Issue 7, 2020

Recycling lithium-ion batteries: adding value with multiple lives

Abstract

Resource extraction and limitations, valuable elements/minerals loss to land-fill, lack of recycling are growing concerns with increasing lithium-ion battery uptake and the synthesis of new cathodes (and more widely completely new materials for each battery). Factors such as these are exasperated in lithium-ion batteries which are currently one of the most expensive batteries to purchase and arguably are one of the most difficult to recycle efficiently. Herein, a mixed metal compound from the separation and processing of spent commercial batteries is compositionally, structurally, and electrochemically characterised as-received and sintered at temperatures up to 1000 °C. Whilst structural characterisation shows the significant presence of typical commercial layered cathode materials and their constituent elements via elemental analysis, this work shows that, without any further modifications to the as-received material, it is capable of delivering reversible capacities of over 300 mA h g−1 at 30 mA g−1 after 100 cycles as an anode in a “second-use” or “second-life” lithium-ion battery. Furthermore, the “second-life” lithium-ion battery has an increased intrinsic elemental value due to higher than normal concentrations of valuable metals (both in the fresh cathode and second-life anode) which can be extracted in future. This can be considered as an alternative approach to lithium-ion battery recycling.

Graphical abstract: Recycling lithium-ion batteries: adding value with multiple lives

Supplementary files

Article information

Article type
Paper
Submitted
21 Қаң. 2020
Accepted
09 Нау. 2020
First published
10 Нау. 2020

Green Chem., 2020,22, 2244-2254

Recycling lithium-ion batteries: adding value with multiple lives

J. Wu, A. Mackenzie and N. Sharma, Green Chem., 2020, 22, 2244 DOI: 10.1039/D0GC00269K

To request permission to reproduce material from this article, please go to the Copyright Clearance Center request page.

If you are an author contributing to an RSC publication, you do not need to request permission provided correct acknowledgement is given.

If you are the author of this article, you do not need to request permission to reproduce figures and diagrams provided correct acknowledgement is given. If you want to reproduce the whole article in a third-party publication (excluding your thesis/dissertation for which permission is not required) please go to the Copyright Clearance Center request page.

Read more about how to correctly acknowledge RSC content.

Social activity

Spotlight

Advertisements