Self-healing materials in biomedicine and the circular economy

Meenakshi R. Venkateswaran, Arezoo Khosravi, Atefeh Zarepour, Siavash Iravani and Ali Zarrabi

Environ. Sci.: Nano, 2024, 11, 2771
DOI: 10.1039/D4EN00235K

Scalable assembly of micron boron nitride into high-temperature-resistant insulating papers with superior thermal conductivity

Meng-Xin Liu, Rui-Yu Ma, Zhi-Xing Wang, Zhuo-Yang Li, Gui-Lin Song, Jie Lin, Xin-Yuan Li, Ling Xu, Ding-Xiang Yan, Li-Chuan Jia and Zhong-Ming Li

Mater. Horiz., 2025, 12, 4349
DOI: 10.1039/D4MH01897D

A bio-inspired, ultra-tough, high-sensitivity, and anti-swelling conductive hydrogel strain sensor for motion detection and information transmission

Xiang Di, Jiawen Hou, Mingming Yang, Guolin Wu and Pingchuan Sun

Mater. Horiz., 2022, 9, 3057
DOI: 10.1039/D2MH00456A

Structure–property correlation of hydrogels obtained via radical polymerization using the central cores of multiarm star polymers as crosslinkers

Shohei Ida, Souma Suzuki, Shogo Toda, Hiroki Takeshita, Masatoshi Oyama, Keiji Nakajima and Shokyoku Kanaoka

Polym. Chem., 2025, 16, 1929
DOI: 10.1039/D5PY00014A

Bio-inspired multimimimetic synergistic strategies Cs3Bi2Br9/ZnS organosilicon antifouling flexible films: Coupled micro/nanostructured surfaces, fluorescence, and reactive oxygen species mechanisms

Mai Zhang, Zhirui Wang, Nan Zhou, Linlin Zhang, Jianjun Liao, Ping Zhang and Chengjun Ge

Materials Today Chemistry, 2024, 40, 102217
DOI: 10.1016/j.mtchem.2024.102217

Strong and Ultra-Tough Hydrogel with Hierarchical Cross-Linking Network Architecture Constructed by a Hyperbranched Topological Structure

Ying Zhu, Hanjing Zhang, Qinwen Tan, Yangfei Wu, Mengting Du, Nikos Hadjichristidis, Yu Jiang and Daohong Zhang

Macromolecules, 2025, 58, 6512
DOI: 10.1021/acs.macromol.5c00513

Multiple hydrogen-bonding induced nonconventional red fluorescence emission in hydrogels

Jiayu Wu, Yuhuan Wang, Pan Jiang, Xiaolong Wang, Xin Jia and Feng Zhou

Nat Commun, 2024, 15
DOI: 10.1038/s41467-024-47880-7

Self‐Healing Hydrogel Bioelectronics

Zhikang Li, Jijian Lu, Tian Ji, Yumeng Xue, Libo Zhao, Kang Zhao, Boqing Jia, Bin Wang, Jiaxiang Wang, Shiming Zhang and Zhuangde Jiang

Advanced Materials, 2024, 36
DOI: 10.1002/adma.202306350

An Autofluorescent Hydrogel with Water‐Dependent Emission for Dehydration‐Visualizable Smart Wearable Electronics

Yilei Wang, Hao Liu, Hui Xie and Shaobing Zhou

Adv Funct Materials, 2023, 33
DOI: 10.1002/adfm.202213545

Jellyfish-Inspired Self-Healing Luminescent Elastomers Based on Borate Nanoassemblies for Dual-Model Encryption

Bo Zhou, Xin Yang, Jize Liu, Lidan Lan, Hao Lu, Yuyan Wang, Zhenbo Wei and Xinxing Zhang

Nano Lett., 2024, 24, 8198
DOI: 10.1021/acs.nanolett.4c02512

Jellyfish‐Inspired Polyurea Ionogel with Mechanical Robustness, Self‐Healing, and Fluorescence Enabled by Hyperbranched Cluster Aggregates

Zhipeng Zhang, Lu Qian, Bin Zhang, Chunfeng Ma and Guangzhao Zhang

Angew Chem Int Ed, 2024, 63
DOI: 10.1002/anie.202410335

Promoting the Photoresponse Rate with Micelles in Hydrogels

Junheng Gao, Fu Tang, Yuting Li, Likang Zhang, An Hu, Shuo Li and Lidong Li

Advanced Optical Materials, 2025, 13
DOI: 10.1002/adom.202403352

Tough and self‐healable carrageenan‐based double network microgels enhanced physical hydrogels for strain sensor

