The intent of this article is to provide an overview of the structures and performances of these electrocatalysts, as well as the perspectives and future trends in this field.

Graphical abstract: MOF-based electrocatalysts for high-efficiency CO2 conversion: structure, performance, and perspectives

Article information

Article type
Review Article
Submitted
14 Jul 2021
Accepted
26 Seb 2021
First published
28 Seb 2021

J. Mater. Chem. A, 2021,9, 22710-22728

MOF-based electrocatalysts for high-efficiency CO2 conversion: structure, performance, and perspectives

X. Wang, M. Fan, Y. Guan, Y. Liu, M. Liu, T. N. V. Karsili, J. Yi, X. Zhou and J. Zhang, J. Mater. Chem. A, 2021, 9, 22710 DOI: 10.1039/D1TA05960B

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