Issue 14, 2023

Strain-tunable skyrmions in two-dimensional monolayer Janus magnets

Abstract

The Dzyaloshinskii–Moriya interaction (DMI), which only exists in noncentrosymmetric systems, plays an important role in the formation of exotic chiral magnetic states. However, the absence of the DMI occurs in most two-dimensional (2D) magnetic materials due to their intrinsic inversion symmetry. Here, by using first-principles calculations, we demonstrate that a significant DMI can be obtained in a series of Janus monolayers of dichalcogenides XSeTe (X = Nb, Re) in which the difference between Se and Te on the opposite sides of X breaks the inversion symmetry. Remarkably, the DMI amplitudes of NbSeTe (1.78 meV) and ReSeTe (4.82 meV) are larger than the experimental value of Co/graphene (0.16 meV), and NbSeTe and ReSeTe monolayers have a high Curie temperature of 1023 K and 689 K, respectively. Through the micromagnetic simulation of XSeTe (X= Nb, Re) simulations, we also find that the ReSeTe monolayer can performance for skyrmion states by applying an external magnetic field, and importantly, the skyrmion states can be regulated and controlled under external strain. The findings pave the way for device concepts using chiral magnetic structures in specially designed 2D ferromagnetic materials.

Graphical abstract: Strain-tunable skyrmions in two-dimensional monolayer Janus magnets

Article information

Article type
Paper
Submitted
09 12 2022
Accepted
11 3 2023
First published
13 3 2023

Nanoscale, 2023,15, 6830-6837

Strain-tunable skyrmions in two-dimensional monolayer Janus magnets

Y. Han, W. Ji, P. Wang, P. Li and C. Zhang, Nanoscale, 2023, 15, 6830 DOI: 10.1039/D2NR06870B

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