Positronium formation in dihydroxybenzenes

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Tomasz Goworek, Bożena Jasińska, Jan Wawryszczuk and Krzysztof Ciesielski


Abstract

Lifetime spectra of positrons in solid dihydroxybenzenes have been investigated over a wide range of temperatures. The variation of Ps formation probability with temperature and relative permittivity is an argument in favour of spur model concepts in the description of Ps formation in solids. An attempt to estimate the average excess electron–positron distance in the spur is undertaken. Detailed analysis of the e+ lifetime spectrum in hydroquinone indicates that the long-lived part of that spectrum can be a continuous distribution of lifetimes, not a discrete component.


References

  1. Positrons in Solids, ed. P. Hautojärvi, Springer Verlag, Berlin 1979 Search PubMed.
  2. O. E. Mogensen, J. Chem. Phys., 1974, 60, 998 CrossRef CAS.
  3. L. T. Bugayenko, V. M. Byakov and E. P. Kalazin, in Symposium on Radiation Chemistry of Aqueous Systems, Abstracts, Nauka, Moscow, 1973, p. 4 Search PubMed.
  4. O. E. Mogensen, Positron Annihilation in Chemistry, Springer Verlag, Berlin, 1995 Search PubMed.
  5. T. Goworek, B. Jasińska, J. Wawryszczuk and K. Ciesielski, J. Chem. Soc., Faraday Trans., 1996, 92, 1573 RSC.
  6. P. Kirkegaard, N. J. Pedersen and M. Eldrup, Risø Report M2740, Risø National Laboratory, Denmark, 1989.
  7. J. Kansy, Nucl. Instrum. Methods A., 1996, 374, 235 CrossRef CAS.
  8. D. Lightbody, J. N. Sherwood and M. Eldrup, Chem. Phys., 1985, 94, 475 CrossRef.
  9. B. Levay, M. Lalović and H. J. Ache, J. Chem. Phys., 1989, 90, 3282 CrossRef CAS.
  10. B. Jasińska, A. E. Kozioł and T. Goworek, J. Radioanal. Nucl. Chem., 1996, 210, 617 CAS.
  11. M. Eldrup, D. Lightbody and J. N. Sherwood, Chem. Phys., 1981, 63, 51 CrossRef CAS.
  12. S. J. Tao, Appl. Phys., 1976, 10, 67 Search PubMed.
  13. T. Shigenari, K. Abe, K. Morita, Qi. Qi Ping, E. Kojima and H. Ino, J. Phys. Condens. Matter, 1994, 6, 7469 CrossRef CAS.
  14. Y. Ebisuzaki, L. H. Askari, A. M. Bryan and M. F. Nicol, J. Chem. Phys., 1987, 87, 6659 CrossRef CAS.
  15. S. V. Stepanov and V. M. Byakov, J. Radioanal. Nucl. Chem., 1996, 210, 371 CAS.
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