Themed collection 2023 Frontier and Perspective articles
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Systematics of stable copper and silver clusters protected by small bite chelating bidentate sulfur and selenium ligands related to their polyhedral cavities: analogies to aliphatic compounds and three-dimensional spherical aromatic systems
Silver clusters composed exclusively of fused tetrahedra are analogous to simple saturated organic compounds. Copper clusters with central cuboctahedra and silver clusters with central icosahedra having interstitial metal atoms provide examples of metal superatoms.
Dalton Trans., 2024,53, 2895-2902
https://doi.org/10.1039/D3DT03998F
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Chemical Chartographisis: a contemporary perspective in molecular design and synthesis
We introduce a contemporary perspective in molecular design and synthesis, named "Chemical Chartographisis".
Dalton Trans., 2023,52, 18118-18132
https://doi.org/10.1039/D3DT02459H
Recent advances and prospects of metal–organic frameworks in cancer therapies
This paper presents the latest applications of MOFs in chemodynamic therapy (CDT), sonodynamic therapy (SDT), photodynamic therapy (PDT), photothermal therapy (PTT), immunotherapy (IT), and combination therapy for breast cancer.
Dalton Trans., 2023,52, 17601-17622
https://doi.org/10.1039/D3DT02543H
Thiol and thioether-based metal–organic frameworks: synthesis, structure, and multifaceted applications
Overview of thiol and thioether-based metal–organic frameworks.
Dalton Trans., 2023,52, 17623-17655
https://doi.org/10.1039/D3DT02884D
Decoding the puzzle: recent breakthroughs in understanding degradation mechanisms of Li-ion batteries
This review examines Li-ion battery degradation, with a focus on the cathode-electrolyte interphase (CEI), modification, modeling, and novel characterization tools for improved battery performance.
Dalton Trans., 2023,52, 17061-17083
https://doi.org/10.1039/D3DT02957C
Advances in the research of carbon electrodes for perovskite solar cells
Perovskite solar cells (PSCs) were first proposed in 2009.
Dalton Trans., 2023,52, 16558-16577
https://doi.org/10.1039/D3DT03136E
Recent advances in the nanoarchitectonics of metal–organic frameworks for light-activated tumor therapy
The application of nMOFs to antitumor therapy, including drug delivery strategies, photodynamic therapy (PDT), photothermal therapy (PTT), and combination therapy, is presented.
Dalton Trans., 2023,52, 16085-16102
https://doi.org/10.1039/D3DT02725B
Electron transfer catalysis mediated by 3d complexes of redox non-innocent ligands possessing an azo function: a perspective
The catalytic aspects of metal complexes of redox non-innocent azo ligands in achieving important and useful chemicals by a hassle-free and economical technique have been presented with in-depth mechanistic explications.
Dalton Trans., 2023,52, 15627-15646
https://doi.org/10.1039/D3DT02567E
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Elucidation of the electronic structures of thiolate-protected gold nanoclusters by electrochemical measurements
Electrochemical measurements can elucidate the electronic structures of metal nanoclusters and give deep insight into the electronic structure between the molecule and the metal.
Dalton Trans., 2023,52, 15152-15167
https://doi.org/10.1039/D3DT02005C
Copper trafficking systems in cells: insights into coordination chemistry and toxicity
This review describes the coordination chemistry of a copper trafficking system and the toxicity mechanisms arising from impaired copper homeostasis.
Dalton Trans., 2023,52, 15277-15296
https://doi.org/10.1039/D3DT02166A
A roadmap to enhance gas permselectivity in metal–organic framework-based mixed-matrix membranes
Metal–organic framework-based mixed-matrix membranes design strategies have been discussed with a focus on the challanges related to membrane fabrication, interface design, and gas diffusion pathways.
Dalton Trans., 2023,52, 15253-15276
https://doi.org/10.1039/D3DT01878D
Stepwise construction of multi-component metal–organic frameworks
This review outlines stepwise synthesis strategies for multi-component metal–organic frameworks, emphasizing their distinct advantages for gas adsorption, water remediation, heterogeneous catalysis, luminescence, and chemical sensing.
