Advances in Self-Powered Photodetectors: Unveiling the Potential of 2D Materials and Janus Heterostructures for a Promising Future in Next-Generation Optoelectronics

Abstract

Self-powered photodetectors (SPPDs) are becoming crucial in energy-efficient optoelectronics. They operate without external power, utilizing built-in electric fields and photovoltaic effects. Their applications range from wearable sensors to optical communication. Recent advancements in 2D materials, perovskites, Janus heterostructures, Schottky junctions, and flexible substrates have significantly improved responsivity, broadband absorption, and mechanical flexibility. However, challenges in stability, large-scale fabrication, and charge transport efficiency remain, hindering commercial adoption. This review critically examines recent progress in heterostructure-based SPPDs, addressing key challenges in device performance, material integration, and scalability. While previous research has explored individual material platforms, gaps remain in long-term stability, interface defects, and large-area processing. This study highlights the potential of novel fabrication techniques and doping strategies to enhance detection performance by analyzing advances in interface engineering, band alignment, and hybrid material systems. The results emphasize the promise of self-driven optimization, flexible electronics, and photodetectors based on quantum materials, providing valuable perspectives on the future trajectory of self-powered optoelectronics. This review highlights the existing challenges and opportunities, offering insights for future advancements in high-performance, self-sustaining photodetection technologies.