Huan Sun, Shitong Li, Ke Li, Yanhua Liu, Cheng Tang, Zhuangzhuang Liu, Lin Zhu, Jia Yang, Gang Qin and Qiang Chen

Journal of Polymer Science, 2022, 60, 2720
DOI: 10.1002/pol.20210812

Boosting the performances of lithium metal batteries through in-situ construction of dual-network self-healing gel polymer electrolytes

Xiaoyi Chen, Lingguang Yi, Changfei Zou, Jiali Liu, Li Yang, Zihao Zang, Xiyuan Tao, Zhigao Luo, Baobao Chang, Yongqiang Shen and Xianyou Wang

Electrochimica Acta, 2023, 446, 142084
DOI: 10.1016/j.electacta.2023.142084

High-strength hydrogels: Fabrication, reinforcement mechanisms, and applications

Heyuan Huang, Zhicheng Dong, Xiaoyang Ren, Ben Jia, Guowei Li, Shaowen Zhou, Xin Zhao and Wenzhi Wang

Nano Res., 2023, 16, 3475
DOI: 10.1007/s12274-022-5129-1

High-Strength Anisotropic Fluorescent Hydrogel Based on Solvent Exchange for Patterning

Yanru Liu, Yali Li, Hui Liu, Shengsheng Yu, Shuanhong Ma, Ling-Bao Xing and Feng Zhou

ACS Appl. Mater. Interfaces, 2025, 17, 4114
DOI: 10.1021/acsami.4c16695

Self-Healing Hydrogels: From Synthesis to Multiple Applications

Hongyan Yin, Fangfei Liu, Tursun Abdiryim and Xiong Liu

ACS Materials Lett., 2023, 5, 1787
DOI: 10.1021/acsmaterialslett.3c00320

What Exactly Can Bionic Strategies Achieve for Flexible Sensors?

Hanpeng Gao, Fangyi Zhao, Jiaxi Liu, Zong Meng, Zhiwu Han and Yan Liu

ACS Appl. Mater. Interfaces, 2024, 16, 38811
DOI: 10.1021/acsami.4c06905

Micelle-Containing Hydrogels and Their Applications in Biomedical Research

Jinghua Wu, Huapeng Li, Nan Zhang and Qingfei Zheng

Gels, 2024, 10, 471
DOI: 10.3390/gels10070471

Stimuli-responsive hydrogels as promising platforms for soft actuators

Lizhi Chen, Fangfei Liu, Tursun Abdiryim and Xiong Liu

Materials Today Physics, 2024, 40, 101281
DOI: 10.1016/j.mtphys.2023.101281

Manipulating Toughness and Microstructure in Polyelectrolyte Complex Hydrogels with Competitive Surfactant Micelles

Jiawen Hou, Xiaoliang Wang, Pingchuan Sun and Fenfen Wang

Langmuir, 2025, 41, 986
DOI: 10.1021/acs.langmuir.4c04263

A Supramolecular Hydrogel Enabled by the Synergy of Hydrophobic Interaction and Quadruple Hydrogen Bonding

Liangmei Lu, Wen Zhou, Zhuzuan Chen, Yang Hu, Yu Yang, Guangzhao Zhang and Zhuohong Yang

Gels, 2022, 8, 244
DOI: 10.3390/gels8040244

Smart Hydrogels for Bone Reconstruction via Modulating the Microenvironment

Weikai Chen, Hao Zhang, Qirong Zhou, Fengjin Zhou, Qin Zhang and Jiacan Su

Research, 2023, 6
DOI: 10.34133/research.0089

Red Room Temperature Phosphorescence from Lignin

Hongda Guo, Huanjie Cheng, Ruixia Liu, Xiaoxia Chen, Luyao Wang, Chenhui Yang, Shujun Li, Shouxin Liu, Jian Li, Qingjiang Pan, Tony D. James and Zhijun Chen

Angewandte Chemie, 2025, 137
DOI: 10.1002/ange.202421112

Hydrogel fabrication techniques for advanced artificial sensory systems

Wonhee Gong, Jeongyeon Kim, Chaeyoon Kim, Hyewon Chang, Yejin Ahn, David V Schaffer and Jieung Baek