Dalton Trans., 2023,52, 15233-15252
https://doi.org/10.1039/D3DT01668D
Recent advances on the construction of long-wavelength emissive supramolecular coordination complexes for photo-diagnosis and therapy
Schematic diagram of the diagnosis and treatment of NIR-II emissive SCCs.
Dalton Trans., 2023,52, 15193-15202
https://doi.org/10.1039/D3DT01893H
Recent advances in porous molecular cages for photocatalytic organic conversions
Photocatalytic organic conversion is considered an efficient, environmentally friendly, and energy-saving strategy for organic synthesis. Porous molecular cages exhibit significant potential in the realm of photocatalytic organic conversion.
Dalton Trans., 2023,52, 15216-15232
https://doi.org/10.1039/D3DT01679J
Emerging enzyme-based nanocomposites for catalytic biomedicine
In this review, we discuss key aspects of enzyme-based catalytic biomedicine. We also highlighted the field's challenges and provided a prospect for the rational design and application of the enzyme-based nanocomposites.
Dalton Trans., 2023,52, 15203-15215
https://doi.org/10.1039/D3DT01381B
Olefin-linked covalent organic frameworks: synthesis and applications
In this review, we highlight the design principles, synthesis strategies, and impactful applications of olefin-linked covalent organic frameworks. Besides, the challenges and perspectives in this research field have been provided.
Dalton Trans., 2023,52, 15178-15192
https://doi.org/10.1039/D3DT01684F
Insights into the self-assembly of giant polyoxomolybdates from building blocks to supramolecular structures
Gaining an in-depth understanding of the self-assembly mechanism of giant polyoxomolybdates is the key for the designable clusters synthesis. This will in turn promote related supramolecular self-assembly and application research.
Dalton Trans., 2023,52, 15168-15177
https://doi.org/10.1039/D3DT00105A
Fluorescent and chromogenic organic probes to detect group 10 metal ions: design strategies and sensing applications
This study highlights various fluorescent and colorimetric organic sensors for detection of group 10 metal ions. Existing receptor design issues, challenges and promising development prospects are presented.
Dalton Trans., 2023,52, 14704-14732
https://doi.org/10.1039/D3DT01723K
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Cooperation towards nobility: equipping first-row transition metals with an aluminium sword
This perspective offers an overview of the state-of-the-art regarding heterobimetallic complexes featuring a bond between aluminium and a first-row transition metal. Their synthesis, reactivity and prospective catalytic applications are discussed.
Dalton Trans., 2023,52, 14259-14286
https://doi.org/10.1039/D3DT02722H
Room-temperature chemiresistive ammonia sensors based on 2D MXenes and their hybrids: recent developments and future prospects
This article offers a thorough overview of current advancements, potential applications and future improvement approaches for room-temperature ammonia sensors based on 2D MXene-based gas sensing technology.
Dalton Trans., 2023,52, 13831-13851
https://doi.org/10.1039/D3DT02401F
Recent advances of H-intercalated Pd-based nanocatalysts for electrocatalytic reactions
A comprehensive review in terms of the engineering and applications of Pd hydrides is summarized.
Dalton Trans., 2023,52, 13452-13466
https://doi.org/10.1039/D3DT02201C
Recent progress in trivalent europium (Eu3+)-based inorganic phosphors for solid-state lighting: an overview
Narrow band red-emitting phosphors are significant constituents but still a bottleneck for next-generation smart displays and high-performance lighting (solid-state lighting based white light-emitting diodes (WLEDs)) technology.
Dalton Trans., 2023,52, 13027-13057
https://doi.org/10.1039/D3DT00303E
Recent advances in oxidative catalytic applications of polyoxovanadate-based inorganic–organic hybrids
The oxidative catalytic applications of polyoxovanadate-based inorganic–organic hybrid (POVH) materials have been summarized for the transformation of organic compounds in this perspective article.
Dalton Trans., 2023,52, 12582-12596
https://doi.org/10.1039/D3DT02249H
Management of typical VOCs in air with adsorbents: status and challenges
The primary adsorption materials including activated carbon, zeolites and metal organic frameworks, and their modification methods are reviewed. The key factors controlling VOCs adsorption and the removal mechanisms are discussed.
