Issue 4, 2022

Photoelectron spectroscopy in molecular physical chemistry

Abstract

Photoelectron spectroscopy has long been a powerful method in the toolbox of experimental physical chemistry and molecular physics. Recent improvements in coincidence methods, charged-particle imaging, and electron energy resolution have greatly expanded the variety of environments in which photoelectron spectroscopy can be applied, as well as the range of questions that can now be addressed. In this Perspectives Article, we focus on selected recent studies that highlight these advances and research areas. The topics include reactive intermediates and new thermochemical data, high-resolution comparisons of experiment and theory using methods based on pulsed-field ionisation (PFI), and the application of photoelectron spectroscopy as an analytical tool to monitor chemical reactions in complex environments, like model flames, catalytic or high-temperature reactors.

Graphical abstract: Photoelectron spectroscopy in molecular physical chemistry

Article information

Article type
Perspective
Submitted
01 11 2021
Accepted
05 1 2022
First published
05 1 2022

Phys. Chem. Chem. Phys., 2022,24, 1944-1959

Author version available

Photoelectron spectroscopy in molecular physical chemistry

I. Fischer and S. T. Pratt, Phys. Chem. Chem. Phys., 2022, 24, 1944 DOI: 10.1039/D1CP04984D

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