Issue 7, 2020

Tailoring surface wetting states for ultrafast solar-driven water evaporation

Abstract

Solar-driven interfacial evaporation has significant potential to improve the energy utilization efficiency and provides a means for sustainable seawater desalination and water purification technologies. Although rational design of evaporative materials and surfaces is essential to the interfacial solar water vaporization process, tailoring the surface wettability states of solar evaporators to accelerate the vapor generation rate remains unexplored. Here we demonstrate hydrophilic hydrogel evaporators with hydrophobic island-shaped patches, capable of achieving a record evaporation rate of ∼4.0 kg m−2 h−1 with 93% efficiency under 1 sun irradiation (1 kW m−2). This exceptional high rate results from both wetting regions, which function synergistically. The increased thickness of the water layer in the hydrophilic region leads to the rapid escape of water molecules, while relatively long contact lines promise considerable water evaporation from the hydrophobic region, further contributing to this process. Molecular dynamics simulations provide a consistent outcome on a molecular basis, in which an inhomogeneous surface wetting property could modulate the escape behavior of water molecules to speed the evaporation. Under natural sunlight, a 3D printed portable solar water purification jug using this hydrogel evaporator delivers purified water far above the EPA drinking water standards, highlighting its potential for water purification.

Graphical abstract: Tailoring surface wetting states for ultrafast solar-driven water evaporation

Supplementary files

Article information

Article type
Paper
Submitted
07 فرؤری 2020
Accepted
05 مارٕچ 2020
First published
17 مارٕچ 2020

Energy Environ. Sci., 2020,13, 2087-2095

Tailoring surface wetting states for ultrafast solar-driven water evaporation

Y. Guo, X. Zhao, F. Zhao, Z. Jiao, X. Zhou and G. Yu, Energy Environ. Sci., 2020, 13, 2087 DOI: 10.1039/D0EE00399A

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