Dalton Trans., 2023,52, 12169-12184
https://doi.org/10.1039/D3DT01930F
Recent progress in the stabilization of low band-gap black-phase iodide perovskite solar cells
This perspective presents a summary of diverse approaches used to stabilize the black phase of iodide perovskites, along with their practical implementation in photovoltaic devices.
Dalton Trans., 2023,52, 11750-11767
https://doi.org/10.1039/D3DT01581E
Engineering metallenes for boosting electrocatalytic biomass-oxidation-assisted hydrogen evolution reaction
A systematic review regarding the engineering of metallenes toward biomass-oxidation-assisted hydrogen evolution is presented.
Dalton Trans., 2023,52, 11378-11389
https://doi.org/10.1039/D3DT01562A
Interactions of Mn complexes with DNA: the relevance of therapeutic applications towards cancer treatment
Design of manganese-based drug conjugates for selective targeting of cancer cells will be a major breakthrough in the field of cancer research.
Dalton Trans., 2023,52, 10639-10656
https://doi.org/10.1039/D3DT00659J
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Atmospheric-pressure atomic layer deposition: recent applications and new emerging applications in high-porosity/3D materials
Atmospheric-pressure atomic layer deposition (ALD) is an upcoming technology poised to revolutionize the commercial production of large-area substrates and unlock new applications in high-porosity/3D materials.
Dalton Trans., 2023,52, 10254-10277
https://doi.org/10.1039/D3DT01204B
How does chemistry contribute to circular economy in nuclear energy systems to make them more sustainable and ecological?
Nuclear fuel recycling basically follows a concept of circular economy, while it actually suffers from several problems. This perspective discusses how chemistry works for resolving them as well as what task academic scientists should take on.
Dalton Trans., 2023,52, 9866-9881
https://doi.org/10.1039/D3DT01019H
Recent trends in phenol synthesis by photocatalytic oxidation of benzene
This perspective introduces current homogeneous and heterogeneous photocatalytic systems for phenol synthesis and outlines several strategies to enhance phenol selectivity.
Dalton Trans., 2023,52, 9525-9540
https://doi.org/10.1039/D3DT01360J
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Amidoboronates: bringing together the synthesis of BN-heterocycles via a reductive coupling and dynamic covalent chemistry
This Perspective discusses the synthesis of amidoboronates and the dynamic covalent chemistry of the C–C, B–N and B–O bonds.
Dalton Trans., 2023,52, 9189-9201
https://doi.org/10.1039/D3DT01863F
Stabilization of transition metal heterojunctions inside porous materials for high-performance catalysis
The developed strategies for stabilizing heterojunctions in different porous materials with improved synergistic effect, catalytic properties and stability are summarized and discussed.
Dalton Trans., 2023,52, 8834-8849
https://doi.org/10.1039/D3DT01020A
The enhanced sensing properties of MOS-based resistive gas sensors by Au functionalization: a review
Au-functionalized MOS-based gas sensing materials.
Dalton Trans., 2023,52, 8503-8529
https://doi.org/10.1039/D3DT01078C
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The quest for organo-alkali metal monomers: unscrambling the structure–reactivity relationship
This perspective explores the strategies that have been employed to isolate low aggregate and, in particular, monomeric complexes of the most common alkali metal alkyls and the relationship between aggregation, structure and reactivity.
Dalton Trans., 2023,52, 8172-8192
https://doi.org/10.1039/D3DT00980G
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Oligozwitterions in coordination polymers and frameworks – a structural view
Uranyl ion cluster formation about a trizwitterion.
Dalton Trans., 2023,52, 7772-7786
https://doi.org/10.1039/D3DT00849E
Engineering of metal–organic frameworks (MOFs) for thermometry
The construction of luminescent MOF and its thermometry application.
Dalton Trans., 2023,52, 7383-7404
https://doi.org/10.1039/D3DT01048A
Progress and prospects of dealloying methods for energy-conversion electrocatalysis
Developing hydrogen production and utilization technologies is a promising way to achieve large-scale applications of renewable energy.