Int. J. Extrem. Manuf., 2025, 7, 062002
DOI: 10.1088/2631-7990/ade8b8

Intelligent electric energy driven ultrathin Graphene-Based Janus Films: Pioneering design for dynamic Electrochromism and superior microwave absorption

Tian Li, Jiatong Li, Zhengkang Xu, Jinzhe Li, Tinghao Liao, Jiani Du, Shanshan Wang, Qing Qi, Li Ma and Fanbin Meng

Chemical Engineering Journal, 2025, 506, 160008
DOI: 10.1016/j.cej.2025.160008

Physical strategies to engineer supramolecular composite hydrogels for advanced biomedical applications

Sravan Baddi, Auphedeous Y. Dang-i, Fengli Gao, Xiaxin Qiu and Chuanliang Feng

Progress in Materials Science, 2025, 151, 101428
DOI: 10.1016/j.pmatsci.2025.101428

Recyclable Dynamic Hydrogen Bonding and Disulfide Based Polymer‐Silver Nanoparticle Hybrid Triboelectric Nanogenerator for Artificial Intelligence‐Assisted High‐Precision Smart Insoles

Kaiming Zhang, Lixin Sun, Jiongyao Xu, Vinita Dhaware, Zhe Wang, Yiming Chen, Yahui Wu, Long Gu, Yuetao Liu and Richard Hoogenboom

Adv Funct Materials, 2025, 35
DOI: 10.1002/adfm.202501277

Cold-induced shape memory hydrogels for strong and programmable artificial muscles

Luqin Hua, Chuanzhuang Zhao, Xin Guan, Jianlei Lu and Jiawei Zhang

Sci. China Mater., 2022, 65, 2274
DOI: 10.1007/s40843-021-1971-9

A Biomimetic Soft Actuator Achieves Efficient Fluorescence via Covalent Cross‐Linking

Shijie Liao, Gaolei Dong, Bing Han, Junwen Wei, Yangdong Zhang, Yihao Guo, Tengfei Lin, Cong Lin, Chunlin Zhao, Min Gao, Xiao Wu, Na Wen, Hanliang Fan, Yinjie Zheng, Fei Gao and Xiaochun Zheng

Small, 2025
DOI: 10.1002/smll.202503597

Multifunctional Organohydrogel with Ultralow‐Hysteresis, Ultrafast‐Response, and Whole‐Strain‐Range Linearity for Self‐Powered Sensors

Jian Zou, Xin Jing, Zhuo Chen, Sheng‐Ji Wang, Xiang‐Shu Hu, Pei‐Yong Feng and Yue‐Jun Liu

Adv Funct Materials, 2023, 33
DOI: 10.1002/adfm.202213895

BSA‐Gold Nanoclusters Enhanced Clusterization‐Triggered–Emission of Nonconventional Luminophores‐Hydrogels in Dilute Aqueous Solution

Fengjiao Chen, Hao Dang, Hanlin Li, Hongbin Su, Liuxian Chen, Yao Gong, Lanxin Jiang, Hua Tang, Rui Chen and Wei Cheng

Adv Funct Materials, 2024, 34
DOI: 10.1002/adfm.202313098

3D Printable Active Hydrogels with Supramolecular Additive‐Driven Adaptiveness

Xiao Li, Zhecun Guan, Jiayu Zhao and Jinhye Bae

Small, 2024, 20
DOI: 10.1002/smll.202311164

Stability of Quadruple Hydrogen Bonds in an Ionic Liquid Environment

Chenming Li, Rajesh Bhandary, Anja Marinow, Stephanie Bachmann, Ann‐Christin Pöppler and Wolfgang H. Binder

Macromol. Rapid Commun., 2024, 45
DOI: 10.1002/marc.202300464

Smart hydrogel: A new platform for cancer therapy

Li Guo, Ziming Fu, Haoran Li, Ruibo Wei, Jing Guo, Haiwang Wang and Jian Qi

Advances in Colloid and Interface Science, 2025, 340, 103470
DOI: 10.1016/j.cis.2025.103470

Anthracene-based structural color films with luminescence enhancement, rapid patterning and wettability response for multi-dimensional encryption and anti-counterfeiting applications

Guoyi Pan, Jiaying Zhang, Jiaxin Li, Zilun Tang, Wenjing Lin, Xiaofeng Lin, Yingjuan Sun and Guobin Yi

