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Abstract | Cited by

The two-electron reduced mixed-valence polyoxometalate [GeV14O40]8− presents an unusual paramagnetic behaviour as a consequence of the partial trapping of these electrons. The effect of applying an electric field is that of inducing antiferromagnetic coupling between the two delocalized electronic spins.

Graphical abstract: Modelling electric field control of the spin state in the mixed-valence polyoxometalate [GeV14O40]8−

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