Dalton Trans., 2023,52, 7370-7382
https://doi.org/10.1039/D3DT00449J
Transition metal complexes as self-activating chemical nucleases: proficient DNA cleavage without any exogenous redox agents
This perspective presents DNA cleavage via self-activation based on transition metal complexes employing copper, zinc and iron with their mechanistic investigation.
Dalton Trans., 2023,52, 6961-6977
https://doi.org/10.1039/D3DT00368J
Noncovalent tailoring of coordination complexes by resorcin[4]arene-based supramolecular hosts
Resorcin[4]arene-based molecular hosts can accommodate coordination complexes in a noncovalent manner to afford a unique host–guest systems, in which the chemical and physical properties of the guests are altered by encapsulation.
Dalton Trans., 2023,52, 6604-6618
https://doi.org/10.1039/D3DT00710C
Current status and prospects of MOFs in controlled delivery of Pt anticancer drugs
This review focuses on the application of platinum as an anticancer drug and the MOF materials loading platinum species; the prospect for its future development is also discussed.
Dalton Trans., 2023,52, 6226-6238
https://doi.org/10.1039/D3DT00413A
Light hydrocarbon conversion to acrylonitrile and acetonitrile – a review
Acrylonitrile can be produced by (i) propylene using a bismuth molybdate catalyst and (ii) propane using a MoVTeNb mixed oxide catalyst. Acetonitrile can be synthesized either from C2 (ethylene and ethane) using Co/HZSM-5 or C1 (methane) using solid-state-pyrolysis-made GaN.
Dalton Trans., 2023,52, 6211-6225
https://doi.org/10.1039/D2DT03795E
Addressing the gaps in homeostatic mechanisms of copper and copper dithiocarbamate complexes in cancer therapy: a shift from classical platinum-drug mechanisms
This review will focus on copper homeostasis in mammalian cells and on our current understanding of copper dysregulation in cancer and recent therapeutic breakthroughs using copper coordination complexes as anticancer drugs.
Dalton Trans., 2023,52, 5823-5847
https://doi.org/10.1039/D3DT00366C
Single-atom catalysts for catalytic benzene oxidation to phenol: recent progress and future perspectives
A comprehensive review with a particular focus on the significant roles of single atom sites and supports played in the substantial improvement of catalytic activity and selectivity towards the oxidation of benzene to phenol, is organized.
Dalton Trans., 2023,52, 5399-5417
https://doi.org/10.1039/D3DT00649B
Sn(IV)-porphyrinoids for photodynamic anticancer and antimicrobial chemotherapy
Research on recently reported Sn(IV) porphyrinoids, including corroles, chlorins and N-confused porphyrins, focusing primarily on their photodynamic therapy (PDT) and photodynamic antimicrobial chemotherapy (PACT) activity properties is reviewed.
Dalton Trans., 2023,52, 5000-5018
https://doi.org/10.1039/D3DT00603D
Polyoxotantalate chemistry: from synthetic strategies to structural diversity and applications
In this review, complexes including isopolyoxotantalates (IPOTas), organic–inorganic hybrid POTas, Ta/W mixed polyoxometalates and heteropolyoxotantalates (HPOTas) are introduced, in order to provide guidance for further exploration of intriguing POTas.
Dalton Trans., 2023,52, 4632-4642
https://doi.org/10.1039/D2DT03319D
Metal complexes with valuable biomolecules produced by Pseudomonas aeruginosa: a review of the coordination properties of pyocyanin, pyochelin and pyoverdines
A survey of the results achieved in the field of metal complexes with the natural products derived from Pseudomonas aeruginosa, namely pyocyanin, pyochelin, and pyoverdines, has been presented.
Dalton Trans., 2023,52, 4276-4289
https://doi.org/10.1039/D3DT00287J
Challenges and developments for the blue perovskite nanocrystal light-emitting diodes
The above figure is the thermal diagram of blue-light PeLEDs. From this diagram, it can be seen that the main research direction of blue-light LED is still efficiency and stability.