Dyes and Pigments, 2026, 244, 113129
DOI: 10.1016/j.dyepig.2025.113129

Bioinspired Supramolecular Hydrogel from Design to Applications

Feng Gao, Xuhao Yang and Wenlong Song

Small Methods, 2024, 8
DOI: 10.1002/smtd.202300753

Self-Healing Behavior of Polymer/Protein Hybrid Hydrogels

Maria Bercea

Polymers, 2021, 14, 130
DOI: 10.3390/polym14010130

Red Room Temperature Phosphorescence from Lignin

Hongda Guo, Huanjie Cheng, Ruixia Liu, Xiaoxia Chen, Luyao Wang, Chenhui Yang, Shujun Li, Shouxin Liu, Jian Li, Qingjiang Pan, Tony D. James and Zhijun Chen

Angew Chem Int Ed, 2025, 64
DOI: 10.1002/anie.202421112

Microporous PdCuB nanotag-based electrochemical aptasensor with Au@CuCl2 nanowires interface for ultrasensitive detection of PD-L1-positive exosomes in the serum of lung cancer patients

Luyue Chang, Haiping Wu, Rui Chen, Xiaoqing Sun, Yi Yang, Changwu Huang, Shijia Ding, Changjin Liu and Wei Cheng

J Nanobiotechnol, 2023, 21
DOI: 10.1186/s12951-023-01845-y

Extended rubber-elasticity model for non-Gaussian isotropic hyperelasticity of polyelectrolyte hydrogels undergoing curl-to-stretch transition

Weilin Shi, Haibao Lu and Yong-Qing Fu

Phys. Scr., 2024, 99, 085954
DOI: 10.1088/1402-4896/ad5ca7

Jellyfish‐Inspired Artificial Spider Silk for Luminous Surgical Sutures

Kai Wen, Chao Zhang, Guanghao Zhang, Meilin Wang, Guangkai Mei, Zhenzhen Zhang, Weiqiang Zhao, Wenjin Guo, Qiang Zhou, Enzhao Liu, Yutian Zhu, Jie Bai, Meifang Zhu, Wei Wang, Zunfeng Liu and Xiang Zhou

Advanced Materials, 2024
DOI: 10.1002/adma.202314158

A supramolecular hydrogel leveraging hierarchical multi-strength hydrogen-bonds hinged strategy achieving a striking adhesive-mechanical balance

Jumin Yang, Wenguang Liu and Wei Wang

Bioactive Materials, 2025, 43, 32
DOI: 10.1016/j.bioactmat.2024.09.014

A Shift from Efficiency to Adaptability: Recent Progress in Biomimetic Interactive Soft Robotics in Wet Environments

Jielun Fang, Yanfeng Zhuang, Kailang Liu, Zhuo Chen, Zhou Liu, Tiantian Kong, Jianhong Xu and Cheng Qi

Advanced Science, 2022, 9
DOI: 10.1002/advs.202104347

Stimuli-responsive actuators in water environment: a review and future research agenda

Xin Zhao, Gangqiang Tang, Dong Mei, Chun Zhao, Lijie Li and Yanjie Wang

Int. J. Extrem. Manuf., 2025, 7, 022013
DOI: 10.1088/2631-7990/ad9fbb

Excitation-wavelength-dependent fluorescent organohydrogel for dynamic information anti-counterfeiting

Dong Guo, Xiaoxia Le, Hui Shang, Fuqing Shan, Danyang Li, Chunfa Ouyang and Tao Chen

Chinese Chemical Letters, 2023, 34, 108347
DOI: 10.1016/j.cclet.2023.108347

Jellyfish‐Inspired Polyurea Ionogel with Mechanical Robustness, Self‐Healing, and Fluorescence Enabled by Hyperbranched Cluster Aggregates

Zhipeng Zhang, Lu Qian, Bin Zhang, Chunfeng Ma and Guangzhao Zhang

Angewandte Chemie, 2024, 136
DOI: 10.1002/ange.202410335

Bioinspired Self‐healing Soft Electronics

Miao Qi, Ruiqi Yang, Zhe Wang, Yanting Liu, Qichong Zhang, Bing He, Kaiwei Li, Qing Yang, Lei Wei, Caofeng Pan and Mengxiao Chen

Adv Funct Materials, 2023, 33
DOI: 10.1002/adfm.202214479