Dalton Trans., 2023,52, 3921-3941
https://doi.org/10.1039/D3DT00122A
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The effect of size, shape, coating and functionalization on nuclear relaxation properties in iron oxide core–shell nanoparticles: a brief review of the situation
Intrinsic parameters (magnetic core composition, size, shape, coating, and surface functionalization) and extrinsic parameters (solvent, magnetic field, and temperature) relevant for describing the nuclear relaxation in MNP core–shell nanoparticles are discussed.
Dalton Trans., 2023,52, 3551-3562
https://doi.org/10.1039/D2DT03387A
Precision syntheses of molecular necklaces based on coordination interactions
Precision syntheses and potential applications of molecular necklaces based on coordination interactions.
Dalton Trans., 2023,52, 2915-2923
https://doi.org/10.1039/D2DT03594D
Strategies to mitigate the shuttle effect in room temperature sodium–sulfur batteries: improving cathode materials
Challenges and insights into high-performance sulfur electrodes for optimizing RT-Na/S batteries are discussed.
Dalton Trans., 2023,52, 2548-2560
https://doi.org/10.1039/D3DT00008G
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Thermodynamics-based rules of thumb to evaluate the interaction of chelators and kinetically-labile metal ions in blood serum and plasma
Chelators and metal-ligand complexes can be stable or evolve in a biological system depending on thermodynamics and kinetics. For thermodynamic consideration the inclusion of all essential metals and metal-binding proteins is crucial.
Dalton Trans., 2023,52, 2197-2208
https://doi.org/10.1039/D2DT03875G
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Low-concentration CO2 capture using metal–organic frameworks – current status and future perspectives
Metal–organic frameworks with tailored pore sizes, structures and surface chemistry are promising sorbents for CO2 capture from low concentration CO2 sources.
Dalton Trans., 2023,52, 1841-1856
https://doi.org/10.1039/D2DT04088C
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Ferrocene-triazole conjugates: do we know why they are biologically active?
Using the click-chemistry approach, ferrocene has been linked to different organic structures of medicinal importance. Biologically active ferrocene-triazole conjugates, reported since 2012, are reviewed according to the type of their effect.
Dalton Trans., 2023,52, 1501-1517
https://doi.org/10.1039/D2DT03161B
Four-membered C^N chelation in main-group organometallic chemistry
This perspective deals with the synthesis, structure and applications of main-group organometallic compounds containing four-membered C^N chelation.
Dalton Trans., 2023,52, 1159-1176
https://doi.org/10.1039/D2DT03494H
Aiming for dynamic behaviours of molecular metal chains
This paper focuses on dynamic behaviors of the Pd chains supported by linear tetraphosphines, and current development on fine-tuning of metal chains by introducing heterometal atoms, which are considered promising dynamic components.
Dalton Trans., 2023,52, 1147-1158
https://doi.org/10.1039/D2DT03442E
Nanostructured mixed transition metal oxide spinels for supercapacitor applications
Illustration of the transition metal oxides considered and their supercapacitor studies.
Dalton Trans., 2023,52, 839-856
https://doi.org/10.1039/D2DT02733J
Pentagonal-bipyramidal 4d and 5d complexes with unquenched orbital angular momentum as a unique platform for advanced single-molecule magnets: current state and perspectives
Pentagonal-bipyramidal 4d3/5d3 complexes with unquenched orbital angular momentum are a unique platform for advanced single-molecule magnets due to anisotropic Ising-type exchange interactions, H = −Jxy(Sx5dSx3d + Sy5dSy3d) − JzSz5dSz3d.
Dalton Trans., 2023,52, 509-539
https://doi.org/10.1039/D2DT02954E
Introducing Te for boosting electrocatalytic reactions
Te-based nanocatalysts with multiple structures have been summarized for boosting electrocatalytic reactions.
Dalton Trans., 2023,52, 245-259
https://doi.org/10.1039/D2DT03253H
Anderson-type polyoxometalates for catalytic applications
Anderson-type polyoxometalates shown exceptional catalytic abilities. The unique combination of heteroatoms, organic grafting, and network immobilization gives a distinct advantage in catalytic performance.
Dalton Trans., 2023,52, 18133-18136
https://doi.org/10.1039/D3DT03274D
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Redox-active ligands – a viable route to reactive main group metal compounds
This article highlights studies that probe the oxidation/reduction of main group metal compounds possessing redox-active ligands and comments on the prospects for this relatively untapped avenue of research.
Dalton Trans., 2023,52, 17666-17678
https://doi.org/10.1039/D3DT03100D
Utility of all-pyrazole heteroscorpionates in f-element chemistry
A new generation of heteroscorpionates, known as all-pyrazole heteroscorpionates is dicussed as a platform for the generation of f-element compounds with robust structural diversity, desirable photoluminescent and molecular magnetism properties.
Dalton Trans., 2023,52, 17656-17665
https://doi.org/10.1039/D3DT02737F
Coordination polymers: a promising candidate for photo-responsive electronic device application
This study emphasizes recent advances in the designing of coordination polymers for photo-responsive electronic device applications in regard to crystal engineering aspects and structure–property relationship.
Dalton Trans., 2023,52, 17084-17098
https://doi.org/10.1039/D3DT02768F
Multivariate metal–organic frameworks generated through post-synthetic modification: impact and future directions
Reticular chemistry has proven to be invaluable over time, thanks to the structural versatility, and tailored porosity observed in structures like metal–organic frameworks (MOFs), covalent–organic frameworks (COFs), and metal–organic polyhedra (MOPs).
Dalton Trans., 2023,52, 16578-16585
https://doi.org/10.1039/D3DT01936E
Zeolite encapsulated organometallic complexes as model catalysts
Encapsulated complexes have potential as model heterogeneous catalysts for gap-phase reactions.
Dalton Trans., 2023,52, 16103-16112
https://doi.org/10.1039/D3DT02126B
The fascinating story of axial ligand dependent spectroscopy and redox-properties in iron(II) phthalocyanines
Iron phthalocyanines play crucial fundamental and applied roles ranging from bulk colorants to components of advanced materials. In this mini-review, we discuss the influence of axial ligand identity on spectroscopic and redox properties of iron(II) phthalocyanines.
Dalton Trans., 2023,52, 15647-15655
https://doi.org/10.1039/D3DT02565A
Cage-based sensors for circular dichroism analysis
Three-dimensional cages are promising platforms for chiral CD due to their stereochemical flexibility and cavity. In this minireview, we discuss recent advances, future challenges, and opportunities in the quantitative sensing of small molecules.
Dalton Trans., 2023,52, 15303-15312
https://doi.org/10.1039/D3DT02054A
Chemical bottom-up approach for inorganic single-atomic layers aiming beyond graphene
A chemical bottom-up approach for single-atomic-layered materials like graphene is attractive due to the possibility of introducing or tuning functions. This article focuses on the synthesis and properties of the inorganic layers.
Dalton Trans., 2023,52, 15297-15302
https://doi.org/10.1039/D3DT01636F
Hydrogen peroxide photo-fuel cells
H2O2-photofuel cell (PFC) is an important photoelectrochemical device contributing to the realization of a solar-driven clean energy cycle named the “hydrogen peroxide-keyed energy cycle” through combination with the photocatalytic H2O2 synthesis.
Dalton Trans., 2023,52, 14733-14741
https://doi.org/10.1039/D3DT02518G
Advances and opportunities in Group 15 porphyrin chemistry
The article summarizes recent advances in Group 15 porphyrin chemistry and attempts to unravel the tremendous opportunities of these remarkable porphyrins.
Dalton Trans., 2023,52, 14287-14296
https://doi.org/10.1039/D3DT02583G
Metal-ion doping in metal–organic-frameworks: modulating the electronic structure and local coordination for enhanced oxygen evolution reaction activity
Metal-ion doping modulates electronic structure and coordination environment in MOFs, leading to partial exposure of metal nodes, thus enhancing the active sites, and accelerating the OER.
Dalton Trans., 2023,52, 13852-13857
https://doi.org/10.1039/D3DT02405A
About this collection
This web collection contains the Frontier and Perspective articles published in Dalton Transactions in 2023.